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Register a new userDilute magnetism in graphene
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The phase diagram of graphene decorated with magnetic adatoms distributed either on a single sublattice, or evenly over the two sublattices, is computed for adatom concentrations as low as $sim1%$. Within the framework of the $s$-$d$ interaction, we take into account disorder effects due to the random positioning of the adatoms and/or to the thermal fluctuations in the direction of magnetic moments. Despite the presence of disorder, the magnetic phases are shown to be stable down to the lowest concentration accessed here. This result agrees with several experimental observations where adatom decorated graphene has been shown to have a magnetic response. In particular, the present theory provides a qualitative understanding for the results of Hwang et al. [Sci. Rep. 6, 21460 (2016)], where a ferromagnetic phase has been found below $sim30,text{K}$ for graphene decorated with S-atoms.
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Magnetism in single-side hydrogenated (C$_2$H) and fluorinated (C$_2$F) graphene is analyzed in terms of the Heisenberg model with parameters determined from first principles. We predict a frustrated ground state for both systems, which means the instability of collinear spin structures and sheds light on the absence of a conventional magnetic ordering in defective graphene demonstrated in recent experiments. Moreover, our findings suggest a highly correlated magnetic behavior at low temperatures offering the possibility of a spin-liquid state.
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We discuss the conditions under which the predicted (but not yet observed) zero-field interlayer excitonic condensation in double layer graphene has a critical temperature high enough to allow detection. Crucially, disorder arising from charged impurities and corrugation in the lattice structure --- invariably present in all real samples --- affects the formation of the condensate via the induced charge inhomogeneity. In the former case, we use a numerical Thomas-Fermi-Dirac theory to describe the local fluctuations in the electronic density in double layer graphene devices and estimate the effect these realistic fluctuations have on the formation of the condensate. To make this estimate, we calculate the critical temperature for the interlayer excitonic superfluid transition within the mean-field BCS theory for both optimistic (unscreened) and conservative (statically screened) approximations for the screening of the interlayer Coulomb interaction. We also estimate the effect of allowing dynamic contributions to the interlayer screening. We then conduct similar calculations for double quadratic bilayer graphene, showing that the quadratic nature of the low-energy bands produces pairing with critical temperature of the same order of magnitude as the linear bands of double monolayer graphene.
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