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Register a new userProbing quantum thermalization of a disordered dipolar spin ensemble with discrete time-crystalline order
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We investigate thermalization dynamics of a driven dipolar many-body quantum system through the stability of discrete time crystalline order. Using periodic driving of electronic spin impurities in diamond, we realize different types of interactions between spins and demonstrate experimentally that the interplay of disorder, driving and interactions leads to several qualitatively distinct regimes of thermalization. For short driving periods, the observed dynamics are well described by an effective Hamiltonian which sensitively depends on interaction details. For long driving periods, the system becomes susceptible to energy exchange with the driving field and eventually enters a universal thermalizing regime, where the dynamics can be described by interaction-induced dephasing of individual spins. Our analysis reveals important differences between thermalization of long-range Ising and other dipolar spin models.
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Understanding quantum dynamics away from equilibrium is an outstanding challenge in the modern physical sciences. It is well known that out-of-equilibrium systems can display a rich array of phenomena, ranging from self-organized synchronization to dynamical phase transitions. More recently, advances in the controlled manipulation of isolated many-body systems have enabled detailed studies of non-equilibrium phases in strongly interacting quantum matter. As a particularly striking example, the interplay of periodic driving, disorder, and strong interactions has recently been predicted to result in exotic time-crystalline phases, which spontaneously break the discrete time-translation symmetry of the underlying drive. Here, we report the experimental observation of such discrete time-crystalline order in a driven, disordered ensemble of $sim 10^6$ dipolar spin impurities in diamond at room-temperature. We observe long-lived temporal correlations at integer multiples of the fundamental driving period, experimentally identify the phase boundary and find that the temporal order is protected by strong interactions; this order is remarkably stable against perturbations, even in the presence of slow thermalization. Our work opens the door to exploring dynamical phases of matter and controlling interacting, disordered many-body systems.
Conventional wisdom holds that macroscopic classical phenomena naturally emerge from microscopic quantum laws. However, despite this mantra, building direct connections between these two descriptions has remained an enduring scientific challenge. In particular, it is difficult to quantitatively predict the emergent classical properties of a system (e.g. diffusivity, viscosity, compressibility) from a generic microscopic quantum Hamiltonian. Here, we introduce a hybrid solid-state spin platform, where the underlying disordered, dipolar quantum Hamiltonian gives rise to the emergence of unconventional spin diffusion at nanometer length scales. In particular, the combination of positional disorder and on-site random fields leads to diffusive dynamics that are Fickian yet non-Gaussian. Finally, by tuning the underlying parameters within the spin Hamiltonian via a combination of static and driven fields, we demonstrate direct control over the emergent spin diffusion coefficient. Our work opens the door to investigating hydrodynamics in many-body quantum spin systems.
The discrete time crystal (DTC) is a recently discovered phase of matter that spontaneously breaks time-translation symmetry. Disorder-induced many-body-localization is required to stabilize a DTC to arbitrary times, yet an experimental investigation of this localized regime has proven elusive. Here, we observe the hallmark signatures of a many-body-localized DTC using a novel quantum simulation platform based on individually controllable $^{13}$C nuclear spins in diamond. We demonstrate the characteristic long-lived spatiotemporal order and confirm that it is robust for generic initial states. Our results are consistent with the realization of an out-of-equilibrium Floquet phase of matter and establish a programmable quantum simulator based on solid-state spins for exploring many-body physics.
Symmetries are well known to have had a profound role in our understanding of nature and are a critical design concept for the realization of advanced technologies. In fact, many symmetry-broken states associated with different phases of matter appear in a variety of quantum technology applications. Such symmetries are normally broken in spatial dimension, however they can also be broken temporally leading to the concept of discrete time symmetries and their associated crystals. Discrete time crystals (DTCs) are a novel state of matter emerging in periodically-driven quantum systems. Typically, they have been investigated assuming individual control operations with uniform rotation errors across the entire system. In this work we explore a new paradigm arising from non-uniform rotation errors, where two dramatically different phases of matter coexist in well defined regions of space. We consider a quantum spin network possessing long-range interactions where different driving operations act on different regions of that network. What results from its inherent symmetries is a system where one region is a DTC, while the second is ferromagnetic. We envision our work to open a new avenue of research on Chimera-like phases of matter where two different phases coexist in space.
A quantum phase of matter can be understood from the symmetry of the systems Hamiltonian. The system symmetry along the time axis has been proposed to show a new phase of matter referred as discrete-time crystals (DTCs). A DTC is a quantum phase of matter in non-equilibrium systems, and it is also intimately related to the symmetry of the initial state. DTCs that are stable in isolated systems are not necessarily resilient to the influence from the external reservoir. In this paper, we discuss the dynamics of the DTCs under the influence of an environment. Specifically, we consider a non-trivial situation in which the initial state is prepared to partly preserve the symmetry of the Liouvillian. Our analysis shows that the entire system evolves towards a DTC phase and is stabilised by the effect of dephasing. Our results provide a new understanding of quantum phases emerging from the competition between the coherent and incoherent dynamics in dissipative non-equilibrium quantum systems.
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