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Register a new userSlow interaction quench in BCS superconductors: emergence of pre-formed pairs
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Added by
Jean-Sebastien Bernier
Publication date
2019
fields
Physics
and research's language is
English
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We investigate the non-equilibrium behavior of BCS superconductors subjected to slow ramps of their internal interaction strength. We identify three dynamical regimes as a function of ramp duration. For short ramp times, these systems become non-superconducting; however, fermions with opposite momenta remain paired albeit with reduced amplitudes, and the associated pair amplitude distribution is non-thermal. In this first regime, the disappearance of superconductivity is due to the loss of phase coherence between pairs. By contrast, for intermediate ramp times, superconductivity survives but the magnitude of the order parameter is reduced and presents long-lived oscillations. Finally, for long ramp times, phase coherence is almost fully retained during the slow interaction quench, and the steady-state is characterized by a thermal-like pair amplitude distribution. Using this approach, one can therefore dynamically tune the coherence between pairs in order to control the magnitude of the superconducting order parameter and even engineer a non-equilibrium state made of pre-formed pairs.
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The physics of the crossover between weak-coupling Bardeen-Cooper-Schrieffer (BCS) and strong-coupling Bose-Einstein-condensate (BEC) limits gives a unified framework of quantum bound (superfluid) states of interacting fermions. This crossover has been studied in the ultracold atomic systems, but is extremely difficult to be realized for electrons in solids. Recently, the superconducting semimetal FeSe with a transition temperature $T_{rm c}=8.5$ K has been found to be deep inside the BCS-BEC crossover regime. Here we report experimental signatures of preformed Cooper pairing in FeSe below $T^*sim20$ K, whose energy scale is comparable to the Fermi energies. In stark contrast to usual superconductors, large nonlinear diamagnetism by far exceeding the standard Gaussian superconducting fluctuations is observed below $T^*sim20$ K, providing thermodynamic evidence for prevailing phase fluctuations of superconductivity. Nuclear magnetic resonance (NMR) and transport data give evidence of pseudogap formation at $sim T^*$. The multiband superconductivity along with electron-hole compensation in FeSe may highlight a novel aspect of the BCS-BEC crossover physics.
We study the quench dynamics of a topological $p$-wave superfluid with two competing order parameters, $Delta_pm(t)$. When the system is prepared in the $p+ip$ ground state and the interaction strength is quenched, only $Delta_+(t)$ is nonzero. However, we show that fluctuations in the initial conditions result in the growth of $Delta_-(t)$ and chaotic oscillations of both order parameters. We term this behavior phase III. In addition, there are two other types of late time dynamics -- phase I where both order parameters decay to zero and phase II where $Delta_+(t)$ asymptotes to a nonzero constant while $Delta_-(t)$ oscillates near zero. Although the model is nonintegrable, we are able to map out the exact phase boundaries in parameter space. Interestingly, we find phase III is unstable with respect to breaking the time reversal symmetry of the interaction. When one of the order parameters is favored in the Hamiltonian, the other one rapidly vanishes and the previously chaotic phase III is replaced by the Floquet topological phase III that is seen in the integrable chiral $p$-wave model.
We present resistivity and thermal-conductivity measurements of superconducting FeSe in intense magnetic fields up to 35 T applied parallel to the $ab$ plane. At low temperatures, the upper critical field $mu_0 H_{c2}^{ab}$ shows an anomalous upturn, while thermal conductivity exhibits a discontinuous jump at $mu_0 H^{ast}approx 24$ T well below $mu_0 H_{c2}^{ab}$, indicating a first-order phase transition in the superconducting state. This demonstrates the emergence of a distinct field-induced superconducting phase. Moreover, the broad resistive transition at high temperatures abruptly becomes sharp upon entering the high-field phase, indicating a dramatic change of the magnetic-flux properties. We attribute the high-field phase to the Fulde-Ferrel-Larkin-Ovchinnikov (FFLO) state, where the formation of planar nodes gives rise to a segmentation of the flux-line lattice. We point out that strongly orbital-dependent pairing as well as spin-orbit interactions, the multiband nature, and the extremely small Fermi energy are important for the formation of the FFLO state in FeSe.
Superconductivity arises from two distinct quantum phenomena: electron pairing and long-range phase coherence. In conventional superconductors, the two quantum phenomena generally take place simultaneously, while the electron pairing occurs at higher temperature than the long-range phase coherence in the underdoped high-Tc cuprate superconductors. Recently, whether electron pairing is also prior to long-range phase coherence in single-layer FeSe film on SrTiO3 substrate is under debate. Here, by measuring Knight shift and nuclear spin-lattice relaxation rate, we unambiguously reveal a pseudogap behavior below Tp ~ 60 K in two layered FeSe-based superconductors with quasi-two-dimension. In the pseudogap regime, a weak diamagnetic signal and a remarkable Nernst effect are also observed, which indicate that the observed pseudogap behavior is related to superconducting fluctuations. These works confirm that strong phase fluctuation is an important character in the two-dimensional iron-based superconductors as widely observed in high-Tc cuprate superconductors.
We theoretically show that a two-band system with very different masses harbors a resonant pair scattering that leads to novel pairing properties, as highlighted by the Bardeen-Cooper-Schrieffer (BCS) to Bose-Einstein condensation (BEC) crossover. Most importantly, the interband pair-exchange coupling induces an effective intraband attraction in each band, enhancing the superfluidity/superconductivity. The effect, a kind of Suhl-Kondo mechanism, is specifically enhanced when the second band has a heavy mass and is incipient (lying close to, but just above, the chemical potential, $mu$), which we call a resonant pair scattering. By elucidating the dependence of the effective interactions and gap functions on $mu$, we can draw an analogy between the resonant pair scattering and the Feshbach resonance.
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