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Register a new userThermal transport in out of equilibrium quantum harmonic chains
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Added by
Fernando Nicacio Ph.D.
Publication date
2014
fields
Physics
and research's language is
English
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We address the problem of heat transport in a chain of coupled quantum harmonic oscillators, exposed to the influences of local environments of various nature, stressing the effects that the specific nature of the environment has on the phenomenology of the transport process. We study in detail the behavior of thermodynamically relevant quantities such as heat currents and mean energies of the oscillators, establishing rigorous analytical conditions for the existence of a steady state, whose features we analyse carefully. In particular we assess the conditions that should be faced to recover trends reminiscent of the classical Fourier law of heat conduction and highlight how such a possibility depends on the environment linked to our system.
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In d-dimensional lattices of coupled quantum harmonic oscillators, we analyze the heat current caused by two thermal baths of different temperature, which are coupled to opposite ends of the lattice, with focus on the validity of Fouriers law of heat conduction. We provide analytical solutions of the heat current through the quantum system in the non-equilibrium steady state using the rotating-wave approximation and bath interactions described by a master equation of Lindblad form. The influence of local dephasing in the transition of ballistic to diffusive transport is investigated.
We discuss how the thermalization of an elementary quantum system is modified when the system is placed in an environment out of thermal equilibrium. To this aim we provide a detailed investigation of the dynamics of an atomic system placed close to a body of arbitrary geometry and dielectric permittivity, whose temperature $T_M$ is different from that of the surrounding walls $T_W$. A suitable master equation for the general case of an $N$-level atom is first derived and then specialized to the cases of a two- and three-level atom. Transition rates and steady states are explicitly expressed as a function of the scattering matrices of the body and become both qualitatively and quantitatively different from the case of radiation at thermal equilibrium. Out of equilibrium, the system steady state depends on the system-body distance, on the geometry of the body and on the interplay of all such parameters with the body optical resonances. While a two-level atom tends toward a thermal state, this is not the case already in the presence of three atomic levels. This peculiar behavior can be exploited, for example, to invert the populations ordering and to provide an efficient cooling mechanism for the internal state of the quantum system. We finally provide numerical studies and asymptotic expressions when the body is a slab of finite thickness. Our predictions can be relevant for a wide class of experimental configurations out of thermal equilibrium involving different physical realizations of two or three-level systems.
Harmonic oscillator chains connecting two harmonic reservoirs at different constant temperatures cannot act as thermal diodes, irrespective of structural asymmetry. However, here we prove that perfectly harmonic junctions can rectify heat once the reservoirs (described by white Langevin noise) are placed under temperature gradients, which are asymmetric at the two sides, an effect that we term temperature-gradient harmonic oscillator diodes. This nonlinear diode effect results from the additional constraint -- the imposed thermal gradient at the boundaries. We demonstrate the rectification behavior based on the exact analytical formulation of steady state heat transport in harmonic systems coupled to Langevin baths, which can describe quantum and classical transport, both regimes realizing the diode effect under the involved boundary conditions. Our study shows that asymmetric harmonic systems, such as room-temperature hydrocarbon molecules with varying side groups and end groups, or a linear lattice of trapped ions may rectify heat by going beyond simple boundary conditions.
We study the internal dynamics of an elementary quantum system placed close to a body held at a temperature different from that of the surrounding radiation. We derive general expressions for lifetime and density matrix valid for bodies of arbitrary geometry and dielectric permittivity. Out of equilibrium, the thermalization process and steady states become both qualitatively and quantitatively significantly different from the case of radiation at thermal equilibrium. For the case of a three-level atom close to a slab of finite thickness, we predict the occurrence of population inversion and an efficient cooling mechanism for the quantum system, whose effective internal temperature can be driven to values much lower than both involved temperatures. Our results show that non-equilibrium configurations provide new promising ways to control the state of an atomic system.
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