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Considerable efforts have been recently devoted to combining ultracold atoms and nanophotonic devices to obtain not only better scalability and figures of merit than in free-space implementations, but also new paradigms for atom-photon interactions. Dielectric waveguides offer a promising platform for such integration because they enable tight transverse confinement of the propagating light, strong photon-atom coupling in single-pass configurations and potentially long-range atom-atom interactions mediated by the guided photons. However, the preparation of non-classical quantum states in such atom-waveguide interfaces has not yet been realized. Here, by using arrays of individual caesium atoms trapped along an optical nanofibre, we observe a single collective atomic excitation coupled to a nanoscale waveguide. The stored collective entangled state can be efficiently read out with an external laser pulse, leading to on-demand emission of a single photon into the guided mode. We characterize the emitted single photon via the suppression of the two-photon component and confirm the single character of the atomic excitation, which can be retrieved with an efficiency of about 25%. Our results demonstrate a capability that is essential for the emerging field of waveguide quantum electrodynamics, with applications to quantum networking, quantum nonlinear optics and quantum many-body physics.
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We study the dynamics of a single excitation coherently shared amongst an ensemble of atoms and coupled to a one-dimensional wave guide. The coupling between the matter and the light field gives rise to collective phenomena such as superradiant states with an enhanced initial decay rate, but also to the coherent exchange of the excitation between the atoms. We find that the competition between the two phenomena provides a characteristic dynamics for the decay of the excitations, and remarkably exhibits an algebraic behavior, instead of the expected standard exponential one, for a large number of atoms. The analysis is first performed for a chiral waveguide, where the problem can be solved analytically, and then is extended to the bidirectional waveguide.
Ordered atomic arrays trapped in the vicinity of nanoscale waveguides offer original light-matter interfaces, with applications to quantum information and quantum non-linear optics. Here, we study the decay dynamics of a single collective atomic excitation coupled to a waveguide in different configurations. The atoms are arranged as a linear array and only a segment of them is excited to a superradiant mode and emits light into the waveguide. Additional atomic chains placed on one or both sides play a passive role, either reflecting or absorbing this emission. We show that when varying the geometry, such a one-dimensional atomic system could be able to redirect the emitted light, to directionally reduce or enhance it, and in some cases to localize it in a cavity formed by the atomic mirrors bounding the system.
We experimentally and theoretically investigate collective radiative effects in an ensemble of cold atoms coupled to a single-mode optical nanofiber. Our analysis unveils the microscopic dynamics of the system, showing that collective interactions between the atoms and a single guided photon gradually build-up along the atomic array in the direction of propagation of light. These results are supported by time-resolved measurements of the light transmitted and reflected by the ensemble after excitation via nanofiber-guided laser pulses, whose rise and fall times are shorter than the atomic lifetime. Superradiant decays more than one order of magnitude faster than the single-atom free-space decay rate are observed for emission in the forward-propagating guided mode, while at the same time no speed-up of the decay rate are measured in the backward direction. In addition, position-resolved measurements of the light that is transmitted past the atoms are performed by inserting the nanofiber-coupled atomic array in a 45-m long fiber ring-resonator, which allow us to experimentally reveal the progressive growth of the collective response of the atomic ensemble. Our results highlight the unique opportunities offered by nanophotonic cold atom systems for the experimental investigation of collective light-matter interaction.
We study the cooperative optical coupling between regularly spaced atoms in a one-dimensional waveguide using decompositions to subradiant and superradiant collective excitation eigenmodes, direct numerical solutions, and analytical transfer-matrix methods. We illustrate how the spectrum of transmitted light through the waveguide including the emergence of narrow Fano resonances can be understood by the resonance features of the eigenmodes. We describe a method based on superradiant and subradiant modes to engineer the optical response of the waveguide and to store light. The stopping of light is obtained by transferring an atomic excitation to a subradiant collective mode with the zero radiative resonance linewidth by controlling the level shift of an atom in the waveguide. Moreover, we obtain an exact analytic solution for the transmitted light through the waveguide for the case of a regular lattice of atoms and provide a simple description how the light transmission may present large resonance shifts when the lattice spacing is close, but not exactly equal, to half of the wavelength of the light. Experimental imperfections such as fluctuations of the positions of the atoms and loss of light from the waveguide are easily quantified in the numerical simulations, which produce the natural result that the optical response of the atomic array tends toward the response of a gas with random atomic positions.
Planar nanostructures allow near-ideal extraction of emission from a quantum emitter embedded within, thereby realizing deterministic single-photon sources. Such a source can be transformed into M single-photon sources by implementing active temporal-to-spatial mode demultiplexing. We report on the realization of such a demultiplexed source based on a quantum dot embedded in a nanophotonic waveguide. Efficient outcoupling (>60%) from the waveguide into a single mode optical fiber is obtained with high-efficiency grating couplers. As a proof-of-concept, active demultiplexing into M=4 spatial channels is demonstrated by the use of electro-optic modulators with an end-to-end efficiency of >81% into single-mode fibers. Overall we demonstrate four-photon coincidence rates of >1 Hz even under non-resonant excitation of the quantum dot. The main limitation of the current source is the residual population of other exciton transitions that corresponds to a finite preparation efficiency of the desired transition. We quantitatively extract a preparation efficiency of 15% using the second-order correlation function measurements. The experiment highlights the applicability of planar nanostructures as efficient multiphoton sources through temporal-to-spatial demultiplexing and lays out a clear path way of how to scale up towards demonstrating quantum advantages with the quantum dot sources.
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