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Register a new userDynamical Mechanism of Two-Dimensional Plasmon Launching by Swift Electrons
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Launching of surface plasmons by swift electrons has long been utilized in electron-energy-loss spectroscopy (EELS) to investigate plasmonic properties of ultrathin, or two-dimensional (2D), electron systems. However, its spatio-temporal process has never been revealed. This is because the impact of an electron will generate not only plasmons, but also photons, whose emission cannot be achieved at a single space-time point, as fundamentally determined from the uncertainty principle. Here, we propose that such a space-time limitation also applies to surface plasmon generation in EELS experiment. On the platform of graphene, we demonstrate within the framework of classical electrodynamics that the launching of 2D plasmons by an electrons impact is delayed after a hydrodynamic splashing-like process, which occurs during the plasmonic formation time when the electron traverses the formation zone. Considering this newly revealed process, we show that previous estimates on the yields of graphene plasmons in EELS have been overestimated.
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Diffraction of light at lateral inhomogenities is a central process in the near-field studies of nanoscale phenomena, especially the propagation of surface waves. Theoretical description of this process is extremely challenging due to breakdown of plane-wave methods. Here, we present and analyze an exact solution for electromagnetic wave diffraction at the linear junction between two-dimensional electron systems (2DES) with dissimilar surface conductivities. The field at the junction is a combination of three components with different spatial structure: free-field component, non-resonant edge component, and surface plasmon-polariton (SPP). We find closed-form expressions for efficiency of photon-to-plasmon conversion by the edge being the ratio of electric fields in SPP and incident wave. Particularly, the conversion efficiency can considerably exceed unity for the contact between metal and 2DES with large impedance. Our findings can be considered as a first step toward quantitative near-field microscopy of inhomogeneous systems and polaritonic interferometry.
We experimentally demonstrate the use of subwavelength optical nanoantennae to assist the gentle ablation of nanostructures directly using ultralow fluence from a Ti: sapphire oscillator through the excitation of surface plasmon waves. We show that this ablation mechanism is the same for metal and dielectric. The analytical solutions of ablation threshold are in excellent agreement with the experiment estimations. Surface plasmon assisted locally enhanced ablation at nanoscale provides a method for nanomachining, manipulation and modification the nanostructures without collateral thermal damage to the materials. It is also shown that this ablation can deposit low-density high quality thin nano film.
Bandgap control is of central importance for semiconductor technologies. The traditional means of control is to dope the lattice chemically, electrically or optically with charge carriers. Here, we demonstrate for the first time a widely tunable bandgap (renormalisation up to 650 meV at room-temperature) in two-dimensional (2D) semiconductors by coherently doping the lattice with plasmonic hot electrons. In particular, we integrate tungsten-disulfide (WS$_2$) monolayers into a self-assembled plasmonic crystal, which enables coherent coupling between semiconductor excitons and plasmon resonances. Accompanying this process, the plasmon-induced hot electrons can repeatedly fill the WS$_2$ conduction band, leading to population inversion and a significant reconstruction in band structures and exciton relaxations. Our findings provide an innovative and effective measure to engineer optical responses of 2D semiconductors, allowing a great flexiblity in design and optimisation of photonic and optoelectronic devices.
Interference between light waves is one of the widely known phenomena in physics, which is widely used in modern optics, ranging from precise detection at the nanoscale to gravitational-wave observation. Akin to light, both classical and quantum interferences between surface plasmon polaritons (SPPs) have been demonstrated. However, to actively control the SPP interference within subcycle in time (usually less than several femtoseconds in the visible range) is still missing, which hinders the ultimate manipulation of SPP interference on ultrafast time scale. In this paper, the interference between SPPs launched by a hole dimer, which was excited by a grazing incident free electron beam without direct contact, was manipulated through both propagation and initial phase difference control. Particularly, using cathodoluminescence spectroscopy, the appearance of higher-order interference orders was obtained through propagation phase control by increasing separation distances of the dimer. Meanwhile, the peak-valley-peak evolution at a certain wavelength through changing the accelerating voltages was observed, which originates from the initial phase difference control of hole launched SPPs. In particular, the time resolution of this kind of control is shown to be in the ultrafast attosecond (as) region. Our work suggests that fast electron beams can be an efficient tool to control polarition interference in subcycle temporal scale, which can be potentially used in ultrafast optical processing or sensing.
We investigate the spin dynamics of high-mobility two-dimensional electrons in GaAs/AlGaAs quantum wells grown along the $[001]$ and $[110]$ directions by time-resolved Faraday rotation at low temperatures. In measurements on the $(001)$-grown structures without external magnetic fields, we observe coherent oscillations of the electron spin polarization about the effective spin-orbit field. In non-quantizing magnetic fields applied normal to the sample plane, the cyclotron motion of the electrons rotates the effective spin-orbit field. This rotation leads to fast oscillations in the spin polarization about a non-zero value and a strong increase in the spin dephasing time in our experiments. These two effects are absent in the $(110)$-grown structure due to the different symmetry of its effective spin-orbit field. The measurements are in excellent agreement with our theoretical model.
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