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Register a new userA coupled harmonic oscillator model to describe the near-field radiative heat transfer between nanoparticles and planar surfaces
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Added by
Karthik Sasihithlu Dr
Publication date
2018
fields
Physics
and research's language is
English
Authors
Karthik Sasihithlu
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When two objects made of a material which supports surface modes are brought in close proximity to each other such that the vacuum gap between them is less than the thermal wavelength of radiation, then the coupling between the surface modes provides an important channel for the heat transfer to occur which is different from that mediated by long range propagating electromagnetic waves. Indeed, the heat transfer then exceeds Plancks blackbody limit by several orders of magnitude, and consequently has been used for several energy applications such as near-field thermophotovoltaic systems. This near-field radiative heat exchange has been traditionally and successfully described using fluctuational electrodynamics principles. Here, we describe an alternate coupled harmonic oscillator model approach which can be used to model the coupling between surface modes and hence the resultant near-field heat transfer. We apply this theory to estimate the near-field heat transfer for the configurations of two metallic nanoparticles and two planar metal surfaces and compare the result with predictions from fluctuational electrodynamics theory.
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We study the interplay of conductive and radiative heat transfer (RHT) in planar geometries and predict that temperature gradients induced by radiation can play a significant role on the behavior of RHT with respect to gap sizes, depending largely on geometric and material parameters and not so crucially on operating temperatures. Our findings exploit rigorous calculations based on a closed-form expression for the heat flux between two plates separated by vacuum gaps $d$ and subject to arbitrary temperature profiles, along with an approximate but accurate analytical treatment of coupled conduction--radiation in this geometry. We find that these effects can be prominent in typical materials (e.g. silica and sapphire) at separations of tens of nanometers, and can play an even larger role in metal oxides, which exhibit moderate conductivities and enhanced radiative properties. Broadly speaking, these predictions suggest that the impact of RHT on thermal conduction, and vice versa, could manifest itself as a limit on the possible magnitude of RHT at the nanoscale, which asymptotes to a constant (the conductive transfer rate when the gap is closed) instead of diverging at short separations.
The dynamic heat transfer between two half-spaces separated by a vacuum gap due to coupling of their surface modes is modelled using the theory that describes the dynamic energy transfer between two coupled harmonic oscillators each separately connected to a heat bath and with the heat baths maintained at different temperatures. The theory is applied for the case when the two surfaces are made up of a polar crystal which supports surface polaritons that can be excited at room temperature and the predicted heat transfer is compared with the steady state heat transfer value calculated from standard fluctuational electrodynamics theory. It is observed that for small time intervals the value of heat flux can reach as high as 1.5 times that of steady state value.
Extreme near-field heat transfer between metallic surfaces is a subject of debate as the state-of-the-art theory and experiments are in disagreement on the energy carriers driving heat transport. In an effort to elucidate the physics of extreme near-field heat transfer between metallic surfaces, this Letter presents a comprehensive model combining radiation, acoustic phonon and electron transport across sub-10-nm vacuum gaps. The results obtained for gold surfaces show that in the absence of bias voltage, acoustic phonon transport is dominant for vacuum gaps smaller than ~2 nm. The application of a bias voltage significantly affects the dominant energy carriers as it increases the phonon contribution mediated by the long-range Coulomb force and the electron contribution due to a lower potential barrier. For a bias voltage of 0.6 V, acoustic phonon transport becomes dominant at a vacuum gap of 5 nm, whereas electron tunneling dominates at sub-1-nm vacuum gaps. The comparison of the theory against experimental data from the literature suggests that well-controlled measurements between metallic surfaces are needed to quantify the contributions of acoustic phonon and electron as a function of the bias voltage.
We show that periodic multilayered structures allow to drastically enhance near-field radiative heat transfer between nanoparticles. In particular, when the two nanoparticles are placed on each side of the multilayered structure, at the same interparticle distance the resulting heat transfer is more than five orders of magnitude higher than that in the absence of the multilayered structure. This enhancement takes place in a broad range of distances and is due to the fact that the intermediate multilayered structure supports hyperbolic phonon polaritons with the key feature that the edge frequencies of the Type I and Type II Reststrahlen bands coincide with each other at a value extremely close to the particle resonance. This allow a very high-k evanescent modes resonating with the nanoparticles. Our predictions can be relevant for effective managing of energy at the nano-scale.
Metasurfaces, the two-dimensional (2D) counterpart of metamaterials, have recently attracted a great attention due to their amazing properties such as negative refraction, hyperbolic dispersion, manipulation of the evanescent spectrum. In this work, we propose a theory model for the near field radiative heat transfer (NFRHT) between two nanoparticles in the presence of an anisotropic metasurface. Specifically, we set the metasurface as an array of graphene strips (GS) since it is an ideal platform to implement any metasurface topology, ranging from isotropic to hyperbolic propagation. We show that the NFRHT between two nanoparticles can not only be significantly amplified when they are placed in proximity of the GS, but also be regulated over several orders of magnitude. In this configuration, the anisotropic surface plasmon polaritons (SPPs) supported by the GS are excited and provide a new channel for the near-field energy transport. We analyze how the conductance between two nanoparticles depends on the orientation, the structure parameters and the chemical potential of the GS, on the particle-surface or the particle-surface distances by clearly identifying the characteristics of the anisotropic SPPs such as dispersion relations, propagation length and decay length. Our findings provide a powerful way to regulate the energy transport in the particle systems, meanwhile in turn, open up a way to explore the anisotropic optical properties of the metasurface based on the measured heat transfer properties.
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