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Register a new userAll-Optical Spin Locking in Alkali-Vapor Magnetometers
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The nonlinear Zeeman effect can induce splittings and asymmetries of magnetic-resonance lines in the geophysical magnetic-field range. We demonstrate a scheme to suppress the nonlinear Zeeman effect all optically based on spin locking. Spin locking is achieved with an effective oscillating magnetic field provided by the AC Stark-shift of an intensity-modulated and polarization-modulated laser beam. This results in the collapse of the multi-component asymmetric magnetic-resonance line with about 100 Hz width in the Earth-field range into a peak with a central component width of 25Hz. The technique is expected to be broadly applicable in practical magnetometry, potentially boosting the sensitivity and accuracy of Earth-surveying magnetometers by increasing the magnetic-resonance amplitude and decreasing its width. Advantage of an all-optical approach is the absence of cross-talk between nearby sensors when these are used in a gradiometric or in an array arrangement.
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The nonlinear Zeeman effect can induce splitting and asymmetries of magnetic-resonance lines in the geophysical magnetic field range. This is a major source of heading error for scalar atomic magnetometers. We demonstrate a method to suppress the nonlinear Zeeman effect and heading error based on spin locking. In an all-optical synchronously pumped magnetometer with separate pump and probe beams, we apply a radio-frequency field which is in-phase with the precessing magnetization. In an earth-range field, a multi-component asymmetric magnetic-resonance line with ? 60 Hz width collapses into a single peak with a width of 22 Hz, whose position is largely independent of the orientation of the sensor. The technique is expected to be broadly applicable in practical magnetometry, potentially boosting the sensitivity and accuracy of earth-surveying magnetometers by increasing the magnetic resonance amplitude, decreasing its width and removing the important and limiting heading-error systematic.
We report an experimental observation of degenerate mirrorless lasing in forward direction under excitation of a dilute atomic Rb vapor with a single linearly polarized cw laser light resonant with cycling Fe > Fg atomic D2 transitions. Light polarized orthogonally to the laser light is generated for the input light intensity exceeding a threshold value of about 3 mW/cm^2. Application of a transverse magnetic field directed along the input light polarization reveals a sharp about 20 mG wide magnetic resonance centered at B = 0. Increasing the incident light intensity from 3 to 300 mW/cm^2, the generated light undergoes rapid amplitude increase followed by a decline and resonance broadening. Such nonlinear behavior of the observed magnetic resonance is attributed to the population inversion on optical transitions between magnetic sublevels established under linearly polarized excitation. We present observations that indicate that a combination of nonlinear-optical effects occurs in this system, including degenerate mirrorless lasing and four-wave mixing.
We present a joint experimental and theoretical study of spin coherence properties of 39K, 85Rb, 87Rb, and 133Cs atoms trapped in a solid parahydrogen matrix. We use optical pumping to prepare the spin states of the implanted atoms and circular dichroism to measure their spin states. Optical pumping signals show order-of-magnitude differences depending on both matrix growth conditions and atomic species. We measure the ensemble transverse relaxation times (T2*) of the spin states of the alkali-metal atoms. Different alkali species exhibit dramatically different T2* times, ranging from sub-microsecond coherence times for high mF states of 87Rb, to ~100 microseconds for 39K. These are the longest ensemble T2* times reported for an electron spin system at high densities (n > 10^16 cm^-3). To interpret these observations, we develop a theory of inhomogenous broadening of hyperfine transitions of ^2S atoms in weakly-interacting solid matrices. Our calculated ensemble transverse relaxation times agree well with experiment, and suggest ways to longer coherence times in future work.
We report on widefield microwave vector field imaging with sub um resolution using a microfabricated alkali vapor cell. The setup can additionally image dc magnetic fields, and can be configured to image microwave electric fields. Our camera-based widefield imaging system records 2D images with a 6x6 mm2 field of view at a rate of 10 Hz. It provides up to 50 um spatial resolution, and allows imaging of fields as close as 150 um above structures, through the use of thin external cell walls. This is crucial in allowing us to take practical advantage of the high spatial resolution, as feature sizes in near-fields are on the order of the distance from their source, and represents an order of magnitude improvement in surface-feature resolution compared to previous vapor cell experiments. We present microwave and dc magnetic field images above a selection of devices, demonstrating a microwave sensitivity of 1.4 uT/sqrt-Hz per 50x50x140 um3 voxel, at present limited by the speed of our camera system. Since we image 120x120 voxels in parallel, a single scanned sensor would require a sensitivity of at least 12 nT/sqrt-Hz to produce images with the same sensitivity. Our technique could prove transformative in the design, characterisation, and debugging of microwave devices, as there are currently no satisfactory established microwave imaging techniques. Moreover, it could find applications in medical imaging.
We present an experimental investigation of alkali atom vapor cells coated with a high quality anti-relaxation coating material based on alkenes. The prepared cells with single compound alkene based coating showed the longest spin relaxation times which have been measured up to now with room temperature vapor cells. Suggestions are made that chemical binding of a cesium atom and an alkene molecule by attack to the C=C bond plays a crucial role in such improvement of anti-relaxation coating quality.
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