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Register a new userParasitic nonlinearities in photon pair generation via integrated spontaneous four-wave mixing: critical problem or distraction?
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We consider integrated photon pair sources based on spontaneous four-wave mixing and derive expressions for the pump powers at which various nonlinear processes become relevant for a variety of source materials and structures. These expressions serve as rules of thumb in identifying reasonable parameter regimes for the design of such sources. We demonstrate that if pump powers are kept low enough to suppress cross-phase modulation, multi-pair events as well as many other nonlinear effects are often also constrained to negligible levels.
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We develop a general Hamiltonian treatement of spontaneous four-wave mixing in a microring resonator side-coupled to a channel waveguide. The effect of scattering losses in the ring is included, as well as parasitic nonlinear effects including self- and cross-phase modulation. A procedure for computing the output of such a system for arbitrary parameters and pump states is presented. For the limit of weak pumping an expression for the joint spectral intensity of generated photon pairs, as well as the singles-to-coincidences ratio, is derived.
We calculate that an appropriate modification of the field associated with only one of the photons of a photon pair can suppress generation of the pair entirely. From this general result, we develop a method for suppressing the generation of undesired photon pairs utilizing photonic stop bands. For a third-order nonlinear optical source of frequency-degenerate photons we calculate the modified frequency spectrum (joint spectral intensity) and show a significant increase in a standard metric, the coincidence to accidental ratio. These results open a new avenue for photon-pair frequency correlation engineering.
Optical nanoantennas have shown a great capacity for efficient extraction of photons from the near to the far-field, enabling directional emission from nanoscale single-photon sources. However, their potential for the generation and extraction of multi-photon quantum states remains unexplored. Here we demonstrate experimentally the nanoscale generation of two-photon quantum states at telecommunication wavelengths based on spontaneous parametric down-conversion in an optical nanoantenna. The antenna is a crystalline AlGaAs nanocylinder, possessing Mie-type resonances at both the pump and the bi-photon wavelengths and when excited by a pump beam generates photonpairs with a rate of 35 Hz. Normalized to the pump energy stored by the nanoantenna, this rate corresponds to 1.4 GHz/Wm, being one order of magnitude higher than conventional on-chip or bulk photon-pair sources. Our experiments open the way for multiplexing several antennas for coherent generation of multi-photon quantum states with complex spatial-mode entanglement and applications in free-space quantum communications and sensing.
We consider the effect of self-phase modulation and cross-phase modulation on the joint spectral amplitude of photon pairs generated by spontaneous four-wave mixing. In particular, the purity of a heralded photon from a pair is considered, in the context of schemes that aim to maximise the purity and minimise correlation in the joint spectral amplitude using birefringent phase-matching and short pump pulses. We find that non-linear phase modulation effects will be detrimental, and will limit the quantum interference visibility that can be achieved at a given generation rate. An approximate expression for the joint spectral amplitude with phase modulation is found by considering the group velocity walk-off between each photon and the pump, but neglecting the group-velocity dispersion at each wavelength. The group-velocity dispersion can also be included with a numerical calculation, and it is shown that it only has a small effect on the purity for the realistic parameters considered.
Using four-wave mixing in a hot atomic vapor, we generate a pair of entangled twin beams in the microsecond pulsed regime near the D1 line of $^{85}$Rb, making it compatible with commonly used quantum memory techniques. The beams are generated in the bright and vacuum-squeezed regimes, requiring two separate methods of analysis, without and with local oscillators, respectively. We report a noise reduction of up to $3.8pm 0.2$ dB below the standard quantum limit in the pulsed regime and a level of entanglement that violates an Einstein--Podolsky--Rosen inequality.
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