Producing positronium (Ps) in the metastable $2^3text{S}$ state is of interest for various applications in fundamental physics. We report here about an experiment in which Ps atoms are produced in this long-lived state by spontaneous radiative decay of Ps excited to the $3^3text{P}$ level manifold. The Ps cloud excitation is obtained with a UV laser pulse in an experimental vacuum chamber in presence of guiding magnetic field of 25 mT and an average electric field of 300 V/cm. The indication of the $2^3text{S}$ state production is obtained from a novel analysis technique of single-shot positronium annihilation lifetime spectra. Its production efficiency relative to the total amount of formed Ps is evaluated by fitting a simple rate equations model to the experimental data and found to be $ (2.1 pm 1.3) , % $.
We explore coherent control of Penning and associative ionization in cold collisions of metastable He$^*({2}^3text{S})$ atoms via the quantum interference between different states of the He$_2^*$ collision complex. By tuning the preparation coefficients of the initial atomic spin states, we can benefit from the quantum interference between molecular channels to maximize or minimize the cross sections for Penning and associative ionization. In particular, we find that we can enhance the ionization ratio by 30% in the cold regime. This work is significant for the coherent control of chemical reactions in the cold and ultracold regime.
We determine the frequency of the ultranarrow $^{87}text{Sr}$ ${^{1}text{S}_{0}} - {^{3}text{P}_{2}}$ transition by spectroscopy of an ultracold gas. This transition is referenced to four molecular iodine lines that are observed by Doppler-free saturation spectroscopy of hot iodine vapor. The frequency differences between the Sr and the I$_2$ transitions are measured with an uncertainty of 250 kHz. The absolute frequency of the $^{87}text{Sr}$ ${^{1}text{S}_{0}} - {^{3}text{P}_{2}}$ ($text{F}=7/2$) transition is 446648775(30) MHz and limited in accuracy by the iodine reference. This work prepares the use of the Sr ${^{1}text{S}_{0}} - {^{3}text{P}_{2}}$ transition for quantum simulation and computation.
We show that the lifetime of ultracold ground-state $^{87}$Rb$^{133}$Cs molecules in an optical trap is limited by fast optical excitation of long-lived two-body collision complexes. We partially suppress this loss mechanism by applying square-wave modulation to the trap intensity, such that the molecules spend 75% of each modulation cycle in the dark. By varying the modulation frequency, we show that the lifetime of the collision complex is $0.53pm0.06$ ms in the dark. We find that the rate of optical excitation of the collision complex is $3^{+4}_{-2}times10^{3}$ W$^{-1}$ cm$^2$ s$^{-1}$ for $lambda = 1550$ nm, leading to a lifetime of <100 ns for typical trap intensities. These results explain the two-body loss observed in experiments on nonreactive bialkali molecules.
Two anomalously weak transitions within the $2 ^3{rm S}_1~-~3 ^3{rm P}_J$ manifolds in $^3$He have been identified. Their transition strengths are measured to be 1,000 times weaker than that of the strongest transition in the same group. This dramatic suppression of transition strengths is due to the dominance of the hyperfine interaction over the fine structure interaction. An alternative selection rule based on textit{IS}-coupling (where the nuclear spin is first coupled to the total electron spin) is proposed. This provides qualitative understanding of the transition strengths. It is shown that the small deviations from the textit{IS}-coupling model are fully accounted for by an exact diagonalization of the strongly interacting states.
Laser spectroscopy of short-lived radium isotopes in a linear Paul trap has been performed. The isotope shifts of the $6d,^2$D$_{3/2},$ - $7p,^2$P$_{1/2},$ transition in $^{209-214}$Ra$^+$ were measured, which are sensitive to the short range part of the atomic wavefunctions. The results are essential experimental input for improving the precision of atomic structure calculation. This is indispensable for parity violation in Ra$^+$ aiming at the determination of the weak mixing angle.
S. Aghion
,C. Amsler
,M. Antonello
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(2018)
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"Producing long-lived $2^3text{S}$ Ps via $3^3text{P}$ laser excitation in magnetic and electric fields"
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Ruggero Caravita Dr
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