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Collective radiative dynamics of an ensemble of cold atoms coupled to an optical waveguide

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 Added by Riccardo Pennetta
 Publication date 2021
  fields Physics
and research's language is English




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We experimentally and theoretically investigate collective radiative effects in an ensemble of cold atoms coupled to a single-mode optical nanofiber. Our analysis unveils the microscopic dynamics of the system, showing that collective interactions between the atoms and a single guided photon gradually build-up along the atomic array in the direction of propagation of light. These results are supported by time-resolved measurements of the light transmitted and reflected by the ensemble after excitation via nanofiber-guided laser pulses, whose rise and fall times are shorter than the atomic lifetime. Superradiant decays more than one order of magnitude faster than the single-atom free-space decay rate are observed for emission in the forward-propagating guided mode, while at the same time no speed-up of the decay rate are measured in the backward direction. In addition, position-resolved measurements of the light that is transmitted past the atoms are performed by inserting the nanofiber-coupled atomic array in a 45-m long fiber ring-resonator, which allow us to experimentally reveal the progressive growth of the collective response of the atomic ensemble. Our results highlight the unique opportunities offered by nanophotonic cold atom systems for the experimental investigation of collective light-matter interaction.



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We study the dynamics of a single excitation coherently shared amongst an ensemble of atoms and coupled to a one-dimensional wave guide. The coupling between the matter and the light field gives rise to collective phenomena such as superradiant states with an enhanced initial decay rate, but also to the coherent exchange of the excitation between the atoms. We find that the competition between the two phenomena provides a characteristic dynamics for the decay of the excitations, and remarkably exhibits an algebraic behavior, instead of the expected standard exponential one, for a large number of atoms. The analysis is first performed for a chiral waveguide, where the problem can be solved analytically, and then is extended to the bidirectional waveguide.
Photons in a nonlinear medium can repel or attract each other, resulting in a strongly correlated quantum many-body system. Typically, such strongly correlated states of light arise from the extreme nonlinearity granted by quantum emitters that are strongly coupled to a photonic mode. However, in these approaches, unavoidable dissipation, like photon loss, blurs nonlinear quantum effects. Here, we generate strongly correlated photon states using only weak coupling and taking advantage of dissipation. We launch light through an ensemble of non-interacting waveguide-coupled atoms, which induce correlations between simultaneously arriving photons through collectively enhanced nonlinear interactions. These correlated photons then experience less dissipation than the uncorrelated ones. Depending on the number of atoms, we experimentally observe strong photon bunching or anti-bunching of the transmitted light. This realization of a collectively enhanced nonlinearity may turn out transformational for quantum information science and opens new avenues for generating nonclassical light, covering frequencies from the microwave to the X-ray regime.
Considerable efforts have been recently devoted to combining ultracold atoms and nanophotonic devices to obtain not only better scalability and figures of merit than in free-space implementations, but also new paradigms for atom-photon interactions. Dielectric waveguides offer a promising platform for such integration because they enable tight transverse confinement of the propagating light, strong photon-atom coupling in single-pass configurations and potentially long-range atom-atom interactions mediated by the guided photons. However, the preparation of non-classical quantum states in such atom-waveguide interfaces has not yet been realized. Here, by using arrays of individual caesium atoms trapped along an optical nanofibre, we observe a single collective atomic excitation coupled to a nanoscale waveguide. The stored collective entangled state can be efficiently read out with an external laser pulse, leading to on-demand emission of a single photon into the guided mode. We characterize the emitted single photon via the suppression of the two-photon component and confirm the single character of the atomic excitation, which can be retrieved with an efficiency of about 25%. Our results demonstrate a capability that is essential for the emerging field of waveguide quantum electrodynamics, with applications to quantum networking, quantum nonlinear optics and quantum many-body physics.
We experimentally demonstrate a ring geometry all-fiber cavity system for cavity quantum electrodynamics with an ensemble of cold atoms. The fiber cavity contains a nanofiber section which mediates atom-light interactions through an evanescent field. We observe well-resolved, vacuum Rabi splitting of the cavity transmission spectrum in the weak driving limit due to a collective enhancement of the coupling rate by the ensemble of atoms within the evanescent field, and we present a simple theoretical model to describe this. In addition, we demonstrate a method to control and stabilize the resonant frequency of the cavity by utilizing the thermal properties of the nanofiber.
Systems consisting of cold atoms trapped near photonic crystal waveguides have recently emerged as an exciting platform for quantum atom-light interfaces. Such a system enables realization of tunable long-range interactions between internal states of atoms (spins), mediated by guided photons. Currently, experimental platforms are still limited by low filling fractions, where the atom number is much smaller than the number of sites at which atoms can potentially be trapped. Here, we show that this regime in fact enables interesting many-body quantum phenomena, which are typically associated with short-range disordered systems. As an example, we show how the system can realize the so-called random singlet phase, in which all atoms pair into entangled singlets, but the pairing occurs over a distribution of ranges as opposed to nearest neighbors. We use a renormalization group method to obtain the distribution of spin entanglement in the random singlet phase, and show how this state can be approximately reached via adiabatic evolution from the ground state of a non-interacting Hamiltonian. We also discuss how experimentally this random singlet phase can be observed. We anticipate that this work will accelerate the route toward the exploration of strongly correlated matter in atom-nanophotonics interfaces, by avoiding the requirement of perfectly filled lattices.
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