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Register a new userDimensional crossover and incipient quantum size effects in superconducting niobium nanofilms
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Superconducting and normal state properties of sputtered Niobium nanofilms have been systematically investigated, as a function of film thickness in a d=9-90 nm range, on different substrates. The width of the superconducting-to-normal transition for all films remained in few tens of mK, thus remarkably narrow, confirming their high quality. We found that the superconducting critical current density exhibits a pronounced maximum, three times larger than its bulk value, for film thickness around 25 nm, marking the 3D-to-2D crossover. The extracted magnetic penetration depth shows a sizeable enhancement for the thinnest films, aside the usual demagnetization effects. Additional amplification effects of the superconducting properties have been obtained in the case of sapphire substrates or squeezing the lateral size of the nanofilms. For thickness close to 20 nm we also measured a doubled perpendicular critical magnetic field compared to its saturation value for d>33 nm, indicating shortening of the correlation length and the formation of small Cooper pairs in the condensate. Our data analysis evidences an exciting interplay between quantum-size and proximity effects together with strong-coupling effects and importance of disorder in the thinnest films, locating the ones with optimally enhanced critical properties close to the BCS-BEC crossover regime.
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Recent experiments [I.V. Grigorieva et al., Phys. Rev. Lett. 96, 077005 (2006)] on visualization of vortices using the Bitter decoration technique revealed vortex shells in mesoscopic superconducting Nb disks containing up to L=40 vortices. Some of the found configurations did not agree with those predicted theoretically. We show here that this discrepancy can be traced back to the larger disks with radii R ~ 1 to 2.5mu m, i.e., R ~ 50-100xi(0) used in the experiment, while in previous theoretical studies vortex states with vorticity L < 40 were analyzed for smaller disks with R ~ 5-20xi(0). The present analysis is done for thin disks (mesoscopic regime) and for thick (macroscopic) disks where the London screening is taken into account. We found that the radius of the superconducting disk has a pronounced influence on the vortex configuration in contrast to, e.g., the case of parabolic confined charged particles. The missing vortex configurations and the region of their stability are found, which are in agreement with those observed in the experiment.
Structural and superconducting properties of high quality Niobium nanofilms with different thicknesses are investigated on silicon oxide and sapphire substrates. The role played by the different substrates and the superconducting properties of the Nb films are discussed based on the defectivity of the films and on the presence of an interfacial oxide layer between the Nb film and the substrate. The X-ray absorption spectroscopy is employed to uncover the structure of the interfacial layer. We show that this interfacial layer leads to a strong proximity effect, specially in films deposited on a SiO$_2$ substrate, altering the superconducting properties of the Nb films. Our results establish that the critical temperature is determined by an interplay between quantum-size effects, due to the reduction of the Nb film thicknesses, and proximity effects.
We show how the two-dimensional (2D) topological insulator evolves, by stacking, into a strong or weak topological insulator with different topological indices, proposing a new conjecture that goes beyond an intuitive picture of the crossover from quantum spin Hall to the weak topological insulator. Studying the conductance under different boundary conditions, we demonstrate the existence of two conduction regimes in which conduction happens through either surface- or edge-conduction channels. We show that the two conduction regimes are complementary and exclusive. Conductance maps in the presence and absence of disorder are introduced, together with 2D $mathbb{Z}_2$-index maps, describing the dimensional crossover of the conductance from the 2D to the 3D limit. Stacking layers is an effective way to invert the gap, an alternative to controlling the strength of spin-orbit coupling. The emerging quantum spin Hall insulator phase is not restricted to the case of odd numbers of layers.
To decipher the mechanism of high temperature superconductivity, it is important to know how the superconducting pairing emerges from the unusual normal states of cuprate superconductors, including pseudogap, anomalous Fermi liquid and strange metal (SM). A long-standing issue under debate is how the superconducting pairing is formed and condensed in the SM phase because the superconducting transition temperature is the highest in this phase. Here, we report the first experimental observation of a pressure-induced crossover from two- to three-dimensional superconducting states in the optimally-doped Bi2Sr2CaCu2O8+delta bulk superconductor at a pressure above 2.8 GPa, through state-of-the-art in-situ high-pressure measurements of resistance, magnetoresistance and magnetic susceptibility. By analyzing the temperature dependence of resistance, we find that the two-dimensional (2D) superconducting transition exhibits a Berezinski-Kosterlitz-Thouless-like behavior. The emergence of this 2D superconducting transition provides direct and strong evidence that the SM state is predominantly 2D-like. This is important to a thorough understanding of the phase diagram of cuprate superconductors.
We present an experimental study of two-dimensional superconducting quantum interference filters (2D-SQIFs) in the presence of a magnetic field B. The dependences of the dc voltage on the applied magnetic field are characterized by a unique delta-like dip at B=0, which depends on the distribution of the areas of the individual loops, and on the bias current. The voltage span of the dip scales proportional to the number of rows simultaneously operating at the same working point. In addition, the voltage response of the 2D-SQIF is sensitive to a field gradient generated by a control line and superimposed to the homogeneous field coil. This feature opens the possibility to use 2D superconducting quantum interference filters as highly sensitive detectors of spatial gradients of magnetic field.
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