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Register a new userSupersolid symmetry breaking from compressional oscillations in a dipolar quantum gas
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The existence of a paradoxical supersolid phase of matter, possessing the apparently incompatible properties of crystalline order and superfluidity, was predicted 50 years ago. Solid helium was the natural candidate, but there supersolidity has not been observed yet, despite numerous attempts. Ultracold quantum gases have recently shown the appearance of the periodic order typical of a crystal, due to various types of controllable interactions. A crucial feature of a D-dimensional supersolid is the occurrence of up to D+1 gapless excitations reflecting the Goldstone modes associated with the spontaneous breaking of two continuous symmetries: the breaking of phase invariance, corresponding to the locking of the phase of the atomic wave functions at the origin of superfluid phenomena, and the breaking of translational invariance due to the lattice structure of the system. The occurrence of such modes has been the object of intense theoretical investigations, but their experimental observation is still missing. Here we demonstrate the supersolid symmetry breaking through the appearance of two distinct compressional oscillation modes in a harmonically trapped dipolar Bose-Einstein condensate, reflecting the gapless Goldstone excitations of the homogeneous system. We observe that the two modes have different natures, with the higher frequency mode associated with an oscillation of the periodicity of the emergent lattice and the lower one characterizing the superfluid oscillations. Our work paves the way to explore the two quantum phase transitions between the superfluid, supersolid and solid-like configurations that can be accessed by tuning a single interaction parameter.
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Distintictive features of supersolids show up in their rotational properties. We calculate the moment of inertia of a harmonically trapped dipolar Bose-Einstein condensed gas as a function of the tunable scattering length parameter, providing the transition from the (fully) superfluid to the supersolid phase and eventually to an incoherent crystal of self-bound droplets. The transition from the superfluid to the supersolid phase is characterized by a jump in the moment on inertia, revealing its first order nature. In the case of elongated trapping in the plane of rotation we show that the the moment of inertia determines the value of the frequency of the scissors mode, which is significantly affected by the reduction of superfluidity in the supersolid phase. The case of isotropic trapping is instead well suited to study the formation of quantized vortices, which are shown to be characterized, in the supersolid phase, by a sizeable deformed core, caused by the presence of the sorrounding density peaks.
By combining theory and experiments, we demonstrate that dipolar quantum gases of both $^{166}$Er and $^{164}$Dy support a state with supersolid properties, where a spontaneous density modulation and a global phase coherence coexist. This paradoxical state occurs in a well defined parameter range, separating the phases of a regular Bose-Einstein condensate and of an insulating droplet array, and is rooted in the roton mode softening, on the one side, and in the stabilization driven by quantum fluctuations, on the other side. Here, we identify the parameter regime for each of the three phases. In the experiment, we rely on a detailed analysis of the interference patterns resulting from the free expansion of the gas, quantifying both its density modulation and its global phase coherence. Reaching the phases via a slow interaction tuning, starting from a stable condensate, we observe that $^{166}$Er and $^{164}$Dy exhibit a striking difference in the lifetime of the supersolid properties, due to the different atom loss rates in the two systems. Indeed, while in $^{166}$Er the supersolid behavior only survives a few tens of milliseconds, we observe coherent density modulations for more than $150,$ms in $^{164}$Dy. Building on this long lifetime, we demonstrate an alternative path to reach the supersolid regime, relying solely on evaporative cooling starting from a thermal gas.
In the short time since the first observation of supersolid states of ultracold dipolar atoms, substantial progress has been made in understanding the zero-temperature phase diagram and low-energy excitations of these systems. Less is known, however, about their finite-temperature properties, particularly relevant for supersolids formed by cooling through direct evaporation. Here, we explore this realm by characterizing the evaporative formation and subsequent decay of a dipolar supersolid by combining high-resolution in-trap imaging with time-of-flight observables. As our atomic system cools towards quantum degeneracy, it first undergoes a transition from thermal gas to a crystalline state with the appearance of periodic density modulation. This is followed by a transition to a supersolid state with the emergence of long-range phase coherence. Further, we explore the role of temperature in the development of the modulated state.
We present an experimental and theoretical study of the high-energy excitation spectra of a dipolar supersolid. Using Bragg spectroscopy, we study the scattering response of the system to a high-energy probe, enabling measurements of the dynamic structure factor. We experimentally observe a continuous reduction of the response when tuning the contact interaction from an ordinary Bose-Einstein condensate to a supersolid state. Yet the observed reduction is faster than the one theoretically predicted by the Bogoliubov-de-Gennes theory. Based on an intuitive semi-analytic model and real-time simulations, we primarily attribute such a discrepancy to the out-of-equilibrium phase dynamics, which although not affecting the system global coherence, reduces its response.
Motivated by a recent experiment [L.Chomaz et al., Nature Physics 14, 442 (2018)], we perform numerical simulations of a dipolar Bose-Einstein Condensate (BEC) in a tubular confinement at T=0 within Density Functional Theory, where the beyond-mean-field correction to the ground state energy is included in the Local Density Approximation. We study the excitation spectrum of the system by solving the corresponding Bogoliubov-de Gennes equations. The calculated spectrum shows a roton minimum, and the roton gap decreases by reducing the effective scattering length. As the roton gap disappears, the system spontaneously develops in its ground-state a periodic, linear structure formed by denser clusters of atomic dipoles immersed in a dilute superfluid background. This structure shows the hallmarks of a supersolid system, i.e. (i) a finite non-classical translational inertia along the tube axis and (ii) the appearance, besides the phonon mode, of the Nambu-Goldstone gapless mode corresponding to phase fluctuations, and related to the spontaneous breaking of the gauge symmetry. A further decrease in the scattering length eventually leads to the formation of a periodic linear array of self-bound droplets.
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