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Quantifying and controlling the magnetic dipole contribution to 1.5 $mu$m light emission in erbium-doped yttrium oxide

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 Added by Rashid Zia
 Publication date 2014
  fields Physics
and research's language is English




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We experimentally quantify the contribution of magnetic dipole (MD) transitions to the near-infrared light emission from trivalent erbium-doped yttrium oxide (Er$^{3+}$:Y$_2$O$_3$). Using energy-momentum spectroscopy, we demonstrate that the $^4$I$_{13/2}{to}^4$I$_{15/2}$ emission near 1.5 $mu$m originates from nearly equal contributions of electric dipole (ED) and MD transitions that exhibit distinct emission spectra. We then show how these distinct spectra, together with the differing local density of optical states (LDOS) for ED and MD transitions, can be leveraged to control Er$^{3+}$ emission in structured environments. We demonstrate that far-field emission spectra can be tuned to resemble almost pure emission from either ED or MD transitions, and show that the observed spectral modifications can be accurately predicted from the measured ED and MD intrinsic emission rates.



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Silicon-based light sources including light-emitting diodes (LEDs) and laser diodes (LDs) for information transmission are urgently needed for developing monolithic integrated silicon photonics. Silicon doped by ion implantation with erbium ions (Er$^{3+}$) is considered a promising approach, but suffers from an extremely low quantum efficiency. Here we report an electrically pumped superlinear emission at 1.54 $mu$m from Er/O-doped silicon planar LEDs, which are produced by applying a new deep cooling process. Stimulated emission at room temperature is realized with a low threshold current of ~6 mA (~0.8 A/cm2). Time-resolved photoluminescence and photocurrent results disclose the complex carrier transfer dynamics from the silicon to Er3+ by relaxing electrons from the indirect conduction band of the silicon. This picture differs from the frequently-assumed energy transfer by electron-hole pair recombination of the silicon host. Moreover, the amplified emission from the LEDs is likely due to a quasi-continuous Er/O-related donor band created by the deep cooling technique. This work paves a way for fabricating superluminescent diodes or efficient LDs at communication wavelengths based on rare-earth doped silicon.
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