No Arabic abstract
The exact factorization approach, originally developed for electron-nuclear dynamics, is extended to light-matter interactions within the dipole approximation. This allows for a Schrodinger equation for the photonic wavefunction, in which the potential contains exactly the effects on the photon field of its coupling to matter. We illustrate the formalism and potential for a two-level system representing the matter, coupled to an infinite number of photon modes in the Wigner-Weisskopf approximation, as well as a single mode with various coupling strengths. Significant differences are found with the potential used in conventional approaches, especially for strong-couplings. We discuss how our exact factorization approach for light-matter interactions can be used as a guideline to develop semiclassical trajectory methods for efficient simulations of light-matter dynamics.
A key concept underlying the specific functionalities of metasurfaces, i.e. arrays of subwavelength nanoparticles, is the use of constituent components to shape the wavefront of the light, on-demand. Metasurfaces are versatile and novel platforms to manipulate the scattering, colour, phase or the intensity of the light. Currently, one of the typical approaches for designing a metasurface is to optimize one or two variables, among a vast number of fixed parameters, such as various materials properties and coupling effects, as well as the geometrical parameters. Ideally, it would require a multi-dimensional space optimization through direct numerical simulations. Recently, an alternative approach became quite popular allowing to reduce the computational cost significantly based on a deep-learning-assisted method. In this paper, we utilize a deep-learning approach for obtaining high-quality factor (high-Q) resonances with desired characteristics, such as linewidth, amplitude and spectral position. We exploit such high-Q resonances for the enhanced light-matter interaction in nonlinear optical metasurfaces and optomechanical vibrations, simultaneously. We demonstrate that optimized metasurfaces lead up to 400+ folds enhancement of the third harmonic generation (THG); at the same time, they also contribute to 100+ folds enhancement in optomechanical vibrations. This approach can be further used to realize structures with unconventional scattering responses.
This thesis offers novel strategies for the measurement of quantum correlations present in controllable quantum systems, as well as for a full-fledged implementation of the models of light-matter interaction through which these correlations can be generated. We propose the use of an ancillary qubit to efficiently access both time-correlation functions and entanglement monotones, and we provide two experimental demonstrations of our methods, measuring time correlations in an NMR setup and entanglement monotones in a photonic system. Moreover, we explain how time-correlation functions could be exploited for the quantum simulation of open quantum dynamics, and we provide an experimental recipe for the measurement of entanglement monotones in trapped ion technologies. On the other hand, we explore the quantum simulation of quantum optical models of light-matter interaction for inaccessible coupling regimes, providing experimental proposals for their implementation, both in ions and superconducting circuits. Finally, we also provide an experimental proposal for the quantum simulation of spin models in trapped ions following a digital-analog simulation scheme.
Dispersive interactions of matter qubits with bright squeezed light in a high-Q cavity is studied. Numerical simulation shows that higher fidelity of operations to obtain a certain phase shift of the pulse through the dispersive light-matter interaction may be reached using bright squeezed light than that using bright coherent light.
We show that molecular spin qudits provide an ideal platform to simulate the quantum dynamics of photon fields strongly interacting with matter. The basic unit of the proposed molecular quantum simulator can be realized by a simple dimer of a spin 1/2 and a spin $S$ transition metal ion, solely controlled by microwave pulses. The spin $S$ ion is exploited to encode the photon field in a flexible architecture, which enables the digital simulation of a wide range of spin-boson models much more efficiently than by using a multi-qubit register. The effectiveness of our proposal is demonstrated by numerical simulations using realistic molecular parameters, whose prerequisites delineating possible chemical approaches are also discussed.
We analyze the coupling of atoms or atom-like emitters to nanophotonic waveguides in the presence of propagating acoustic waves. Specifically, we show that strong index modulations induced by such waves can drastically modify the effective photonic density of states and thereby influence the strength, the directionality, as well as the overall characteristics of photon emission and absorption processes. These effects enable a complete dynamical control of light-matter interactions in waveguide structures, which even in a two dimensional system can be used to efficiently exchange individual photons along selected directions and with a very high fidelity. Such a quantum acousto-optical control provides a versatile tool for various quantum networking applications ranging from the distribution of entanglement via directional emitter-emitter interactions to the routing of individual photonic quantum states via acoustic conveyor belts.