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Register a new userTopological Map of the Hofstadter Butterfly and Van Hove Singularities
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The Hofstadter butterfly is a quantum fractal with a highly complex nested set of gaps, where each gap represents a quantum Hall state whose quantized conductivity is characterized by topological invariants known as the Chern numbers. Here we obtain simple rules to determine the Chern numbers at all scales in the butterfly fractal and lay out a very detailed topological map of the butterfly. Our study reveals the existence of a set of critical points, each corresponding to a macroscopic annihilation of orderly patterns of both the positive and the negative Cherns that appears as a fine structure in the butterfly. Such topological collapses are identified with the Van Hove singularities that exists at every band center in the butterfly landscape. We thus associate a topological character to the Van Hove anomalies. Finally, we show that this fine structure is amplified under perturbation, inducing quantum phase transitions to higher Chern states in the system.
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Wave kinetic theory has been developed to describe the statistical dynamics of weakly nonlinear, dispersive waves. However, we show that systems which are generally dispersive can have resonant sets of wave modes with identical group velocities, leading to a local breakdown of dispersivity. This shows up as a geometric singularity of the resonant manifold and possibly as an infinite phase measure in the collision integral. Such singularities occur widely for classical wave systems, including acoustical waves, Rossby waves, helical waves in rotating fluids, light waves in nonlinear optics and also in quantum transport, e.g. kinetics of electron-hole excitations (matter waves) in graphene. These singularities are the exact analogue of the critical points found by Van Hove in 1953 for phonon dispersion relations in crystals. The importance of these singularities in wave kinetics depends on the dimension of phase space $D=(N-2)d$ ($d$ physical space dimension, $N$ the number of waves in resonance) and the degree of degeneracy $delta$ of the critical points. Following Van Hove, we show that non-degenerate singularities lead to finite phase measures for $D>2$ but produce divergences when $Dleq 2$ and possible breakdown of wave kinetics if the collision integral itself becomes too large (or even infinite). Similar divergences and possible breakdown can occur for degenerate singularities, when $D-deltaleq 2,$ as we find for several physical examples, including electron-hole kinetics in graphene. When the standard kinetic equation breaks down, then one must develop a new singular wave kinetics. We discuss approaches from pioneering 1971 work of Newell & Aucoin on multi-scale perturbation theory for acoustic waves and field-theoretic methods based on exact Schwinger-Dyson integral equations for the wave dynamics.
Van Hove singularity are electronic instabilities that lead to many fascinating interactions, such as superconductivity and charge-density waves. And despite much interest, the nexus of emergent correlation effects from van Hove singularities and topological states of matter remains little explored in experiments. By utilizing synchrotron-based angle-resolved photoemission spectroscopy and Density Functional Theory, here we provide the first discovery of the helicoid quantum nature of topological Fermi arcs inducing van Hove singularities. In particular, in topological chiral conductors RhSi and CoSi we directly observed multiple types of inter- and intra-helicoid-arc mediated singularities, which includes the type-I and type-II van Hove singularity. We further demonstrate that the energy of the helicoid-arc singularities are easily tuned by chemical engineering. Taken together, our work provides a promising route to engineering new electronic instabilities in topological quantum materials.
We study distributions of the ratios of level spacings of a rectangular and an Africa-shaped superconducting microwave resonator containing circular scatterers on a triangular grid, so-called Dirac billiards (DBs). The high-precision measurements allowed the determination of all 1651 and 1823 eigenfrequencies in the first two bands, respectively. The resonance densities are similar to that of graphene. They exhibit two sharp peaks at the van Hove singularities, that separate the band structure into regions with a linear and a quadratic dispersion relation, respectively. In their vicinity we observe rapid changes, e.g., in the wavefunction structure. Accordingly, the question arose, whether there the spectral properties are still determined by the shapes of the DBs. The commonly used statistical measures, however, are no longer applicable whereas, as demonstrated in this Letter, the ratio distributions provide most suitable ones.
In this work, we study the topological phases of the dimerized square lattice in the presence of an external magnetic field. The dimerization pattern in the lattices hopping amplitudes can induce a series of bulk energy gap openings in the Hofstadter spectrum at certain fractional fillings, giving rise to various topological phases. In particular, we show that at $frac{1}{2}$-filling the topological quadrupole insulator phase with a quadrupole moment quantized to $frac{e}{2}$ and associated corner-localized mid-gap states exists in certain parameter regime for all magnetic fluxes. At $frac{1}{4}$ filling, the system can host obstructed atomic limit phases or Chern insulator phases. For those configurations gapped at fillings below $frac{1}{4}$, the system is in Chern insulator phases of various non-vanishing Chern numbers. Across the phase diagram, both bulk-obstructed and boundary-obstructed topological phase transitions exist in this model.
The possibility of triggering correlated phenomena by placing a singularity of the density of states near the Fermi energy remains an intriguing avenue towards engineering the properties of quantum materials. Twisted bilayer graphene is a key material in this regard because the superlattice produced by the rotated graphene layers introduces a van Hove singularity and flat bands near the Fermi energy that cause the emergence of numerous correlated phases, including superconductivity. While the twist angle-dependence of these properties has been explored, direct demonstration of electrostatic control of the superlattice bands over a wide energy range has, so far, been critically missing. This work examines a functional twisted bilayer graphene device using in-operando angle-resolved photoemission with a nano-focused light spot. A twist angle of 12.2$^{circ}$ is selected such that the superlattice Brillouin zone is sufficiently large to enable identification of van Hove singularities and flat band segments in momentum space. The doping dependence of these features is extracted over an energy range of 0.4 eV, expanding the combinations of twist angle and doping where they can be placed at the Fermi energy and thereby induce new correlated electronic phases in twisted bilayer graphene.
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