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Simon Trebst
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In transition-metal compounds with partially filled $4d$ and $5d$ shells spin-orbit entanglement, electronic correlations, and crystal-field effects conspire to give rise to a variety of novel forms of topological quantum matter. This includes Kitaev materials -- a family of spin-orbit assisted Mott insulators, in which local, spin-orbit entangled $j=1/2$ moments form that are subject to strong bond-directional interactions. On a conceptual level, Kitaev materials attract much interest for their unconventional forms of magnetism, such as spin liquid physics in two- and three-dimensional lattice geometries or the formation of non-trivial spin textures. Experimentally, a number of Kitaev materials have been synthesized, which includes the honeycomb materials Na$_2$IrO$_3$, $alpha$-Li$_2$IrO$_3$, and RuCl$_3$, the triangular materials Ba$_3$Ir$_x$Ti$_{3-x}$O$_9$, as well as the three-dimensional hyper-honeycomb and stripy-honeycomb materials $beta$-Li$_2$IrO$_3$ and $gamma$-Li$_2$IrO$_3$. These lecture notes provide a short review of the current status of the theoretical and experimental exploration of these Kitaev materials.
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Recent thermal-conductivity measurements evidence a magnetic-field-induced non-Abelian spin liquid phase in the Kitaev material $alpha$-$mathrm{RuCl}_{3}$. Although the platform is a good Mott insulator, we propose experiments that electrically probe the spin liquids hallmark chiral Majorana edge state and bulk anyons, including their exotic exchange statistics. We specifically introduce circuits that exploit interfaces between electrically active systems and Kitaev materials to `perfectly convert electrons from the former into emergent fermions in the latter---thereby enabling variations of transport probes invented for topological superconductors and fractional quantum Hall states. Along the way we resolve puzzles in the literature concerning interacting Majorana fermions, and also develop an anyon-interferometry framework that incorporates nontrivial energy-partitioning effects. Our results illuminate a partial pathway towards topological quantum computation with Kitaev materials.
The Kitaev spin liquid provides a rare example of well-established quantum spin liquids in more than one dimension. It is obtained as the exact ground state of the Kitaev spin model with bond-dependent anisotropic interactions. The peculiar interactions can be yielded by the synergy of spin-orbit coupling and electron correlations for specific electron configuration and lattice geometry, which is known as the Jackeli-Khaliullin mechanism. Based on this mechanism, there has been a fierce race for the materialization of the Kitaev spin liquid over the last decade, but the candidates have been still limited mostly to $4d$- and $5d$-electron compounds including cations with the low-spin $d^5$ electron configuration, such as Ir$^{4+}$ and Ru$^{3+}$. Here we discuss recent efforts to extend the material perspective beyond the Jackeli-Khaliullin mechanism, by carefully reexamining the two requisites, formation of the $j_{rm eff}=1/2$ doublet and quantum interference between the exchange processes, for not only $d$- but also $f$-electron systems. We present three examples: the systems including Co$^{2+}$ and Ni$^{3+}$ with the high-spin $d^7$ electron configuration, Pr$^{4+}$ with the $f^1$-electron configuration, and polar asymmetry in the lattice structure. In particular, the latter two are intriguing since they may realize the antiferromagnetic Kitaev interactions, in contrast to the ferromagnetic ones in the existing candidates. This partial overview would stimulate further material exploration of the Kitaev spin liquids and its topological properties due to fractional excitations.
Recently, the family of rare-earth chalcohalides were proposed as candidate compounds to realize the Kitaev spin liquid (KSL). In the present work, we firstly propose an effective spin Hamiltonian consistents with the symmetry group of the crystal structure. Then we apply classical Monte Carlo simulations to preliminarily study the model and establish a phase diagram. When approaching to the low temperature limit, several magnetic long range orders are observed, including the stripe, the zigzag, the antiferromagnetic (AFM), the ferromagnetic (FM), the incommensurate spiral (IS), the Multi-$pmb {Q}$ and the 120{deg}. We further calculate the thermodynamic properties of the system, such as the temperature dependence of the magnetic susceptibility and the heat capacity. The ordering transition temperatures reflected in the two quantities agree with each other. For most interaction regions, the system is magnetically more susceptible in the $ab$-plane than in the $c$-direction. The stripe phase is special, where the susceptibility is fairly isotropic in the whole temperature region. These features provide useful information to understand the magnetic properties of related materials.
Kitaev materials are promising materials for hosting quantum spin liquids and investigating the interplay of topological and symmetry-breaking phases. We use an unsupervised and interpretable machine-learning method, the tensorial-kernel support vector machine, to study the honeycomb Kitaev-$Gamma$ model in a magnetic field. Our machine learns the global classical phase diagram and the associated analytical order parameters, including several distinct spin liquids, two exotic $S_3$ magnets, and two modulated $S_3 times Z_3$ magnets. We find that the extension of Kitaev spin liquids and a field-induced suppression of magnetic order already occur in the large-$S$ limit, implying that critical parts of the physics of Kitaev materials can be understood at the classical level. Moreover, the two $S_3 times Z_3$ orders are induced by competition between Kitaev and $Gamma$ spin liquids and feature a different type of spin-lattice entangled modulation, which requires a matrix description instead of scalar phase factors. Our work provides a direct instance of a machine detecting new phases and paves the way towards the development of automated tools to explore unsolved problems in many-body physics.
We gauge the fermion parity symmetry of the Kitaev chain. While the bulk of the model becomes an Ising chain of gauge-invariant spins in a tilted field, near the boundaries the global fermion parity symmetry survives gauging, leading to local gauge-invariant Majorana operators. In the absence of vortices, the Higgs phase exhibits fermionic symmetry-protected topological (SPT) order distinct from the Kitaev chain. Moreover, the deconfined phase can be stable even in the presence of vortices. We also undertake a comprehensive study of a gently gauged model which interpolates between the ordinary and gauged Kitaev chains. This showcases rich quantum criticality and illuminates the topological nature of the Higgs phase. Even in the absence of superconducting terms, gauging leads to an SPT phase which is intrinsically gapless due to an emergent anomaly.
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