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Register a new userThe role of master clock stability in scalable quantum information processing
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Experimentalists seeking to improve the coherent lifetimes of quantum bits have generally focused on mitigating decoherence mechanisms through, for example, improvements to qubit designs and materials, and system isolation from environmental perturbations. In the case of the phase degree of freedom in a quantum superposition, however, the coherence that must be preserved is not solely internal to the qubit, but rather necessarily includes that of the qubit relative to the master clock (e.g. a local oscillator) that governs its control system. In this manuscript we articulate the impact of instabilities in the master clock on qubit phase coherence, and provide tools to calculate the contributions to qubit error arising from these processes. We first connect standard oscillator phase-noise metrics to their corresponding qubit dephasing spectral densities. We then use representative lab-grade and performance-grade oscillator specifications to calculate operational fidelity bounds on trapped-ion and superconducting qubits with relatively slow and fast operation times. We discuss the relevance of these bounds for quantum error correction in contemporary experiments and future large-scale quantum information systems, and discuss potential means to improve master clock stability.
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A major question for condensed matter physics is whether a solid-state quantum computer can ever be built. Here we discuss two different schemes for quantum information processing using semiconductor nanostructures. First, we show how optically driven coupled quantum dots can be used to prepare maximally entangled Bell and Greenberger-Horne-Zeilinger states by varying the strength and duration of selective light pulses. The setup allows us to perform an all-optical generation of the quantum teleportation of an excitonic state in an array of coupled quantum dots. Second, we give a proposal for reliable implementation of quantum logic gates and long decoherence times in a quantum dots system based on nuclear magnetic resonance (NMR), where the nuclear resonance is controlled by the ground state transitions of few-electron QDs in an external magnetic field. The dynamical evolution of these systems in the presence of environmentally-induced decoherence effects is also discussed.
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Spin-bearing molecules are promising building blocks for quantum technologies as they can be chemically tuned, assembled into scalable arrays, and readily incorporated into diverse device architectures. In molecular systems, optically addressing ground-state spins would enable a wide range of applications in quantum information science, as has been demonstrated for solid-state defects. However, this important functionality has remained elusive for molecules. Here, we demonstrate such optical addressability in a series of synthesized organometallic, chromium(IV) molecules. These compounds display a ground-state spin that can be initialized and read out using light, and coherently manipulated with microwaves. In addition, through atomistic modification of the molecular structure, we tune the spin and optical properties of these compounds, paving the way for designer quantum systems synthesized from the bottom-up.
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