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Register a new userDriven Electronic States at the Surface of a Topological Insulator
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Added by
Benjamin M. Fregoso
Publication date
2013
fields
Physics
and research's language is
English
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Motivated by recent photoemission experiments on the surface of topological insulators we compute the spectrum of driven topological surface excitations in the presence of an external light source. We completely characterize the spectral function of these non-equilibrium electron excitations for both linear and circular polarizations of the incident light. We find that in the latter case, the circularly polarized light gaps out the surface states, whereas linear polarization gives rise to an anisotropic metal with multiple Dirac cones. We compare the sizes of the gaps with recent pump-probe photoemission measurements and find good agreement. We also identify theoretically several new features in the time-dependent spectral function, such as shadow Dirac cones.
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The surfaces of three dimensional topological insulators (3D TIs) are generally described as Dirac metals, with a single Dirac cone. It was previously believed that a gapped surface implied breaking of either time reversal $mathcal T$ or U(1) charge conservation symmetry. Here we discuss a novel possibility in the presence of interactions, a surface phase that preserves all symmetries but is nevertheless gapped and insulating. Then the surface must develop topological order of a kind that cannot be realized in a 2D system with the same symmetries. We discuss candidate surface states - non-Abelian Quantum Hall states which, when realized in 2D, have $sigma_{xy}=1/2$ and hence break $mathcal T$ symmetry. However, by constructing an exactly soluble 3D lattice model, we show they can be realized as $mathcal T$ symmetric surface states. The corresponding 3D phases are confined, and have $theta=pi$ magnetoelectric response. Two candidate states have the same 12 particle topological order, the (Read-Moore) Pfaffian state with the neutral sector reversed, which we term T-Pfaffian topological order, but differ in their $mathcal T$ transformation. Although we are unable to connect either of these states directly to the superconducting TI surface, we argue that one of them describes the 3D TI surface, while the other differs from it by a bosonic topological phase. We also discuss the 24 particle Pfaffian-antisemion topological order (which can be connected to the superconducting TI surface) and demonstrate that it can be realized as a $mathcal T$ symmetric surface state.
The Kondo insulator SmB6 has long been known to exhibit low temperature transport anomalies whose origin is of great interest. Here we uniquely access the surface electronic structure of the anomalous transport regime by combining state-of-the-art laser- and synchrotron-based angle-resolved photoemission techniques. We observe clear in-gap states (up to 4 meV), whose temperature dependence is contingent upon the Kondo gap formation. In addition, our observed in-gap Fermi surface oddness tied with the Kramers points topology, their coexistence with the two-dimensional transport anomaly in the Kondo hybridization regime, as well as their robustness against thermal recycling, taken together, collectively provide by-far the strongest evidence for protected surface metallicity with a Fermi surface whose topology is consistent with the theoretically predicted topological surface Fermi surface (TSS). Our observations of systematic surface electronic structure provide the fundamental electronic parameters for the anomalous Kondo ground state of the correlated electron material SmB6.
The electronic structure of Bi2Se3 is studied by angle-resolved photoemission and density functional theory. We show that the instability of the surface electronic properties, observed even in ultra-high-vacuum conditions, can be overcome via in-situ potassium deposition. In addition to accurately setting the carrier concentration, new Rashba-like spin-polarized states are induced, with a tunable, reversible, and highly stable spin splitting. Ab-initio slab calculations reveal that these Rashba state are derived from the 5QL quantum-well states. While the K-induced potential gradient enhances the spin splitting, this might be already present for pristine surfaces due to the symmetry breaking of the vacuum-solid interface.
The Kondo insulator SmB6 has long been known to exhibit low temperature (T < 10K) transport anomaly and has recently attracted attention as a new topological insulator candidate. By combining low-temperature and high energy-momentum resolution of the laser-based ARPES technique, for the first time, we probe the surface electronic structure of the anomalous conductivity regime. We observe that the bulk bands exhibit a Kondo gap of 14 meV and identify in-gap low-lying states within a 4 meV window of the Fermi level on the (001)-surface of this material. The low-lying states are found to form electron-like Fermi surface pockets that enclose the X and the Gamma points of the surface Brillouin zone. These states disappear as temperature is raised above 15K in correspondence with the complete disappearance of the 2D conductivity channels in SmB6. While the topological nature of the in-gap metallic states cannot be ascertained without spin (spin-texture) measurements our bulk and surface measurements carried out in the transport-anomaly-temperature regime (T < 10K) are consistent with the first-principle predicted Fermi surface behavior of a topological Kondo insulator phase in this material.
The resistance of a conventional insulator diverges as temperature approaches zero. The peculiar low temperature resistivity saturation in the 4f Kondo insulator (KI) SmB6 has spurred proposals of a correlation-driven topological Kondo insulator (TKI) with exotic ground states. However, the scarcity of model TKI material families leaves difficulties in disentangling key ingredients from irrelevant details. Here we use angle-resolved photoemission spectroscopy (ARPES) to study FeSb2, a correlated d-electron KI candidate that also exhibits a low temperature resistivity saturation. On the (010) surface, we find a rich assemblage of metallic states with two-dimensional dispersion. Measurements of the bulk band structure reveal band renormalization, a large temperature-dependent band shift, and flat spectral features along certain high symmetry directions, providing spectroscopic evidence for strong correlations. Our observations suggest that exotic insulating states resembling those in SmB6 and YbB12 may also exist in systems with d instead of f electrons.
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