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Register a new userArtificially engineered superlattices of pnictide superconductor
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Significant progress has been achieved in fabricating high quality bulk and thinfilm iron-based superconductors. In particular, artificial layered pnictide superlattices offer the possibility of tailoring the superconducting properties and understanding the mechanism of the superconductivity itself. For high field applications, large critical current densities (Jc) and irreversibility fields (Hirr) are indispensable along all crystal directions. On the other hand, the development of superconducting devices such as tunnel junctions requires multilayered heterostructures. Here we show that artificially engineered undoped Ba-122 / Co doped Ba-122 compositionally modulated superlattices produce ab-aligned nanoparticle arrays. These layer and self-assemble along c-axis aligned defects, and combine to produce very large Jc and Hirr enhancements over a wide angular range. We also demonstrate a structurally modulated SrTiO3 (STO) / Co doped Ba-122 superlattice with sharp interfaces. Success in superlattice fabrication involving pnictides will aid the progress of heterostructured systems exhibiting novel interfacial phenomena and device applications.
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In the quest for exotic superconducting pairing states, the Rashba effect, which lifts the electron-spin degeneracy as a consequence of strong spin-orbit interaction (SOI) under broken inversion symmetry, has attracted considerable interest. Here, to introduce the Rashba effect into two-dimensional (2D) strongly correlated electron systems, we fabricate non-centrosymmetric (tricolor) superlattices composed of three kinds of $f$-electron compounds with atomic thickness; $d$-wave heavy fermion superconductor CeCoIn$_5$ sandwiched by two different nonmagnetic metals, YbCoIn$_5$ and YbRhIn$_5$. We find that the Rashba SOI induced global inversion symmetry breaking in these tricolor Kondo superlattices leads to profound changes in the superconducting properties of CeCoIn$_5$, which are revealed by unusual temperature and angular dependences of upper critical fields that are in marked contrast with the bulk CeCoIn$_5$ single crystals. We demonstrate that the Rashba effect incorporated into 2D CeCoIn$_5$ block layers is largely tunable by changing the layer thickness. Moreover, the temperature dependence of in-plane upper critical field exhibits an anomalous upturn at low temperatures, which is attributed to a possible emergence of a helical or stripe superconducting phase. Our results demonstrate that the tricolor Kondo superlattices provide a new playground for exploring exotic superconducting states in the strongly correlated 2D electron systems with the Rashba effect.
Although nanoscale deformation, such as nanostrain in iron chalcogenide (FeSexTe1-x, FST) thin films, has attracted attention owing to the enhancement of general superconducting properties, including critical current density (Jc) and critical transition temperature, its formation has proven to be an extremely challenging and complex process thus far. Herein, we successfully fabricated an epitaxial FST thin film with uniformly distributed nanostrain by injection of a trace amount of CeO2 inside FST matrix using sequential pulsed laser deposition. Using transmission electron microscopy and geometrical phase analysis, we verified that a trace amount of CeO2 injection forms nanoscale fine defects with a nanostrained region, which has a tensile strain (ezz ~ 0.02) along the c-axis of the FST matrix. The nanostrained FST thin film achieves a remarkable Jc of 3.5 MA/cm2 for a self-field at 6 K and a highly enhanced Jc under the entire magnetic field with respect to a pristine FST thin film.
We report the observation of low-frequency modes in the Raman spectra of thin-film superlattices of the high-temperature superconductor YBa$ _{2} $Cu$ _{3} $O$ _{7-delta} $ and various manganite perovskites. Our study shows that these modes are caused by the backfolding of acoustic phonons due to the additional periodicity introduced by the superlattice. Such modes were previously only observed for ultra-pure semiconductor superlattices. They can be used to determine the bilayer thickness of the superlattice and its speed of sound. Moreover, we use the spatial resolution of Raman microscopy to map the film thickness inhomogeneity across a sample, making these modes a useful tool to characterize thin-film superlattices.
We report specific heat under different magnetic fields for recently discovered quasi-one dimensional Nb2PdS5 superconductor. The studied compound is superconducting below 6 K. Nb2PdS5 is quite robust against magnetic field with dHc/dT of -42 kOe/K. The estimated upper critical field [Hc2(0)] is 190 kOe, clearly surpassing the Pauli-paramagnetic limit of 1.84Tc. Low temperature heat capacity in superconducting state of Nb2PdS5 under different magnetic fields showed s-wave superconductivity with two different gaps. Two quasi-linear slopes in Somerfield-coefficient as a function of applied magnetic field and two band behavior of the electronic heat capacity demonstrate that Nb2PdS5 is a multiband su-perconductor in weak coupling limit with deltagamma/deltaTc=0.9.
Here we report the discovery of the first ternary molybdenum pnictide based superconductor K2Mo3As3. Polycrystalline samples were synthesized by the conventional solid state reaction method. X-ray diffraction analysis reveals a quasi-one-dimensional hexagonal crystal structure with (Mo3As3)2- linear chains separated by K+ ions, similar as previously reported K2Cr3As3, with the space group of P-6m2 (No. 187) and the refined lattice parameters a = 10.145(5) {AA} and c = 4.453(8) {AA}. Electrical resistivity, magnetic susceptibility, and heat capacity measurements exhibit bulk superconductivity with the onset Tc at 10.4 K in K2Mo3As3 which is higher than the isostructural Cr-based superconductors. Being the same group VIB transition elements and with similar structural motifs, these Cr and Mo based superconductors may share some common underlying origins for the occurrence of superconductivity and need more investigations to uncover the electron pairing within a quasi-one-dimensional chain structure.
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