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Register a new userDevelopment of a low background liquid scintillation counter for a shallow underground laboratory
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Pacific Northwest National Laboratory has recently opened a shallow underground laboratory intended for measurement of low-concentration levels of radioactive isotopes in samples collected from the environment. The development of a low-background liquid scintillation counter is currently underway to further augment the measurement capabilities within this underground laboratory. Liquid scintillation counting is especially useful for measuring charged particle (e.g., $beta$, $alpha$) emitting isotopes with no (or very weak) gamma-ray yields. The combination of high-efficiency detection of charged particle emission in a liquid scintillation cocktail coupled with the low-background environment of an appropriately-designed shield located in a clean underground laboratory provides the opportunity for increased-sensitivity measurements of a range of isotopes. To take advantage of the 35 meters-water-equivalent overburden of the underground laboratory, a series of simulations have evaluated the scintillation counters shield design requirements to assess the possible background rate achievable. This report presents the design and background evaluation for a shallow underground, low background liquid scintillation counter design for sample measurements.
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The Boulby Underground Germanium Suite (BUGS) comprises three low background, high-purity germanium detectors operating in the Boulby Underground Laboratory, located 1.1 km underground in the north-east of England, UK. BUGS utilises three types of detector to facilitate a high-sensitivity, high-throughput radioassay programme to support the development of rare-event search experiments. A Broad Energy Germanium (BEGe) detector delivers sensitivity to low-energy gamma-rays such as those emitted by 210Pb and 234Th. A Small Anode Germanium (SAGe) well-type detector is employed for efficient screening of small samples. Finally, a standard p-type coaxial detector provides fast screening of standard samples. This paper presents the steps used to characterise the performance of these detectors for a variety of sample geometries, including the corrections applied to account for cascade summing effects. For low-density materials, BUGS is able to radio-assay to specific activities down to 3.6 mBq/kg for 234Th and 6.6 mBq/kg for 210Pb both of which have uncovered some significant equilibrium breaks in the 238U chain. In denser materials, where gamma-ray self-absorption increases, sensitivity is demonstrated to specific activities of 0.9 mBq/kg for 226Ra, 1.1 mBq/kg for 228 Ra, 0.3 mBq/kg for 224Ra, and 8.6 mBq/kg for 40K with all upper limits at a 90% confidence level. These meet the requirements of most screening campaigns presently under way for rare-event search experiments, such as the LUX-ZEPLIN (LZ) dark matter experiment. We also highlight the ability of the BEGe detector to probe the X-ray fluorescence region which can be important to identify the presence of radioisotopes associated with neutron production; this is of particular relevance in experiments sensitive to nuclear recoils.
The muon intensity and angular distribution in the shallow-underground laboratory Felsenkeller in Dresden, Germany have been studied using a portable muon detector based on the close cathode chamber design. Data has been taken at four positions in Felsenkeller tunnels VIII and IX, where a new 5 MV underground ion accelerator is being installed, and in addition at four positions in Felsenkeller tunnel IV, which hosts a low-radioactivity counting facility. At each of the eight positions studied, seven different orientations of the detector were used to compile a map of the upper hemisphere with 0.85{deg} angular resolution. The muon intensity is found to be suppressed by a factor of 40 due to the 45 m thick rock overburden, corresponding to 140 meters water equivalent. The angular data are matched by two different simulations taking into account the known geodetic features of the terrain: First, simply by determining the cutoff energy using the projected slant depth in rock and the known muon energy spectrum, and second, in a Geant4 simulation propagating the muons through a column of rock equal to the known slant depth. The present data are instrumental for studying muon-induced effects at these depths and also in the planning of an active veto for accelerator-based underground nuclear astrophysics experiments.
The study of low-yield effects requires not only good quality of the original data but also puts high requirements for their processing procedures to increase the efficiency of the selection of useful events. The exploiting of the large cylindrical proportional counters electrostatic topology allows improving the extrapolation of information about the primary ionization of a multipoint event. Long-term calibration measurements with an external $^{109}$Cd-source allowed the development of a new method for analyzing the pulse shape from a sizeable proportional counter. Optimized analysis of the currents pulse shape from the electron cloud of primary ionization in the counter improved the resolution and energy calibration. As a result, the efficiency of selecting useful events was increased by 25%.
Development of ultra low background gas proportional counters has made the contribution from naturally occurring radioactive isotopes -- primarily $alpha$ and $beta$ activity in the uranium and thorium decay chains -- inconsequential to instrumental sensitivity levels when measurements are performed in above ground surface laboratories. Simple lead shielding is enough to mitigate against gamma rays as gas proportional counters are already relatively insensitive to naturally occurring gamma radiation. The dominant background in these surface laboratory measurements using ultra low background gas proportional counters is due to cosmic ray generated muons, neutrons, and protons. Studies of measurements with ultra low background gas proportional counters in surface and underground laboratories as well as radiation transport Monte Carlo simulations suggest a preferred conceptual design to achieve the highest possible sensitivity from an array of low background gas proportional counters when operated in a surface laboratory. The basis for a low background gas proportional counter array and the preferred shielding configuration is reported, especially in relation to measurements of radioactive gases having low energy decays such as $^{37}$Ar.
Low-background experiments with stable ion beams are an important tool for putting the model of stellar hydrogen, helium, and carbon burning on a solid experimental foundation. The pioneering work in this regard has been done by the LUNA collaboration at Gran Sasso, using a 0.4 MV accelerator. In the present contribution, the status of the project for a higher-energy underground accelerator is reviewed. Two tunnels of the Felsenkeller underground site in Dresden, Germany, are currently being refurbished for the installation of a 5 MV high-current Pelletron accelerator. Construction work is on schedule and expected to complete in August 2017. The accelerator will provide intense, 50 uA, beams of 1H+, 4He+, and 12C+ ions, enabling research on astrophysically relevant nuclear reactions with unprecedented sensitivity.
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