No Arabic abstract
High pressure xenon Time Projection Chambers (TPC) based on secondary scintillation (electroluminescence) signal amplification are being proposed for rare event detection such as directional dark matter, double electron capture and double beta decay detection. The discrimination of the rare event through the topological signature of primary ionisation trails is a major asset for this type of TPC when compared to single liquid or double-phase TPCs, limited mainly by the high electron diffusion in pure xenon. Helium admixtures with xenon can be an attractive solution to reduce the electron diffusion significantly, improving the discrimination efficiency of these optical TPCs. We have measured the electroluminescence (EL) yield of Xe-He mixtures, in the range of 0 to 30% He and demonstrated the small impact on the EL yield of the addition of helium to pure xenon. For a typical reduced electric field of 2.5 kV/cm/bar in the scintillation region, the EL yield is lowered by ~ 2%, 3%, 6% and 10% for 10%, 15%, 20% and 30% of helium concentration, respectively. This decrease is less than what has been obtained from the most recent simulation framework in the literature. The impact of the addition of helium on EL statistical fluctuations is negligible, within the experimental uncertainties. The present results are an important benchmark for the simulation tools to be applied to future optical TPCs based on Xe-He mixtures.
The krypton electroluminescence yield was studied, at room temperature, as a function of electric field in the gas scintillation gap. A large area avalanche photodiode has been used to allow the simultaneous detection of the electroluminescence pulses as well as the direct interaction of x-rays, the latter being used as a reference for the calculation of the number of charge carriers produced by the electroluminescence pulses and, thus, the determination of the number of photons impinging the photodiode. An amplification parameter of 113 photons per kV per drifting electron and a scintillation threshold of 2.7 Td ( 0.7 kV/cm/bar at 293 K ) was obtained, in good agreement with the simulation data reported in the literature. On the other hand, the ionisation threshold in krypton was found to be around 13.5 Td (3.4 kV/cm/bar), less than what had been obtained by the most recent simulation work-package. The krypton amplification parameter is about 80% and 140% of those measured for xenon and argon, respectively. The electroluminescence yield in krypton is of great importance for modeling krypton-based double-phase or high-pressure gas detectors, which may be used in future rare event detection experiments.
We have measured the electroluminescence (EL) yield of Xe-CO2 mixtures, with sub-percent CO2 concentrations. We demonstrate that the EL production is still high in these mixtures, 70% and 35% relative to that produced in pure xenon, for CO2 concentrations around 0.05% and 0.1%, respectively. The contribution of the statistical fluctuations in EL production to the energy resolution increases with increasing CO2 concentration and, for our gas proportional scintillation counter, it is smaller than the contribution of the Fano factor for concentrations below 0.1% CO2. Xe-CO2 mixtures are important alternatives to pure xenon in TPCs based on EL signal amplification with applications in the important field of rare event detection such as directional dark matter, double electron capture and double beta decay detection. The addition of CO2 to pure xenon at the level of 0.05-0.1% can reduce significantly the scale of electron diffusion from 10 mm/sqrt(m) to 2.5 mm/sqrt(m), with high impact on the HPXe TPC discrimination efficiency of the events through pattern recognition of the topology of primary ionisation trails.
Inductively Coupled Plasma Mass Spectrometry (ICP-MS) allows for rapid, high-sensitivity determination of trace impurities, notably the primordial radioisotopes $^{238}$U and $^{232}$Th, in candidate materials for low-background rare-event search experiments. We describe the setup and characterisation of a dedicated low-background screening facility at University College London where we operate an Agilent 7900 ICP-MS. The impact of reagent and carrier gas purity is evaluated and we show that twice-distilled ROMIL-SpA-grade nitric acid and zero-grade Ar gas delivers similar sensitivity to ROMIL-UpA-grade acid and research grade gas. A straightforward procedure for sample digestion and analysis of materials with U/Th concentrations down to 10 ppt g/g is presented. This includes the use of $^{233}$U and $^{230}$Th spikes to correct for signal loss from a range of sources and verification of $^{238}$U and $^{232}$Th recovery through digestion and analysis of a certified reference material with a complex sample matrix. Finally, we demonstrate assays and present results from two sample preparation and assay methods: a high-sensitivity measurement of ultra-pure Ti using open digestion techniques, and a closed vessel microwave digestion of a nickel-chromium-alloy using a multi-acid mixture.
The aim of the presented work was to develop further techniques based on a Micromegas-TPC, in order to reach a high gas gain with good energy resolution, and to search for gas mixtures suitable for rare event detection. This paper focuses on xenon, which is convenient for the search of neutrinoless double beta decay in 136 Xe. Conversely, a small admixture of xenon to CF 4 can reduce attachment in the latter. This gas mixture would be suitable for dark matter searches and the study of solar and reactor neutrinos. Various configurations of the Micromegas plane were investigated and are described.
Type 5A molecular sieves (MS) have been demonstrated to remove radon from SF$_6$ gas. This is important for ultra-sensitive SF$_6$ gas-based directional dark matter and related rare-event physics experiments, as radon can provide a source of unwanted background events. Unfortunately, commercially available sieves intrinsically emanate radon at levels not suitable for ultra-sensitive physics experiments. A method to produce a low radioactive MS has been developed in Nihon University (NU). In this work, we explore the feasibility of the NU-developed 5A type MS for use in such experiments. A comparison with a commercially available Sigma-Aldrich 5A type MS was made. The comparison was done by calculating a parameter indicating the amount of radon intrinsically emanated by the MS per unit radon captured from SF$_6$ gas. The measurements were made using a specially adapted DURRIDGE RAD7 radon detector. The NU-developed 5A MS emanated radon up to 61$pm$9$%$ less per radon captured (2.1$pm$0.1)$times 10^{-3}$, compared to the commercial Sigma-Aldrich MS (5.4$pm$0.4)$times 10^{-3}$, making it a better candidate for use in a radon filtration setup for future ultra-sensitive SF$_6$ gas based experiments.