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Tunneling in a quantum coherent structure is not restricted to only nearest neighbours. Hopping between distant sites is possible via the virtual occupation of otherwise avoided intermediate states. Here we report the observation of long range transitions in the transport through three quantum dots coupled in series. A single electron is delocalized between the left and right quantum dots while the centre one remains always empty. Superpositions are formed and both charge and spin are exchanged between the outermost dots. Detection of the process is achieved via the observation of narrow resonances, insensitive to the transport Pauli spin blockade.
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We study entanglement of Kondo clouds in an open triple quantum dots (OTQDs) system based on the dissipaton equation of motion (DEOM) theory. A comprehensive picture of the long-range entanglement of Kondo clouds is sketched by the spectral functions, spin-spin correlation and dot occupancies of OTQDs. We find that for the configuration (N1,N2,N3) = (1, 0, 1), a conduction electrons peak occurs in the spectral function of intermediate QD in Kondo regime. This peak resulting from the overlapping of the two Kondo clouds forming from between the two peripheral QDs and leads, enhances with decreasing temperature and increasing dot-lead coupling. Both the spin-spin correlations between the two adjacent QDs and the two peripheral QDs owns negative values. It also confirms the physical picuture of the overlapping between left and right Kondo clouds via the intermediate QD. Moreover, the transition of the effective electron occupation and the spectral function of intermediate QD in Kondo regime also indicates the entanglement of Kondo clouds enhancing with decreasing temperature and increasing dot-lead coupling. This investigation will be beneficial to detect the Kondo clouds and to further explore Kondo physics in related experiment setups.
Numerical analysis of the simplest odd-numbered system of coupled quantum dots reveals an interplay between magnetic ordering, charge fluctuations and the tendency of itinerant electrons in the leads to screen magnetic moments. The transition from local-moment to molecular-orbital behavior is visible in the evolution of correlation functions as the inter-dot coupling is increased. Resulting novel Kondo phases are presented in a phase diagram which can be sampled by measuring the zero-bias conductance. We discuss the origin of the even-odd effects by comparing with the double quantum dot.
Environmental noise usually hinders the efficiency of charge transport through coherent quantum systems; an exception is dephasing-assisted transport (DAT). We show that linear triple quantum dots in a transport configuration and subjected to pure dephasing exhibit DAT if the coupling to the drain reservoir exceeds a threshold. DAT occurs for arbitrarily weak dephasing and the enhancement can be directly controlled by the coupling to the drain. Moreover, for specific settings, the enhanced current is accompanied by a reduction in relative shot noise. We identify the quantum Zeno effect and long-distance tunnelling as underlying dynamical processes involved in dephasing-assisted and -suppressed transport. Our analytical results are obtained by using the density matrix formalism and the characteristic polynomial approach to full counting statistics.
Using large-scale, real-time quantum dynamics calculations, we present a detailed analysis of electronic excitation transfer (EET) mechanisms in a multi-particle plasmonic nanoantenna system. Specifically, we utilize real-time, time-dependent, density functional tight binding (RT-TDDFTB) to provide a quantum-mechanical description (at an electronic/atomistic level of detail) for characterizing and analyzing these systems, without recourse to classical approximations. We also demonstrate highly long-range electronic couplings in these complex systems and find that the range of these couplings is more than twice the conventional cutoff limit considered by FRET based approaches. Furthermore, we attribute these unusually long-ranged electronic couplings to the coherent oscillations of conduction electrons in plasmonic nanoparticles. This long-range nature of plasmonic interactions has important ramifications for EET - in particular, we show that the commonly used nearest-neighbor FRET model is inadequate for accurately characterizing EET even in simple plasmonic antenna systems. These findings provide a real-time, quantum-mechanical perspective for understanding EET mechanisms and provide guidance in enhancing plasmonic properties in artificial light-harvesting systems.
Rapid and efficient preparation, manipulation and transfer of quantum states through an array of quantum dots (QDs) is a demanding requisite task for quantum information processing and quantum computation in solid-state physics. Conventional adiabatic protocols, as coherent transfer by adiabatic passage (CTAP) and its variations, provide slow transfer prone to decoherence, which could lower the fidelity to some extent. To achieve the robustness against decoherence, we propose a protocol of speeding up the adiabatic charge transfer in multi-QD systems, sharing the concept of Shortcuts to Adiabaticity (STA). We first apply the STA techniques, including the counterdiabatic driving and inverse engineering, to speed up the direct (long range) transfer between edge dots in triple QDs. Then, we extend our analysis to a multi-dot system. We show how by implementing the modified pulses, fast adiabatic-like charge transport between the outer dots can be eventually achieved without populating intermediate dots. We discuss as well the dependence of the transfer fidelity on the operation time in the presence of dephasing. The proposed protocols for accelerating adiabatic charge transfer directly between the outer dots in a QD array offers a robust mechanism for quantum information processing, by minimizing decoherence and relaxation processes.
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