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Register a new userIntra-layer doping effects on the high-energy magnetic correlations in NaFeAs
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Jonathan Pelliciari
Publication date
2016
fields
Physics
and research's language is
English
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We have used Resonant Inelastic X-ray Scattering (RIXS) and dynamical susceptibility calculations to study the magnetic excitations in NaFe$_{1-x}$Co$_x$As (x = 0, 0.03, and 0.08). Despite a relatively low ordered magnetic moment, collective magnetic modes are observed in parent compounds (x = 0) and persist in optimally (x = 0.03) and overdoped (x = 0.08) samples. Their magnetic bandwidths are unaffected by doping within the range investigated. High energy magnetic excitations in iron pnictides are robust against doping, and present irrespectively of the ordered magnetic moment. Nevertheless, Co doping slightly reduces the overall magnetic spectral weight, differently from previous studies on hole-doped BaFe$_{2}$As$_{2}$, where it was observed constant. Finally, we demonstrate that the doping evolution of magnetic modes is different for the dopants being inside or outside the Fe-As layer.
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Understanding high-temperature superconductivity requires a prior knowledge of the nature of the enigmatic pseudogap metallic state, out of which the superconducting state condenses. In addition to the electronic orders involving charge degrees of freedoms recently reported inside the pseudogap state, a magnetic intra-unit-cell (IUC) order was discovered in various cuprates to set in just at the pseudogap temperature, T*. In nearly optimally doped YBa$_2$Cu$_3$O$_{6.85}$, polarized neutron scattering measurements, carried out on two different spectrometers, reveal new features. The order is made of finite size planar domains, hardly correlated along the c-axis. At high temperature, only the out-of-plane magnetic components correlate, revealing a strong Ising anistropy, as originally predicted in the loop current model. Below T*, a correlated in-plane response develops, giving rise the apparent tilt of the magnetic moment at low temperature. The discovery of these two regimes put stringent constraints on the intrinsict nature of IUC order, tightly bound to the pseudogap physics.
The pairing glue of high-$T_{rm c}$ superconductivity in heavily electron-doped (e-doped) FeSe, in which hole-pockets are absent, has been an important unsolved problem. Here, we focus on a heavily e-doped bulk superconductor Li$_{1-x}$Fe$_x$OHFeSe ($T_{rm c} sim 40$K). We construct a multiorbital model beyond the rigid band approximation and analyze the spin and orbital fluctuations by taking both vertex corrections (VCs) and self-energy into consideration. Without e-doping ($x=0$), the ferro-orbital order without magnetism in FeSe is reproduced by the VCs.The orbital order quickly disappears when the hole-pocket vanishes at $x sim 0.03$. With increasing $x$ further, the spin fluctuations remain small, whereas orbital fluctuations gradually increase with $x$ due to the VCs. The negative feedback due to the self-energy is crucial to explain experimental phase diagram. Thanks to both vertex and self-energy corrections, the orbital-fluctuation-mediated $s_{++}$-wave state appears for a wide doping range, consistent with experiments.
Impurity effects of Zn and Ni on the low-energy spin excitations were systematically studied in optimally doped La1.85Sr0.15Cu1-yAyO4 (A=Zn, Ni) by neutron scattering. Impurity-free La1.85Sr0.15CuO4 shows a spin gap of 4meV below Tc in the antiferromagnetic(AF) incommensurate spin excitation. In Zn:y=0.004, the spin excitation shows a spin gap of 3meV below Tc. In Zn:y=0.008 and Zn:y=0.011, however, the magnetic signals at 3meV decrease below Tc and increase again at lower temperature, indicating an in-gap state. In Zn:y=0.017, the low-energy spin state remains unchanged with decreasing temperature, and elastic magnetic peaks appear below 20K then exponentially increase. As for Ni:y=0.009 and Ni:y=0.018, the low-energy excitations below 3meV and 2meV disappear below Tc. The temperature dependence at 3meV, however, shows no upturn in constrast with Zn:y=0.008 and Zn:y=0.011, indicating the absence of in-gap state. In Ni:y=0.029, the magnetic signals were observed also at 0meV. Thus the spin gap closes with increasing Ni. Furthermore, as omega increases, the magnetic peak width broadens and the peak position, i.e. incommensurability, shifts toward the magnetic zone center (pi pi). We interpret the impurity effects as follows: Zn locally makes a non-superconducting island exhibiting the in-gap state in the superconducting sea with the spin gap. Zn reduces the superconducting volume fraction, thus suppressing Tc. On the other hand, Ni primarily affects the superconducting sea, and the spin excitations become more dispersive and broaden with increasing energy, which is recognized as a consequence of the reduction of energy scale of spin excitations. We believe that the reduction of energy scale is relevant to the suppression of Tc.
Starting from a recently proposed comprehensive theory for the high-Tc superconductivity in cuprates, we derive a general analytic expression for the planar resistivity, in the presence of an applied external magnetic field $textbf{H}$ and explore its consequences in the different phases of these materials. As an initial probe of our result, we show it compares very well with experimental data for the resistivity of LSCO at different values of the applied field. We also apply our result to Bi2201 and show that the magnetoresistivity in the strange metal phase of this material, exhibits the $H^2$ to $H$ crossover, as we move from the weak to the strong field regime. Yet, despite of that, the magnetoresistivity does not present a quadrature scaling. Remarkably, the resistivity H-field derivative does scale as a function of $frac{H}{T}$, in complete agreement with recent magneto-transport measurements made in the strange metal phase of cuprates cite{Hussey2020}. We, finally, address the issue of the $T$-power-law dependence of the resistivity of overdoped cuprates and compare our results with experimental data for Tl2201. We show that this provides a simple method to determine whether the quantum critical point associated to the pseudogap temperature $T^*(x)$ belongs to the SC dome or not.
The discovery of EuFeAs2, currently the only charge-neutral parent phase of the 112-type iron-pnictide system, provides a new platform for the study of elemental doping effects on magnetism and superconductivity (SC). In this study, a series of polycrystalline EuFe1-yCoyAs2 and Eu0.9Pr0.1Fe1-yCoyAs2 samples are synthesized through solid-state reaction, and the evolutions of SC and magnetism with Co doping in EuFeAs2 and Eu0.9Pr0.1FeAs2 are investigated by electrical transport and magnetic susceptibility measurements. For EuFe1-yCoyAs2, the Eu-related antiferromagnetic (AFM) transition around 40 K is barely affected by Co doping, while the Fe-related spin density wave (SDW) transition temperature drops rapidly. Meanwhile, SC is induced by a trace amount of Co doping, with a highest transition temperature Tc ~ 28 K found in EuFe0.9Co0.1As2. For the Eu0.9Pr0.1Fe1-yCoyAs2 series, the magnetism and superconductivity show similar evolutions upon Co doping, and the highest Tc is enhanced to 30.6 K with an optimum doping level y ~ 0.07. Our results shed light on the competition between SC and SDW with Co doping in the 112-type EuFeAs2 system.
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