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Register a new userInverse magneto-refraction as a mechanism for laser modification of spin-spin exchange parameters and subsequent terahertz emission from iron oxides
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Added by
Rostislav Mikhaylovskiy
Publication date
2014
fields
Physics
and research's language is
English
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Ultrafast non-thermal manipulation of magnetization by light relies on either indirect coupling of the electric field component of the light with spins via spin-orbit interaction or direct coupling between the magnetic field component and spins. Here we propose a novel scenario for coupling between the electric field of light and spins via optical modification of the exchange interaction, one of the strongest quantum effects, the strength of which can reach 1000 Tesla. We demonstrate that this isotropic opto-magnetic effect, which can be called the inverse magneto-refraction, is allowed in a material of any symmetry. Its existence is corroborated by the experimental observation of THz emission by magnetic-dipole active spin resonances optically excited in a broad class of iron oxides with a canted spin configuration. From its strength we estimate that a sub-picosecond laser pulse with a moderate fluence of ~ 1 mJ/cm^2 acts as a pulsed effective magnetic field of 0.01 Tesla, arising from the optically perturbed balance between the exchange parameters. Our findings are supported by a low-energy theory for the microscopic magnetic interactions between non-equilibrium electrons subjected to an optical field which suggests a possibility to modify the exchange interactions by light over 1 %.
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Control of quantum coherence in many-body system is one of the key issues in modern condensed matter. Conventional wisdom is that lattice vibration is an innate source of decoherence, and amounts of research have been conducted to eliminate lattice effects. Challenging this wisdom, here we show that lattice vibration may not be a decoherence source but an impetus of a novel coherent quantum many-body state. We demonstrate the possibility by studying the transverse-field Ising model on a chain with renormalization group and density-matrix renormalization group method, and theoretically discover a stable $mathcal{N}=1$ supersymmetric quantum criticality with central charge $c=3/2$. Thus, we propose an Ising spin chain with strong spin-lattice coupling as a candidate to observe supersymmetry. Generic precursor conditions of novel quantum criticality are obtained by generalizing the Larkin-Pikin criterion of thermal transitions. Our work provides a new perspective that lattice vibration may be a knob for exotic quantum many-body states.
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