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Isotopic 32S/33S ratio as a diagnostic of presolar grains from novae

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 Added by Anuj Parikh
 Publication date 2014
  fields Physics
and research's language is English




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Measurements of sulphur isotopes in presolar grains can help to identify the astrophysical sites in which these grains were formed. A more precise thermonuclear rate of the 33S(p,gamma)34Cl reaction is required, however, to assess the diagnostic ability of sulphur isotopic ratios. We have studied the 33S(3He,d)34Cl proton-transfer reaction at 25 MeV using a high-resolution quadrupole-dipole-dipole-dipole magnetic spectrograph. Deuteron spectra were measured at ten scattering angles between 10 and 55 degrees. Twenty-four levels in 34Cl over Ex = 4.6 - 5.9 MeV were observed, including three levels for the first time. Proton spectroscopic factors were extracted for the first time for levels above the 33S+p threshold, spanning the energy range required for calculations of the thermonuclear 33S(p,gamma)34Cl rate in classical nova explosions. We have determined a new 33S(p,gamma)34Cl rate using a Monte Carlo method and have performed new hydrodynamic nova simulations to determine the impact on nova nucleosynthesis of remaining nuclear physics uncertainties in the reaction rate. We find that these uncertainties lead to a factor of less than 5 variation in the 33S(p,gamma)34Cl rate over typical nova peak temperatures, and variation in the ejected nova yields of S--Ca isotopes by less than 20%. In particular, the predicted 32S/33S ratio is 110 - 130 for the nova model considered, compared to 110 - 440 with previous rate uncertainties. As recent type II supernova models predict ratios of 130 - 200, the 32S/33S ratio may be used to distinguish between grains of nova and supernova origin.



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Recent models for evolved Low Mass Stars (with $M lesssim 3M_odot$), undergoing the AGB phase assume that magnetic flux-tube buoyancy drives the formation of $^{13}$C reservoirs in He-rich layers. We illustrate their crucial properties, showing how the low abundance of $^{13}$C generated below the convective envelope hampers the formation of primary $^{14}$N and the ensuing synthesis of intermediate-mass nuclei, like $^{19}$F and $^{22}$Ne. In the mentioned models, their production is therefore of a purely secondary nature. Shortage of primary $^{22}$Ne has also important effects in reducing the neutron density. Another property concerns AGB winds, which are likely to preserve C-rich subcomponents, isolated by magnetic tension, even when the envelope composition is O-rich. Conditions for the formation of C-rich compounds are therefore found in stages earlier than previously envisaged. These issues, together with the uncertainties related to several nuclear physics quantities, are discussed in the light of the isotopic admixtures of s-process elements in presolar SiC grains of stellar origin, which provide important and precise constraints to the otherwise uncertain parameters. By comparing nucleosynthesis results with measured SiC data, it is argued that such a detailed series of constraints indicates the need for new measurements of weak interaction rates in ionized plasmas, as well as of neutron-capture cross sections, especially near the N = 50 and N = 82 neutron magic numbers. Nontheless, the peculiarity of our models allows us to achieve fits to the presolar grain data of a quality so far never obtained in previously published attempts.
Among presolar materials recovered in meteorites, abundant SiC and Al$_{2}$O$_{3}$ grains of AGB origins were found. They showed records of C, N, O, $^{26}$Al and s-element isotopic ratios that proved invaluable in constraining the nucleosynthesis models for AGB stars cite{zin,gal}. In particular, when these ratios are measured in SiC grains, they clearly reveal their prevalent origin in cool AGB circumstellar envelopes and provide information on both the local physics and the conditions at the nucleosynthesis site (the H- and He-burning layers deep inside the structure). Among the properties ascertained for the main part of the SiC data (the so-called {it mainstream} ones), we mention a large range of $^{14}$N/$^{15}$N ratios, extending below the solar value cite{mar}, and $^{12}$C/$^{13}$C ratios $gtrsim$ 30. Other classes of grains, instead, display low carbon isotopic ratios ($gtrsim 10$) and a huge dispersion for N isotopes, with cases of large $^{15}$N excess. In the same grains, isotopes currently feeded by slow neutron captures reveal the characteristic pattern expected from this process at an efficiency slightly lower than necessary to explain the solar main s-process component. Complementary constraints can be found in oxide grains, especially Al$_{2}$O$_{3}$ crystals. Here, the oxygen isotopes and the content in $^{26}$Al are of a special importance for clarifying the partial mixing processes that are known to affect evolved low-mass stars. Successes in modeling the data, as well as problems in explaining some of the mentioned isotopic ratios through current nucleosynthesis models are briefly outlined.
We report Mo isotopic compositions of 37 presolar SiC grains of types Y (19) and Z (18), rare types commonly argued to have formed in lower-than-solar metallicity asymptotic giant branch (AGB) stars. Direct comparison of the Y and Z grain data with data for mainstream grains from AGB stars of close-to-solar metallicity demonstrates that the three types of grains have indistinguishable Mo isotopic compositions. We show that the Mo isotope data can be used to constrain the maximum stellar temperatures (TMAX) during thermal pulses in AGB stars. Comparison of FRUITY Torino AGB nucleosynthesis model calculations with the grain data for Mo isotopes points to an origin from low-mass (~1.5-3 Msun) rather than intermediate-mass (>3-~9 Msun) AGB stars. Because of the low efficiency of 22Ne({alpha},n)25Mg at the low TMAX values attained in low-mass AGB stars, model calculations cannot explain the large 30Si excesses of Z grains as arising from neutron capture, so these excesses remain a puzzle at the moment.
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Extreme excesses of $^{13}C$ ($^{12}C$/$^{13}C$<10) and $^{15}N$ ($^{14}N$/$^{15}N$<20) in rare presolar SiC grains have been considered diagnostic of an origin in classical novae, though an origin in core collapse supernovae (CCSNe) has also been proposed. We report C, N, and Si isotope data for 14 submicron- to micron-sized $^{13}C$- and $^{15}N$-enriched presolar SiC grains ($^{12}C$/$^{13}C$<16 and $^{14}N$/$^{15}N$<~100) from Murchison, and their correlated Mg-Al, S, and Ca-Ti isotope data when available. These grains are enriched in $^{13}C$ and $^{15}N$, but with quite diverse Si isotopic signatures. Four grains with $^{29,30}Si$ excesses similar to those of type C SiC grains likely came from CCSNe, which experienced explosive H burning occurred during explosions. The independent coexistence of proton- and neutron-capture isotopic signatures in these grains strongly supports heterogeneous H ingestion into the He shell in pre-supernovae. Two of the seven putative nova grains with $^{30}Si$ excesses and $^{29}Si$ depletions show lower-than-solar $^{34}S$/$^{32}S$ ratios that cannot be explained by classical nova nucleosynthetic models. We discuss these signatures within the CCSN scenario. For the remaining five putative nova grains, both nova and supernova origins are viable because explosive H burning in the two stellar sites could result in quite similar proton-capture isotopic signatures. Three of the grains are sub-type AB grains that are also $^{13}C$ enriched, but have a range of higher $^{14}N$/$^{15}N$. We found that $^{15}N$-enriched AB grains (~50<$^{14}N$/$^{15}N$<~100) have distinctive isotopic signatures compared to putative nova grains, such as higher $^{14}N$/$^{15}N$, lower $^{26}Al$/$^{27}Al$, and lack of $^{30}Si$ excess, indicating weaker proton-capture nucleosynthetic environments.
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