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Register a new userCancellation of Collisional Frequency Shifts in Optical Lattice Clocks with Rabi Spectroscopy
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We analyze both the s- and p-wave collision induced frequency shifts and propose a over-$pi$ pulse scheme to cancel the shifts in optical lattice clocks interrogated by a Rabi pulse. The collisional frequency shifts are analytically solved as a function of the pulse area and the inhomogeneity of the Rabi frequencies. Experimentally measured collisional frequency shifts in an Yb optical lattice clock are in good agreement with the analytical calculations. Based on our analysis, the over-$pi$ pulse combined with a small inhomogeneity below 0.1 allows a fractional uncertainty on a level of $10^{-18}$ in both Sr and Yb optical lattice clocks by canceling the collisional frequency shift.
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We have quantified collisional losses, decoherence and the collision shift in a one-dimensional optical lattice clock with bosonic 88Sr. The lattice clock is referenced to the highly forbidden transition 1S0 - 3P0 at 698 nm, which becomes weakly allowed due to state mixing in a homogeneous magnetic field. We were able to quantify three decoherence coefficients, which are due to dephasing collisions, inelastic collisions between atoms in the upper and lower clock state, and atoms in the upper clock state only. Based on the measured coefficients, we determine the operation parameters at which a 1D-lattice clock with 88Sr shows no degradation due to collisions on the relative accuracy level of 10-16.
Collisions with background gas particles can shift the resonance frequencies of atoms in atomic clocks. The internal quantum states of atoms can also become entangled with their motional states due to the recoil imparted by a collision, which leads to a further shift of the clock frequency through the relativistic Doppler shift. It can be complicated to evaluate the Doppler and collisional frequency shifts for clock atoms in such entangled states, but estimates of these shifts are essential in order to improve the accuracy of optical atomic clocks. We present a formalism that describes collisions and relativistic Doppler shifts in a unified manner, and can therefore be used to accurately estimate collisional frequency shifts in trapped-atom clocks.
Recent realisation of three-dimensional optical lattice clocks circumvents short range collisional clock shifts which have been the bottle neck towards higher precision; the long range electronic dipole-dipole interaction between the atoms becomes the primary source of clock shift due to interatomic interactions. We study the Rabi spectroscopy of three-dimensional optical lattice clocks with unity filling. From the Lindblad equation governing the time evolution of the density matrix of the atoms, we derive the Bloch equations in the presence of the external Rabi driving laser field, and solve the equations approximately to the first order of the coupling strength of the dipole-dipole interaction between the atoms. We find that the clock shift equals to the product of the coupling strength, a factor determined by the parameters of the Rabi pulse, and another factor depending on the configuration of the three-dimensional optical lattice. Our result on the clock shift within the Rabi spectroscopy can be checked by measurement in future experiment.
Collisions between background gas particles and the trapped ion in an atomic clock can subtly shift the frequency of the clock transition. The uncertainty in the correction for this effect makes a significant contribution to the total systematic uncertainty budget of trapped-ion clocks. Using a non-perturbative analytic framework that was developed for this problem, we estimate the frequency shift in Al$^+$ ion clocks due to collisions with helium and hydrogen. Our calculations significantly improve the uncertainties in the collisional shift coefficients, and show that the collisional frequency shifts for Al$^+$ are zero to within uncertainty.
We develop a model to describe the motional (i.e., external degree of freedom) energy spectra of atoms trapped in a one-dimensional optical lattice, taking into account both axial and radial confinement relative to the lattice axis. Our model respects the coupling between axial and radial degrees of freedom, as well as other anharmonicities inherent in the confining potential. We further demonstrate how our model can be used to characterize lattice light shifts in optical lattice clocks, including shifts due to higher multipolar (magnetic dipole and electric quadrupole) and higher order (hyperpolarizability) coupling to the lattice field. We compare results for our model with results from other lattice light shift models in the literature under similar conditions.
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