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Register a new userIsometric fluctuation relations for equilibrium states with broken symmetry
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We derive a set of isometric fluctuation relations, which constrain the order parameter fluctuations in finite-size systems at equilibrium and in the presence of a broken symmetry. These relations are exact and should apply generally to many condensed-matter physics systems. Here, we establish these relations for magnetic systems and nematic liquid crystals in a symmetry-breaking external field, and we illustrate them on the Curie-Weiss and the $XY$ models. Our relations also have implications for spontaneous symmetry breaking, which are discussed.
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Fluctuation-dissipation relations or theorems (FDTs) are fundamental for statistical physics and can be rigorously derived for equilibrium systems. Their applicability to non-equilibrium systems is, however, debated. Here, we simulate an active microrheology experiment, in which a spherical colloid is pulled with a constant external force through a fluid, creating near-equilibrium and far-from-equilibrium systems. We characterize the structural and dynamical properties of these systems, and reconstruct an effective generalized Langevin equation (GLE) for the colloid dynamics. Specifically, we test the validity of two FDTs: The first FDT relates the non-equilibrium response of a system to equilibrium correlation functions, and the second FDT relates the memory friction kernel in the GLE to the stochastic force. We find that the validity of the first FDT depends strongly on the strength of the external driving: it is fulfilled close to equilibrium and breaks down far from it. In contrast, we observe that the second FDT is always fulfilled. We provide a mathematical argument why this generally holds for memory kernels reconstructed from a deterministic Volterra equation for correlation functions, even for non-stationary non-equilibrium systems. Motivated by the Mori-Zwanzig formalism, we therefore suggest to impose an orthogonality constraint on the stochastic force, which is in fact equivalent to the validity of this Volterra equation. Such GLEs automatically satisfy the second FDT and are unique, which is desirable when using GLEs for coarse-grained modeling.
We provide numerical evidence that the Onsager symmetry remains valid for systems subject to a spatially dependent magnetic field, in spite of the broken time-reversal symmetry. In addition, for the simplest case in which the field strength varies only in one direction, we analytically derive the result. For the generic case, a qualitative explanation is provided.
We study the effects of the finite number of experimental data on the computation of a generalized fluctuation-dissipation relation around a nonequilibrium steady state of a Brownian particle in a toroidal optical trap. We show that the finite sampling has two different effects, which can give rise to a poor estimate of the linear response function. The first concerns the accessibility of the generalized fluctuation-dissipation relation due to the finite number of actual perturbations imposed to the control parameter. The second concerns the propagation of the error made at the initial sampling of the external perturbation of the system. This can be highly enhanced by introducing an estimator which corrects the error of the initial sampled condition. When these two effects are taken into account in the data analysis, the generalized fluctuation-dissipation relation is verified experimentally.
We study Fluctuation Relations (FRs) for dynamics that are anomalous, in the sense that the diffusive properties strongly deviate from the ones of standard Brownian motion. We first briefly review the concept of transient work FRs for stochastic dynamics modeled by the ordinary Langevin equation. We then introduce three generic types of dynamics generating anomalous diffusion: Levy flights, long-time correlated Gaussian stochastic processes and time-fractional kinetics. By combining Langevin and kinetic approaches we calculate the work probability distributions in the simple nonequilibrium situation of a particle subject to a constant force. This allows us to check the transient FR for anomalous dynamics. We find a new form of FRs, which is intimately related to the validity of fluctuation-dissipation relations. Analogous results are obtained for a particle in a harmonic potential dragged by a constant force. We argue that these findings are important for understanding fluctuations in experimentally accessible systems. As an example, we discuss the anomalous dynamics of biological cell migration both in equilibrium and in nonequilibrium under chemical gradients.
We unveil the universal (model-independent) symmetry satisfied by Schwinger-Keldysh quantum field theories whenever they describe equilibrium dynamics. This is made possible by a generalization of the Schwinger-Keldysh path-integral formalism in which the physical time can be re-parametrized to arbitrary contours in the complex plane. Strong relations between correlation functions, such as the fluctuation-dissipation theorems, are derived as immediate consequences of this symmetry of equilibrium. In this view, quantum non-equilibrium dynamics -- e.g. when driving with a time-dependent potential -- are seen as symmetry-breaking processes. The symmetry-breaking terms of the action are identified as a measure of irreversibility, or entropy creation, defined at the level of a single quantum trajectory. Moreover, they are shown to obey quantum fluctuation theorems. These results extend stochastic thermodynamics to the quantum realm.
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