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The discovery of high temperature superconductivity in the cuprates in 1986 triggered a spectacular outpouring of creative and innovative scientific inquiry. Much has been learned over the ensuing 28 years about the novel forms of quantum matter that are exhibited in this strongly correlated electron system. This progress has been made possible by improvements in sample quality, coupled with the development and refinement of advanced experimental techniques. In part, avenues of inquiry have been motivated by theoretical developments, and in part new theoretical frameworks have been conceived to account for unanticipated experimental observations. An overall qualitative understanding of the nature of the superconducting state itself has been achieved, while profound unresolved issues have come into increasingly sharp focus concerning the astonishing complexity of the phase diagram, the unprecedented prominence of various forms of collective fluctuations, and the simplicity and insensitivity to material details of the normal state at elevated temperatures. New conceptual approaches, drawing from string theory, quantum information theory, and various numerically implemented approximate approaches to problems of strong correlations are being explored as ways to come to grips with this rich tableaux of interrelated phenomena.
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We present a comparative study of magnetic excitations in the first two Ruddlesden-Popper members of the Hg-family of high-temperature superconducting cuprates, which are chemically nearly identical and have the highest critical temperature ($T_mathrm{c}$) among all cuprate families. Our inelastic photon scattering experiments reveal that the two compounds paramagnon spectra are nearly identical apart from an energy scale factor of $sim130%$ that matches the ratio of $T_mathrm{c}$s, as expected in magnetic Cooper pairing theories. By relating our observations to other cuprates, we infer that the strength of magnetic interactions determines how high $T_mathrm{c}$ can reach. Our finding can be viewed as a magnetic analogue of the isotope effect, thus firmly supporting models of magnetically mediated high-temperature superconductivity.
Besides superconductivity, copper-oxide high temperature superconductors are susceptible to other types of ordering. We use scanning tunneling microscopy and resonant elastic x-ray scattering measurements to establish the formation of charge ordering in the high-temperature superconductor Bi2Sr2CaCu2O8+x. Depending on the hole concentration, the charge ordering in this system occurs with the same period as those found in Y-based or La-based cuprates, and displays the analogous competition with superconductivity. These results indicate the similarity of charge organization competing with superconductivity across different families of cuprates. We observe this charge ordering to leave a distinct electron-hole asymmetric signature (and a broad resonance centered at +20 meV) in spectroscopic measurements, thereby indicating that it is likely related to the organization of holes in a doped Mott insulator.
Recent experiments in the cuprates have seen evidence of a transient superconducting state upon optical excitation polarized along the c-axis [R. Mankowsky et al., Nature 516, 71 (2014)]. Motivated by these experiments we propose an extension of the single-layer $t-J-V$ model of cuprates to three dimensions in order to study the effects of inter-plane tunneling on the competition between superconductivity and bond density wave order. We find that an optical pump can suppress the charge order and simultaneously enhance superconductivity, due to the inherent competition between the two. We also provide an intuitive picture of the physical mechanism underlying this effect. Furthermore, based on a simple Floquet theory we estimate the magnitude of the enhancement.
The transition mechanism in high temperature cuprate superconductors is an outstanding puzzle. A previous suggestion on the role of non-linear local lattice instability modes on the microscopic pairing mechanism in high temperature cuprate superconductors cite{Lee:JSNM09} is re-examined to provide a viable mechanism for superconductivity in these cuprates via an unusual lattice vibration in which an electron is predominantly interacting with a nonlinear $Q_2$ mode of the oxygen clusters in the CuO$_2$ planes. It is shown that the interaction has explicit d-wave symmetry and leads to an indirect coupling of d-wave symmetry between electrons. As a follow-up of cite{Lee:JSNM09}, in this paper, we report detailed derivation of the superconducting gap equation and numerical solutions for the transition temperature as inherently integrated into the so-called Extended Hubbard Model (EHM). A unique feature in the EHM is that the transition temperature has an inherent k-dependence. In addition, superconducting gap solutions are restrained to specific regions in the first Brillouin zone (1BZ). It is very feasible to expect that the EHM naturally inherits a huge parameter space in which experimentally measured results, such as the well-known superconducting dome and the phase diagram from electronic Raman scattering cite{Sacuto:RPP13} can be accommodated. The EHM model hence offers a viable venue to search for or confirm any signature in k-point-sensitive experimental measurements.
Subsequent to our recent report of SDW type transition at 190 K and antiferromagnetic order below 20 K in EuFe2As2, we have studied the effect of K-doping on the SDW transition at high temperature and AF order at low temperature. 50% K doping suppresses the SDW transition and in turn gives rise to high-temperature superconductivity below T_c = 32 K, as observed in the electrical resistivity, AC susceptibility as well as magnetization. A well defined anomaly in the specific heat provides additional evidence for bulk superconductivity.
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