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Quantum Oscillations of The Positive Longitudinal Magnetoconductivity: a Fingerprint for Identifying Weyl Semimetals

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 Added by Li Sheng
 Publication date 2018
  fields Physics
and research's language is English




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Weyl semimetals (WSMs) host charged Weyl fermions as emergent quasiparticles. We develop a unified analytical theory for the anomalous positive longitudinal magnetoconductance (LMC) in a WSM, which bridges the gap between the classical and ultra-quantum approaches. More interestingly, the LMC is found to exhibit periodic-in-$1/B$ quantum oscillations, originating from the oscillations of the nonequilibrium chiral chemical potential. The quantum oscillations, superposed on the positive LMC, are a remarkable fingerprint of a WSM phase with chiral anomaly, whose observation is a valid criteria for identifying a WSM material. In fact, such quantum oscillations were already observed by several experiments.



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We study the positive longitudinal magnetoconductivity (LMC) and planar Hall effect as emergent effects of the chiral anomaly in Weyl semimetals, following a recent-developed theory by integrating the Landau quantization with Boltzmann equation. It is found that, in the weak magnetic field regime, the LMC and planar Hall conductivity (PHC) obey $cos^{6}theta$ and $cos^{5}thetasin theta$ dependences on the angle $theta$ between the magnetic and electric fields. For higher magnetic fields, the LMC and PHC cross over to $cos^{2}theta$ and $costhetasintheta$ dependences, respectively. Interestingly, the PHC could exhibit quantum oscillations with varying $theta$, due to the periodic-in-$1/B$ oscillations of the chiral chemical potential. When the magnetic and electric fields are noncollinear, the LMC and PHC will deviate from the classical $B$-quadratic dependence, even in the weak magnetic field regime.
Recently, a class of Dirac semimetals, such as textrm{Na}$_{mathrm{3}}% $textrm{Bi} and textrm{Cd}$_{mathrm{2}}$textrm{As}$_{mathrm{3}}$, are discovered to carry $mathbb{Z}_{2}$ monopole charges. We present an experimental mechanism to realize the $mathbb{Z}_{2}$ anomaly in regard to the $mathbb{Z}_{2}$ topological charges, and propose to probe it by magnetotransport measurement. In analogy to the chiral anomaly in a Weyl semimetal, the acceleration of electrons by a spin bias along the magnetic field can create a $mathbb{Z}_{2}$ charge imbalance between the Dirac points, the relaxation of which contributes a measurable positive longitudinal spin magnetoconductivity (LSMC) to the system. The $mathbb{Z}_{2}$ anomaly induced LSMC is a spin version of the longitudinal magnetoconductivity (LMC) due to the chiral anomaly, which possesses all characters of the chiral anomaly induced LMC. While the chiral anomaly in the topological Dirac semimetal is very sensitive to local magnetic impurities, the $mathbb{Z}_{2}$ anomaly is found to be immune to local magnetic disorder. It is further demonstrated that the quadratic or linear field dependence of the positive LMC is not unique to the chiral anomaly. Base on this, we argue that the periodic-in-$1/B$ quantum oscillations superposed on the positive LSMC can serve as a fingerprint of the $mathbb{Z}_{2}$ anomaly in topological Dirac semimetals.
The manifestation of chiral anomaly in Weyl semimetals typically relies on the observation of longitudinal magnetoconductance (LMC) along with the planar Hall effect, with a specific magnetic field and angle dependence. Here we solve the Boltzmann equation in the semiclassical regime for a prototype of a Weyl semimetal, allowing for both intravalley and intervalley scattering, along with including effects from the orbital magnetic moment (OMM), in a geometry where the electric and magnetic fields are not necessarily parallel to each other. We construct the phase diagram in the relevant parameter space that describes the shift from positive to negative LMC in the presence of OMM and sufficiently strong intervalley scattering, as has been recently pointed out for only parallel electric and magnetic fields. On the other hand, we find that the chiral anomaly contribution to the planar Hall effect always remains positive (unlike the LMC) irrespective of the inclusion or exclusion of OMM, or the strength of the intervalley scattering. Our predictions can be directly tested in experiments, and may be employed as new diagnostic procedures to verify chiral anomaly in Weyl systems.
Type-II Weyl semimetals are characterized by the tilted linear dispersion in the low-energy excitations, mimicking Weyl fermions but with manifest violation of the Lorentz invariance, which has intriguing quantum transport properties. The magnetoconductivity of type-II Weyl semimetals is investigated numerically based on lattice models in parallel electric and magnetic field. We show that in the high-field regime, the sign of the magnetoconductivity of an inversion-symmetry-breaking type-II Weyl semimetals depends on the direction of the magnetic field, whereas in the weak field regime, positive magnetoconductivity is always obtained regardless of magnetic field direction. We find that the weak localization is sensitive to the spatial extent of impurity potential. In time-reversal symmetry breaking type-II Weyl semimetals, the system displays either positive or negative magnetoconductivity along the direction of band tilting, owing to the associated effect of group velocity, Berry curvature and the magnetic field.
Weyl fermions in an external magnetic field exhibit the chiral anomaly, a non-conservation of chiral fermions. In a Weyl semimetal, a spatially inhomogeneous Weyl node separation causes similar effect by creating an intrinsic pseudo-magnetic field with an opposite sign for nodes of opposite chirality. In the present work we study the interplay of external and intrinsic fields. In particular, we focus on quantum oscillations due to bulk-boundary trajectories. When caused by an external field, such oscillations are a proven experimental technique to detect Weyl semimetals. We show that the intrinsic field leaves hallmarks on such oscillations by decreasing the period of the oscillations in an analytically traceable manner. The oscillations can thus be used to test the effect of an intrinsic field and to extract its strength.
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