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Register a new userProtection of excited spin states by a superconducting energy gap
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Added by
Benjamin Heinrich Ph.D.
Publication date
2014
fields
Physics
and research's language is
English
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The latest concepts for quantum computing and data storage envision to address and manipulate single spins. A limitation for single atoms or molecules in contact to a metal surface are the short lifetime of excited spin states, typically picoseconds, due to the exchange of energy and angular momentum with the itinerant electrons of the substrate [1-4]. Here we show that paramagnetic molecules on a superconducting substrate exhibit excited spin states with a lifetime of approximately 10 ns. We ascribe this increase in lifetime by orders of magnitude to the depletion of electronic states within the energy gap at the Fermi level. This prohibits pathways of energy relaxation into the substrate and allows for electrically pumping the magnetic molecule into higher spin states, making superconducting substrates premium candidates for spin manipulation. We further show that the proximity of the scanning tunneling microscope tip modifies the magnetic anisotropy.
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We present a superconducting qubit for the circuit quantum electrodynamics architecture that has a tunable coupling strength g. We show that this coupling strength can be tuned from zero to values that are comparable with other superconducting qubits. At g = 0 the qubit is in a decoherence free subspace with respect to spontaneous emission induced by the Purcell effect. Furthermore we show that in the decoherence free subspace the state of the qubit can still be measured by either a dispersive shift on the resonance frequency of the resonator or by a cycling-type measurement.
Readout and control of fermionic spins in solid-state systems are key primitives of quantum information processing and microscopic magnetic sensing. The highly localized nature of most fermionic spins decouples them from parasitic degrees of freedom, but makes long-range interoperability difficult to achieve. In light of this challenge, an active effort is underway to integrate fermionic spins with circuit quantum electrodynamics (cQED), which was originally developed in the field of superconducting qubits to achieve single-shot, quantum-non-demolition (QND) measurements and long-range couplings. However, single-shot readout of an individual spin with cQED has remained elusive due to the difficulty of coupling a resonator to a particle trapped by a charge-confining potential. Here we demonstrate the first single-shot, cQED readout of a single spin. In our novel implementation, the spin is that of an individual superconducting quasiparticle trapped in the Andreev levels of a semiconductor nanowire Josephson element. Due to a spin-orbit interaction inside the nanowire, this superconducting spin directly determines the flow of supercurrent through the element. We harnessed this spin-dependent supercurrent to achieve both a zero-field spin splitting as well as a long-range interaction between the quasiparticle and a superconducting microwave resonator. Owing to the strength of this interaction in our device, measuring the resultant spin-dependent resonator frequency yielded QND spin readout with 92% fidelity in 1.9 $mu$s and allowed us to monitor the quasiparticles spin in real time. These results pave the way for new fermionic cQED devices: superconducting spin qubits operating at zero magnetic field, devices in which the spin has enhanced governance over the circuit, and time-domain measurements of Majorana modes.
Coupling a normal metal wire to a superconductor induces an excitation gap in the normal metal. In the absence of disorder, the induced excitation gap is strongly suppressed by finite-size effects if the thickness of the superconductor is much smaller than the thickness of the normal metal and the superconducting coherence length. We show that the presence of disorder, either in the bulk or at the exposed surface of the superconductor, significantly enhances the magnitude of the induced gap, such that it approaches the superconducting gap in the limit of strong disorder. We also discuss the shift of energy bands inside the normal-metal wire as a result of the coupling to the superconducting shell.
We consider the energetics of a superconducting double dot, comprising two superconducting islands coupled in series via a Josephson junction. The periodicity of the stability diagram is governed by the competition between the charging energy and the superconducting gap, and the stability of each charge state depends upon its parity. We also find that, at finite temperatures, thermodynamic considerations have a significant effect on the stability diagram.
We have performed microwave spectroscopy of Andreev states in superconducting weak links tailored in an InAs-Al (core-full shell) epitaxially-grown nanowire. The spectra present distinctive features, with bundles of four lines crossing when the superconducting phase difference across the weak link is 0 or $pi.$ We interpret these as arising from zero-field spin-split Andreev states. A simple analytical model, which takes into account the Rashba spin-orbit interaction in a nanowire containing several transverse subbands, explains these features and their evolution with magnetic field. Our results show that the spin degree of freedom is addressable in Josephson junctions, and constitute a first step towards its manipulation.
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