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Deterministic Coherent Writing of a Long-Lived Semiconductor Spin Qubit Using One Ultrafast Optical Pulse

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 Added by Emma Schmidgall
 Publication date 2015
  fields Physics
and research's language is English




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We use one single, few-picosecond-long, variably polarized laser pulse to deterministically write any selected spin state of a quantum dot confined dark exciton whose life and coherence time are six and five orders of magnitude longer than the laser pulse duration, respectively. The pulse is tuned to an absorption resonance of an excited dark exciton state, which acquires non-negligible oscillator strength due to residual mixing with bright exciton states. We obtain a high fidelity one-to-one mapping from any point on the Poincare sphere of the pulse polarization to a corresponding point on the Bloch sphere of the spin of the deterministically photogenerated dark exciton.



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We demonstrate a one to one correspondence between the polarization state of a light pulse tuned to neutral exciton resonances of single semiconductor quantum dots and the spin state of the exciton that it photogenerates. This is accomplished using two variably polarized and independently tuned picosecond laser pulses. The first writes the spin state of the resonantly excited exciton. The second is tuned to biexcitonic resonances, and its absorption is used to read the exciton spin state. The absorption of the second pulse depends on its polarization relative to the exciton spin direction. Changes in the exciton spin result in corresponding changes in the intensity of the photoluminescence from the biexciton lines which we monitor, obtaining thus a one to one mapping between any point on the Poincare sphere of the light polarization to a point on the Bloch sphere of the exciton spin.
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We report the experimental realization of a 3D capacitively-shunt superconducting flux qubit with long coherence times. At the optimal flux bias point, the qubit demonstrates energy relaxation times in the 60-90 $mu$s range, and Hahn-echo coherence time of about 80 $mu$s which can be further improved by dynamical decoupling. Qubit energy relaxation can be attributed to quasiparticle tunneling, while qubit dephasing is caused by flux noise away from the optimal point. Our results show that 3D c-shunt flux qubits demonstrate improved performance over other types of flux qubits which is advantageous for applications such as quantum magnetometry and spin sensing.
Semiconductor qubits rely on the control of charge and spin degrees of freedom of electrons or holes confined in quantum dots (QDs). They constitute a promising approach to quantum information processing [1, 2], complementary to superconducting qubits [3]. Typically, semiconductor qubit-qubit coupling is short range [1, 2, 4, 5], effectively limiting qubit distance to the spatial extent of the wavefunction of the confined particle, which represents a significant constraint towards scaling to reach dense 1D or 2D arrays of QD qubits. Following the success of circuit quantum eletrodynamics [6], the strong coupling regime between the charge [7, 8] and spin [9, 10, 11] degrees of freedom of electrons confined in semiconducting QDs interacting with individual photons stored in a microwave resonator has recently been achieved. In this letter, we demonstrate coherent coupling between a superconducting transmon qubit and a semiconductor double quantum dot (DQD) charge qubit mediated by virtual microwave photon excitations in a tunable high-impedance SQUID array resonator acting as a quantum bus [12, 13, 14]. The transmon-charge qubit coherent coupling rate ($ sim$ 21 MHz) exceeds the linewidth of both the transmon ($ sim$ 0.8 MHz) and the DQD charge ($ sim$ 3 MHz) qubit. By tuning the qubits into resonance for a controlled amount of time, we observe coherent oscillations between the constituents of this hybrid quantum system. These results enable a new class of experiments exploring the use of the two-qubit interactions mediated by microwave photons to create entangled states between semiconductor and superconducting qubits. The methods and techniques presented here are transferable to QD devices based on other material systems and can be beneficial for spin-based hybrid systems.
We demonstrate that the quantum dot-confined dark exciton forms a long-lived integer spin solid state qubit which can be deterministically on-demand initiated in a pure state by one optical pulse. Moreover, we show that this qubit can be fully controlled using short optical pulses, which are several orders of magnitude shorter than the life and coherence times of the qubit. Our demonstrations do not require an externally applied magnetic field and they establish that the quantum dot-confined dark exciton forms an excellent solid state matter qubit with some advantages over the half-integer spin qubits such as the confined electron and hole, separately. Since quantum dots are semiconductor nanostructures that allow integration of electronic and photonic components, the dark exciton may have important implications on implementations of quantum technologies consisting of semiconductor qubits.
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