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Perfect energy-feeding into strongly coupled systems and interferometric control of polariton absorption

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 Added by Simone Zanotto
 Publication date 2016
  fields Physics
and research's language is English




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The ability to feed energy into a system, or - equivalently - to drive that system with an external input is a fundamental aspect of light-matter interaction. The key concept in many photonic applications is the critical coupling condition: at criticality, all the energy fed to the system via an input channel is dissipated within the system itself. Although this idea was crucial to enhance the efficiency of many devices, it was never considered in the context of systems operating in a non-perturbative regime. In this so-called strong coupling regime, the matter and light degrees of freedom are in fact mixed into dressed states, leading to new eigenstates called polaritons. Here we demonstrate that the strong coupling regime and the critical coupling condition can indeed coexist; in this situation, which we term strong critical coupling, all the incoming energy is converted into polaritons. A semiclassical theory - equivalently applicable to acoustics or mechanics - reveals that the strong critical coupling corresponds to a special curve in the phase diagram of the coupled light-matter oscillators. In the more general case of a system radiating via two scattering ports, the phenomenology displayed is that of coherent perfect absorption (CPA), which is then naturally understood and described in the framework of critical coupling. Most importantly, we experimentally verify polaritonic CPA in a semiconductor-based intersubband-polariton photonic-crystal membrane resonator. This result opens new avenues in the exploration of polariton physics, making it possible to control the pumping efficiency of a system almost independently of its Rabi energy, i.e., of the energy exchange rate between the electromagnetic field and the material transition.



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We compare the photoluminescence spectrum of an indium arsenide (InAs) quantum dot (QD) that is strongly coupled to a photonic crystal cavity under above band excitation (ABE) and quasi-resonant excitation (QRE). We show that off-resonant cavity feeding, which manifests itself in a bare cavity emission peak at the strong coupling point, is suppressed by as much as 40% under QRE relative to ABE. We attribute this suppression to a reduced probability of QD charging because electrons and holes are created in pairs inside the QD. We investigate the pump power dependence of the cavity feeding and show that, below saturation, the ratio of the bare cavity emission to polariton emission for ABE is independent of pump power, while for QRE there is linear pump power dependence. These results suggest that the biexciton plays an important role in cavity feeding for QRE.
We experimentally and theoretically challenge the concept of coherent perfect absorption (CPA) as a narrow frequency resonant mechanism associated with scattering processes that respect scale-invariance. Using a microwave platform, consisting of a lossy nonlinear resonator coupled to two interrogating antennas, we show that a coherent incident excitation can trigger a self-induced perfect absorption once its intensity exceeds a critical value. Importantly, a (near) perfect absorption persists for a broad band frequency range around the nonlinear CPA condition. Its origin is traced to a quartic behavior that the absorbance spectrum acquires in the proximity of a CPA associated with a new kind of exceptional point degeneracy related to the zeros of the nonlinear scattering operator.
We investigate the influence of exciton-phonon coupling on the dynamics of a strongly coupled quantum dot-photonic crystal cavity system and explore the effects of this interaction on different schemes for non-classical light generation. By performing time-resolved measurements, we map out the detuning-dependent polariton lifetime and extract the spectrum of the polariton-to-phonon coupling with unprecedented precision. Photon-blockade experiments for different pulse-length and detuning conditions (supported by quantum optical simulations) reveal that achieving high-fidelity photon blockade requires an intricate understanding of the phonons influence on the system dynamics. Finally, we achieve direct coherent control of the polariton states of a strongly coupled system and demonstrate that their efficient coupling to phonons can be exploited for novel concepts in high-fidelity single photon generation.
Two-dimensional photonic crystal membranes provide a versatile planar architecture for integrated photonics to control the propagation of light on a chip employing high quality optical cavities, waveguides, beamsplitters or dispersive elements. When combined with highly non-linear quantum emitters, quantum photonic networks operating at the single photon level come within reach. Towards large-scale quantum photonic networks, selective dynamic control of individual components and deterministic interactions between different constituents are of paramount importance. This indeed calls for switching speeds ultimately on the systems native timescales. For example, manipulation via electric fields or all-optical means have been employed for switching in nanophotonic circuits and cavity quantum electrodynamics studies. Here, we demonstrate dynamic control of the coherent interaction between two coupled photonic crystal nanocavities forming a photonic molecule. By using an electrically generated radio frequency surface acoustic wave we achieve optomechanical tuning, demonstrate operating speeds more than three orders of magnitude faster than resonant mechanical approaches. Moreover, the tuning range is large enough to compensate for the inherent fabrication-related cavity mode detuning. Our findings open a route towards nanomechanically gated protocols, which hitherto have inhibited the realization in all-optical schemes.
66 - Floriana Giannuzzi 2019
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