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Quantitative measurement of orbital angular momentum in electron microscopy

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 Added by Laura Clark
 Publication date 2014
  fields Physics
and research's language is English




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Electron vortex beams have been predicted to enable atomic scale magnetic information measurement, via transfer of orbital angular momentum. Research so far has focussed on developing production techniques and applications of these beams. However, methods to measure the outgoing orbital angular momentum distribution are also a crucial requirement towards this goal. Here, we use a method to obtain the orbital angular momentum decomposition of an electron beam, using a multi-pinhole interferometer. We demonstrate both its ability to accurately measure orbital angular momentum distribution, and its experimental limitations when used in a transmission electron microscope.



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The existing methods for measuring the orbital-angular-momentum (OAM) spectrum suffer from issues such as poor efficiency, strict interferometric stability requirements, and too much loss. Furthermore, most techniques inevitably discard part of the field and measure only a post-selected portion of the true spectrum. Here, we propose and demonstrate an interferometric technique for measuring the true OAM spectrum of optical fields in a single-shot manner. Our technique directly encodes the OAM-spectrum information in the azimuthal intensity profile of the output interferogram. In the absence of noise, the spectrum can be fully decoded using a single acquisition of the output interferogram, and, in the presence of noise, acquisition of two suitable interferograms is sufficient for the purpose. As an important application of our technique, we demonstrate measurements of the angular Schmidt spectrum of the entangled photons produced by parametric down-conversion and report a broad spectrum with the angular Schmidt number 82.1.
Free electrons with a helical phase front, referred to as twisted electrons, possess an orbital angular momentum (OAM) and, hence, a quantized magnetic dipole moment along their propagation direction. This intrinsic magnetic moment can be used to probe material properties. Twisted electrons thus have numerous potential applications in materials science. Measuring this quantity often relies on a series of projective measurements that subsequently change the OAM carried by the electrons. In this Letter, we propose a nondestructive way of measuring an electron beams OAM through the interaction of this associated magnetic dipole with a conductive loop. Such an interaction results in the generation of induced currents within the loop, which are found to be directly proportional to the electrons OAM value. Moreover, the electron experiences no OAM variations and only minimal energy losses upon the measurement, and, hence, the nondestructive nature of the proposed technique.
Manipulation of orbital angular momentum (OAM) of light is essential in OAM-based optical systems. Especially, OAM divider, which can convert the incoming OAM mode into one or several new smaller modes in proportion at different spatial paths, is very useful in OAM-based optical networks. However, this useful tool was never reported yet. For the first time, we put forward a passive OAM divider based on coordinate transformation. The device consists of a Cartesian to log-polar coordinate converter and an inverse converter. The first converter converts the OAM light into a rectangular-shaped plane light with a transverse phase gradient. And the second converter converts the plane light into multiple diffracted light. The OAM of zeroth-order diffracted light is the product of the input OAM and the scaling parameter. The residual light is output from other diffracted orders. Furthermore, we extend the scheme to realize equal N-dividing of OAM and arbitrary dividing of OAM. The ability of dividing OAM shows huge potential for OAM-based classical and quantum information processing.
The coherent control of electron beams and ultrafast electron wave packets dynamics have attracted significant attention in electron microscopy as well as in atomic physics. In order to unify the conceptual pictures developed in both fields, we demonstrate the generation and manipulation of tailored electron orbital angular momentum (OAM) superposition states either by employing customized holographic diffraction masks in a transmission electron microscope or by atomic multiphoton ionization utilizing pulse-shaper generated carrier-envelope phase stable bichromatic ultrashort laser pulses. Both techniques follow similar physical mechanisms based on Fourier synthesis of quantum mechanical superposition states allowing the preparation of a broad set of electron states with uncommon symmetries. We describe both approaches in a unified picture based on an advanced spatial and spectral double slit and point out important analogies. In addition, we analyze the topological charge and discuss the control mechanisms of the free-electron OAM superposition states. Their generation and manipulation by phase tailoring in transmission electron microscopy and atomic multiphoton ionization is illustrated on a 7-fold rotationally symmetric electron density distribution.
114 - Jing Zhu , Pei Zhang , Qichang Li 2018
As a special experimental technique, weak measurement extracts very little information about the measured system and will not cause the measured state collapse. When coupling the orbital angular momentum (OAM) state with a well-defined pre-selected and post-selected system of a weak measurement process, there is an indirect coupling between position and topological charge (TC) of OAM state. Based on these ideas, we propose an experimental scheme that experimentally measure the TC of OAM beams from -14 to 14 through weak measurement.
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