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Absolute frequency measurement of the $^2$S$_{1/2} rightarrow ^2$F$_{7/2}$ optical clock transition in $^{171}$Yb$^+$ with an uncertainty of $4times 10^{-16}$ using a frequency link to International Atomic Time

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 Added by Rachel Godun
 Publication date 2017
  fields Physics
and research's language is English




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The highly forbidden $^2$S$_{1/2} rightarrow ^2$F$_{7/2}$ electric octupole transition in $^{171}$Yb$^+$ is a potential candidate for a redefinition of the SI second. We present a measurement of the absolute frequency of this optical transition, performed using a frequency link to International Atomic Time to provide traceability to the SI second. The $^{171}$Yb$^+$ optical frequency standard was operated for 76% of a 25-day period, with the absolute frequency measured to be 642 121 496 772 645.14(26) Hz. The fractional uncertainty of $4.0 times 10 ^{-16}$ is comparable to that of the best previously reported measurement, which was made by a direct comparison to local caesium primary frequency standards.



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The absolute frequency of the $^{87}{rm Sr}$ clock transition measured in 2015 was reevaluated using an improved frequency link to the SI second. The scale interval of International Atomic Time (TAI) that we used as the reference was calibrated for an evaluation interval of five days instead of the conventional interval of one month which is regularly employed in Circular T. The calibration on a five-day basis removed the uncertainty in assimilating the TAI scale of the five-day mean to that of the one-month mean. The reevaluation resulted in the total uncertainty of $10^{-16}$ level for the first time without local cesium fountains. Since there are presumably no correlations among systematic shifts of cesium fountains worldwide, the measurement is not limited by the systematic uncertainty of a specific primary frequency standard.
We measured the absolute frequency of the optical clock transition 1S0 (F = 1/2) - 3P0 (F = 1/2) of 171Yb atoms confined in a one-dimensional optical lattice and it was determined to be 518 295 836 590 863.5(8.1) Hz. The frequency was measured against Terrestrial Time (TT; the SI second on the geoid) by using an optical frequency comb of which the frequency was phase-locked to an H-maser as a flywheel oscillator traceable to TT. The magic wavelength was also measured as 394 798.48(79) GHz. The results are in good agreement with two previous measurements of other institutes within the specified uncertainty of this work.
Transition frequencies were determined for transitions in Ra in an atomic beam and for reference lines in Te$_2$ molecules in a vapor cell. The absolute frequencies were calibrated against a GPS stabilized Rb-clock by means of an optical frequency comb. The 7s$^2,^1$S$_0$(F = 1/2)-7s7p$,^1$P$_1$(F = 3/2) transition in $^{225}$Ra was determined to be $621,042,124(2),$MHz. The measurements provide input for designing efficient and robust laser cooling of Ra atoms in preparation of a search for a permanent electric dipole moment in Ra isotopes.
We present a measurement of the absolute frequency of the 5s$^2$ $^1$S$_0$ to 5s5p $^3$P$_0$ transition in $^{87}$Sr, which is a secondary representation of the SI second. We describe the optical lattice clock apparatus used for the measurement, and we focus in detail on how its systematic frequency shifts are evaluated with a total fractional uncertainty of $1 times 10^{-17}$. Traceability to the International System of Units is provided via comparison to International Atomic Time (TAI). Gathering data over 5- and 15-day periods, with the lattice clock operating on average 74$%$ of the time, we measure the frequency of the transition to be 429228004229873.1(5) Hz, which corresponds to a fractional uncertainty of $1 times 10^{-15}$. We describe in detail how this uncertainty arises from the intermediate steps linking the optical frequency standard, through our local time scale UTC(NPL), to an ensemble of primary and secondary frequency standards which steer TAI. The calculated absolute frequency of the transition is in good agreement with recent measurements carried out in other laboratories around the world.
Qubits encoded in hyperfine states of trapped ions are ideal for quantum computation given their long lifetimes and low sensitivity to magnetic fields, yet they suffer from off-resonant scattering during detection often limiting their measurement fidelity. In ${}^{171}$Yb$^{+}$ this is exacerbated by a low fluorescence yield, which leads to a need for complex and expensive hardware - a problematic bottleneck especially when scaling up the number of qubits. We demonstrate a detection routine based on electron shelving to address this issue in ${}^{171}$Yb$^{+}$ and achieve a 5.6$times$ reduction in single-ion detection error on an avalanche photodiode to $1.8(2)times10^{-3}$ in a 100 $mu$s detection period, and a 4.3$times$ error reduction on an electron multiplying CCD camera, with $7.7(2)times10^{-3}$ error in 400 $mu$s. We further improve the characterization of a repump transition at 760 nm to enable a more rapid reset of the auxiliary $^2$F$_{7/2}$ states populated after shelving. Finally, we examine the detection fidelity limit using the long-lived $^2$F$_{7/2}$ state, achieving a further 300$times$ and 12$times$ reduction in error to $6(7)times10^{-6}$ and $6.3(3)times10^{-4}$ in 1 ms on the respective detectors. While shelving-rate limited in our setup, we suggest various techniques to realize this detection method at speeds compatible with quantum information processing, providing a pathway to ultra-high fidelity detection in ${}^{171}$Yb$^{+}$.
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