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Register a new userUniversal behaviour of the glass and the jamming transitions in finite dimensions
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Added by
Massimo Pica Ciamarra
Publication date
2017
fields
Physics
and research's language is
English
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We investigate the glass and the jamming transitions of hard spheres in finite dimensions $d$, through a revised cell theory, that combines the free volume and the Random First Order Theory (RFOT). Recent results show that in infinite dimension the ideal glass transition and jamming transitions are distinct, while based on our theory we argue that they indeed coincide for finite $d$. As a consequence, jamming results into a percolation transition described by RFOT, with a static length diverging with exponent $ u=2/d$, which we verify through finite size scaling, and standard critical exponents $alpha = 0$, $beta = 0$ and $gamma = 2$ independent on $d$.
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The question about the existence of a structural glass transition in two dimensions is studied using mode coupling theory (MCT). We determine the explicit d-dependence of the memory functional of mode coupling for one-component systems. Applied to two dimensions we solve the MCT equations numerically for monodisperse hard discs. A dynamic glass transition is found at a critical packing fraction phi_c^{d=2} = 0.697 which is above phi_c^{d=3} = 0.516 by about 35%. phi^d_c scales approximately with phi^d_{rm rcp} the value for random close packing, at least for d=2, 3. Quantities characterizing the local, cooperative cage motion do not differ much for d=2 and d=3, and we e.g. find the Lindemann criterion for the localization length at the glass transition. The final relaxation obeys the superposition principle, collapsing remarkably well onto a Kohlrausch law. The d=2 MCT results are in qualitative agreement with existing results from MC and MD simulations. The mean squared displacements measured experimentally for a quasi-two-dimensional binary system of dipolar hard spheres can be described satisfactorily by MCT for monodisperse hard discs over four decades in time provided the experimental control parameter Gamma (which measures the strength of dipolar interactions) and the packing fraction phi are properly related to each other.
Nearly all dense suspensions undergo dramatic and abrupt thickening transitions in their flow behavior when sheared at high stresses. Such transitions occur when the dominant interactions between the suspended particles shift from hydrodynamic to frictional. Here, we interpret abrupt shear thickening as a precursor to a rigidity transition, and give a complete theory of the viscosity in terms of a universal crossover scaling function from the frictionless jamming point to a rigidity transition associated with friction, anisotropy, and shear. Strikingly, we find experimentally that for two different systems -- cornstarch in glycerol and silica spheres in glycerol -- the viscosity can be collapsed onto a single universal curve over a wide range of stresses and volume fractions. The collapse reveals two separate scaling regimes, due to a crossover between frictionless isotropic jamming and a frictional shear jamming point with different critical exponents. The material-specific behavior due to the microscale particle interactions is incorporated into an additive analytic background (given by the viscosity at low shear rates) and a scaling variable governing the proximity to shear jamming that depends on both stress and volume fraction. This reformulation opens the door to importing the vast theoretical machinery developed to understand equilibrium critical phenomena to elucidate fundamental physical aspects of the shear thickening transition.
Dense assemblies of self-propelled particles undergo a nonequilibrium form of glassy dynamics. Physical intuition suggests that increasing departure from equilibrium due to active forces fluidifies a glassy system. We falsify this belief by devising a model of self-propelled particles where increasing departure from equilibrium can both enhance or depress glassy dynamics, depending on the chosen state point. We analyze a number of static and dynamic observables and suggest that the location of the nonequilibrium glass transition is primarily controlled by the evolution of two-point static density correlations due to active forces. The dependence of the density correlations on the active forces varies non-trivially with the details of the system, and is difficult to predict theoretically. Our results emphasize the need to develop an accurate liquid state theory for nonequilibrium systems.
While frictionless spheres at jamming are isostatic, frictional spheres at jamming are not. As a result, frictional spheres near jamming do not necessarily exhibit an excess of soft modes. However, a generalized form of isostaticity can be introduced if fully mobilized contacts at the Coulomb friction threshold are considered as slipping contacts. We show here that, in this framework, the vibrational density of states (DOS) of frictional discs exhibits a plateau when the generalized isostaticity line is approached. The crossover frequency to elastic behavior scales linearly with the distance from this line. Moreover, we show that the frictionless limit, which appears singular when fully mobilized contacts are treated elastically, becomes smooth when fully mobilized contacts are allowed to slip.
The phenomenon of shear-induced jamming is a factor in the complex rheological behavior of dense suspensions. Such shear-jammed states are fragile, i.e., they are not stable against applied stresses that are incompatible with the stress imposed to create them. This peculiar flow-history dependence of the stress response is due to flow-induced microstructures. To examine jammed states realized under constant shear stress, we perform dynamic simulations of non-Brownian particles with frictional contact forces and hydrodynamic lubrication forces. We find clear signatures that distinguish these fragile states from the more conventional isotropic jammed states.
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