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Register a new userNon-Zhang-Rice singlet character of the first ionization state of T-CuO
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Clemens P J Adolphs
Publication date
2016
fields
Physics
and research's language is
English
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We argue that tetragonal CuO (T-CuO) has the potential to finally settle long-standing modelling issues for cuprate physics. We compare the one-hole quasiparticle (qp) dispersion of T-CuO to that of cuprates, in the framework of the strongly-correlated ($U_{dd}rightarrow infty$) limit of the three-band Emery model. Unlike in CuO$_2$, magnetic frustration in T-CuO breaks the $C_4$ rotational symmetry and leads to strong deviations from the Zhang-Rice singlet picture in parts of the reciprocal space. Our results are consistent with angle-resolved photoemission spectroscopy data but in sharp contradiction to those of a one-band model previously suggested for them. These differences identify T-CuO as an ideal material to test a variety of scenarios proposed for explaining cuprate phenomenology.
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The total spectral weight textit{S} of the emergent low-energy quasipaticles in high-temperature superconductors is explored by x-ray absorption spectroscopy. In order to examine the applicability of the Hubbard model, regimes that cover from zero doping to overdoping are investigated. In contrast to mean field theory, we found that textit{S} deviates from linear dependence on the doping level textit{p}. The slope of textit{S} versus textit{p} changes continuously throughout the whole doping range with no sign of saturation up to textit{p} = 0.23. Therefore, the picture of Zhang-Rice singlet remains intact within the most prominent doping regimes of HTSCs.
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