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Register a new userObservation of hard radiations in a laboratory atmospheric high-voltage discharge
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The new results concerning neutron emission detection from a laboratory high-voltage discharge in the air are presented. Data were obtained with a combination of plastic scintillation detectors and $^3$He filled counters of thermal neutrons. Strong dependence of the hard x-ray and neutron radiation appearance on the field strength near electrodes, which is determined by their form, was found. We have revealed a more sophisticated temporal structure of the neutron bursts observed during of electric discharge. This may indicate different mechanisms for generating penetrating radiation at the time formation and development of the atmospheric discharge.
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The results of the experiments on recording hard gamma radiation and measurements of its angular distribution at the initial stage of a laboratory high-voltage atmospheric discharge are presented. The experiments were performed on an ERG installation at a voltage of $sim 1$ MV, an atmospheric discharge current of up to 12 kA, and a gap of 0.55 m. The duration of the voltage pulse was about 1~$mu$s with a pulse rise time of 150-200 ns. The radiation was recorded by an assembly of 10 identical scintillation detectors installed each 10$^circ$ around the circumference of a quarter of a circle with a curvature of 1 m. In order to separate the radiation with energies from 20 keV to 1.5 MeV, Al and Pb filters of different thicknesses were used. The obtained results show that, as a rule, a multi-beam radiation pattern and several bursts of radiation (each with a directional pattern) are recorded in each shot. In a considerable number of shots, hard radiation with photon energies comparable to or exceeding the maximum electron energy corresponding to the applied voltage is recorded. In these cases, a needle-like radiation pattern is observed, including at large angles to the axis of the discharge. This may indicate the acceleration of electrons in different plasma channels.
Nanoparticles grown in a plasma are used to visualize the process of film deposition in a pulsed radio-frequency (rf) atmospheric pressure glow discharge. Modulating the plasma makes it possible to successfully prepare porous TiO2 films. We study the trapping of the particles in the sheath during the plasma-on phase and compare it with numerical simulations. During the plasma-off phase, the particles are driven to the substrate by the electric field generated by residual ions, leading to the formation of porous TiO2 film. Using video microscopy, the collective dynamics of particles in the whole process is revealed at the most fundamental kinetic level.
We report the development of a laboratory-based Rowland-circle monochromator that incorporates a low poer x-ray (bremsstrahlung) tube source, a spherically-bent crystal analyzer (SBCA), and an energy-resolving solid-state detector. This relatively inexpensive, introductory level instrument achieves 1-eV energy resolution for photon energies of 5 keV to 10 keV while also dmeonstrating a net efficiency previously seen only in laboratory monochromators having much coarser energy resolution. Despite the use of only a compact, air-cooled 10 W x-ray tube, we find count rates for nonresonant x-ray emission spectroscopy (XES) comparable to those achived at monochromatized spectroscopy beamlines at synchrotron light sources. For x-ray absorption near edge structure (XANES), the monochromatized flux is small (due to the use of a low-powered x-ray generator) but still useful for routine transmission-mode studies of concentrated samples. These results indicate that upgrading to a standard commercial high-powered line-focused x-ray tube or rotating anode x-ray generator would result in monochromatized fluxes of order 10^6 to 10^7 photons/s with no loss in energy resolution. This work establishes core technical capabilities for a rejuvenation of laboratory-based x-ray spectroscopies that could have special relevance for contemporary research on catalytic or electrical energy storage systems using transition-metal, lanthanide, or noble-metal active species.
In this work, we present an experimental study of nanosecond high-voltage discharges in a pin-to-pin electrode configuration at atmospheric conditions operating in single-pulse mode (no memory effects). Various discharge parameters, including voltage, current, gas density, rotational/vibrational/gas temperature, and electron number density, were measured. Several different measurement techniques were used, including microwave Rayleigh scattering, laser Rayleigh scattering, optical emission spectroscopy enhanced with a nanosecond probing pulse, fast photography, and electrical parameter measurements. Spark and corona discharge regimes were studied with discharge pulse duration of 90 ns and electrode gap sizes ranging from 2 to 10 mm. The spark regime was observed for gaps < 6 mm using discharge pulse energies of 0.6-1 mJ per mm of the gap length. Higher electron number densities, total electron number per gap length, discharge currents, and gas temperatures were observed for smaller electrode gaps and larger pulse energies, reaching maximal values of about 7.5x10^15 cm-3, 3.5x10^11 electrons per mm, 22 A, and 4,000 K (at 10 us after the discharge), respectively, for a 2 mm gap and 1 mJ/mm discharge pulse energy. Initial breakdown was followed by a secondary breakdown occurring about 30-70 ns later and was associated with ignition of a cathode spot and transition of the discharge to cathodic arc. A majority of the discharge pulse energy was deposited into the gas before the secondary breakdown (85-89%). The electron number density after the ns discharge pulse decayed with a characteristic time scale of 150 ns governed by dissociative recombination and electron attachment to oxygen mechanisms. For the corona regime, substantially lower pulse energies (~0.1 mJ/mm), peak conduction current (1-2 A), and electron numbers (3-5x10^10 electrons per mm), and gas temperatures (360 K) were observed.
The Gamma-Ray Observation of Winter Thunderclouds (GROWTH) collaboration has been performing observation campaigns of high-energy radiation in coastal areas of Japan Sea. Winter thunderstorms in Japan have unique characteristics such as frequent positive-polarity discharges, large discharge current, and low cloud bases. These features allow us to observe both long-duration gamma-ray bursts and lightning-triggered short-duration bursts at sea level. In 2015, we started a mapping observation project using multiple detectors at several new observation sites. We have developed brand-new portable gamma-ray detectors and deployed in the Kanazawa and Komatsu areas as well as the existing site at Kashiwazaki. During three winter seasons from 2015, we have detected 27 long-duration bursts and 8 short-duration bursts. The improved observation network in Kashiwazaki enables us to discover that the short-duration bursts are attributed to atmospheric photonuclear reactions triggered by a downward terrestrial gamma-ray flash. Collaborating with electric-field and radio-band measurements, we have also revealed a relation between abrupt termination of a long-duration burst and a lightning discharge. We demonstrate that the mapping observation project has been providing us clues to understand high-energy atmospheric phenomena associated with thunderstorm activities.
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