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Neutron scattering study of spin ordering and stripe pinning in superconducting La$_{1.93}$Sr$_{0.07}$CuO$_4$

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 Added by John M. Tranquada
 Publication date 2015
  fields Physics
and research's language is English




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The relationships among charge order, spin fluctuations, and superconductivity in underdoped cuprates remain controversial. We use neutron scattering techniques to study these phenomena in La$_{1.93}$Sr$_{0.07}$CuO$_4$, a superconductor with a transition temperature of $T_c = 20$~K. At $Tll T_c$, we find incommensurate spin fluctuations with a quasielastic energy spectrum and no sign of a gap within the energy range from 0.2 to 15 meV. A weak elastic magnetic component grows below $sim10$~K, consistent with results from local probes. Regarding the atomic lattice, we have discovered unexpectedly strong fluctuations of the CuO$_6$ octahedra about Cu-O bonds, which are associated with inequivalent O sites within the CuO$_2$ planes. Furthermore, we observed a weak elastic $(3bar{3}0)$ superlattice peak that implies a reduced lattice symmetry. The presence of inequivalent O sites rationalizes various pieces of evidence for charge stripe order in underdoped lsco. The coexistence of superconductivity with quasi-static spin-stripe order suggests the presence of intertwined orders; however, the rotation of the stripe orientation away from the Cu-O bonds might be connected with evidence for a finite gap at the nodal points of the superconducting gap function.

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81 - S. Sugai , N. Hayamizu 2000
The dynamical stripe structure relating to the 1/8 problem was investigated in La$_{2-x}$Sr$_x$CuO$_4$ utilizing the high frequency response of Raman scattering. The split of the two-magnon peak due to the formation of the stripe structure was observed at whole Sr concentration region from $x=0.035$ to 0.25 at low temperatures. Especially clear split was observed at low carrier concentration region $x=0.035 - 0.06$ and at $x sim 1/8$. The onset temperatures of these stripe structures are as high as 300-350 K, which are much higher than the temperatures measured by slow response probes.
We study superconducting properties in multilayer thin films consisting of superconducting La$_{1.85}$Sr$_{0.15}$CuO$_4$ (LSCO) and Mott insulator Sr$_2$IrO$_4$ (SIO) and report enhanced superconductivity in optimized sample. These multilayer heterostructures show an increase in superconducting transition temperature ($T_C$) as compared to the single layer LSCO films. The temperature dependence of SIO single layer is also investigated under thermal activation, Arrhenius-type behaviour, and variable-range hopping mechanisms for different temperature regimes. The decrease in $T_C$ beyond an optimum thickness of LSCO in these multilayers is analyzed in the framework of a model based on the assumption of induced superconductivity in SIO-LSCO interface due to the doping of La and/or oxygen deficiencies into SIO layers
We present results of inelastic light scattering experiments on single-crystalline La$_{2-x}$Sr$_{x}$CuO$_4$ in the doping range $0.00 le x=p le 0.30$ and Tl$_2$Ba$_2$CuO$_{6+delta}$ at $p=0.20$ and $p=0.24$. The main emphasis is placed on the response of electronic excitations in the antiferromagnetic phase, in the pseudogap range, in the superconducting state, and in the essentially normal metallic state at $x ge 0.26$, where no superconductivity could be observed. In most of the cases we compare B$_{1g}$ and B$_{2g}$ spectra which project out electronic properties close to $(pi,0)$ and $(pi/2, pi/2)$, respectively. In the channel of electron-hole excitations we find universal behavior in B$_{2g}$ symmetry as long as the material exhibits superconductivity at low temperature. In contrast, there is a strong doping dependence in B$_{1g}$ symmetry: (i) In the doping range $0.20 le p le 0.25$ we observe rapid changes of shape and temperature dependence of the spectra. (ii) In La$_{2-x}$Sr$_{x}$CuO$_4$ new structures appear for $x < 0.13$ which are superposed on the electron-hole continuum. The temperature dependence as well as model calculations support an interpretation in terms of charge-ordering fluctuations. For $x le 0.05$ the response from fluctuations disappears at B$_{1g}$ and appears at B$_{2g}$ symmetry in full agreement with the orientation change of stripes found by neutron scattering. While, with a grain of salt, the particle-hole continuum is universal for all cuprates the response from fluctuating charge order in the range $0.05 le p < 0.16$ is so far found only in La$_{2-x}$Sr$_{x}$CuO$_4$. We conclude that La$_{2-x}$Sr$_{x}$CuO$_4$ is close to static charge order and, for this reason, may have a suppressed $T_c$.
Neutron diffraction has been a very prominent tool to investigate high-temperature superconductors, in particular through the discovery of an incommensurate magnetic signal known as stripes. We here report the findings of a neutron diffraction experiment on the superconductor (La,Sr)$_2$CuO$_4$, where a spurious signal appeared to be magnetic stripes. The signal strength was found to be strongly dependent on the neutron energy, peaking at $E = 4.6$~meV. We therefore attribute the origin of this signal to be a combination of multiple scattering and crystal twinning. A forward calculation of the scattering intensity including these two effects almost completely recovers our experimental observations. We emphasise the need for employing such analysis when searching for ways to avoid spurious scattering signals.
We report the observation of a bulk charge modulation in La$_{1.88}$Sr$_{0.12}$CuO$_4$ (LSCO) with a characteristic in-plane wave-vector of (0.236, $pm delta$), with $delta$=0.011 r.l.u. The transverse shift of the ordering wave-vector indicates the presence of rotated charge-stripe ordering, demonstrating that the charge ordering is not pinned to the Cu-O bond direction. On cooling through the superconducting transition, we find an abrupt change in the growth of the charge correlations and a suppression of the charge order parameter indicating competition between the two orderings. Orthorhombic LSCO thus helps bridge the apparent disparities between the behavior previously observed in the tetragonal 214 cuprates and the orthorhombic yttrium and bismuth-based cuprates and thus lends strong support to the idea that there is a common motif to charge order in all cuprate families.
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