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Register a new userPolymer plats and multicomponent anyon gases
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Anyon systems are studied in connection with several interesting applications including high $T_C$ superconductivity and topological quantum computing. In this work we show that these systems can be realized starting from directed polymers braided together to form a nontrivial link configuration belonging to the topological class of plats. The statistical sum of a such plat is related here to the partition function of a two-component anyon gas. The constraints that preserve the topological configuration of the plat are imposed on the polymer trajectories using the so-called Gauss linking number, a topological invariant that has already been well studied in polymer physics. Due to these constraints, short-range forces act on the monomers or, equivalently, on the anyon quasiparticles in a way that closely resembles the appearance of reaction forces in the constrained systems of classical mechanics. If the polymers are homogeneous, the anyon system reaches a self-dual point, in which these forces vanish exactly. A class of self-dual solutions that minimize the energy of the anyons is derived. The two anyon gas discussed here obeys an abelian statistics, while for quantum computing it is known that nonabelian anyons are necessary. However, this is a limitation due to the use of the Gauss linking invariant to impose the topological constraints, which is a poor topological invariant and is thus unable to capture the nonabelian characteristics of the braided polymer chains. A more refined treatment of the topological constraints would require more sophisticated topological invariants, but so far their application to the statistical mechanics of linked polymers is an open problem.
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Multicomponent systems are ubiquitous in nature and industry. While the physics of few-component liquid mixtures (i.e., binary and ternary ones) is well-understood and routinely taught in undergraduate courses, the thermodynamic and kinetic properties of $N$-component mixtures with $N>3$ have remained relatively unexplored. An example of such a mixture is provided by the intracellular fluid, in which protein-rich droplets phase separate into distinct membraneless organelles. In this work, we investigate equilibrium phase behavior and morphology of $N$-component liquid mixtures within the Flory-Huggins theory of regular solutions. In order to determine the number of coexisting phases and their compositions, we developed a new algorithm for constructing complete phase diagrams, based on numerical convexification of the discretized free energy landscape. Together with a Cahn-Hilliard approach for kinetics, we employ this method to study mixtures with $N=4$ and $5$ components. We report on both the coarsening behavior of such systems, as well as the resulting morphologies in three spatial dimensions. We discuss how the number of coexisting phases and their compositions can be extracted with Principal Component Analysis (PCA) and K-Means clustering algorithms. Finally, we discuss how one can reverse engineer the interaction parameters and volume fractions of components in order to achieve a range of desired packing structures, such as nested `Russian dolls and encapsulated Janus droplets.
We investigate by means of molecular dynamics simulation a coarse-grained polymer glass model focusing on (quasi-static and dynamical) shear-stress fluctuations as a function of temperature T and sampling time $Delta t$. The linear response is characterized using (ensemble-averaged) expectation values of the contributions (time-averaged for each shear plane) to the stress-fluctuation relation $mu_{sf}$ for the shear modulus and the shear-stress relaxation modulus $G(t)$. Using 100 independent configurations we pay attention to the respective standard deviations. While the ensemble-averaged modulus $mu_{sf}(T)$ decreases continuously with increasing T for all $Delta t$ sampled, its standard deviation $delta mu_{sf}(T)$ is non-monotonous with a striking peak at the glass transition. The question of whether the shear modulus is continuous or has a jump-singularity at the glass transition is thus ill-posed. Confirming the effective time-translational invariance of our systems, the $Delta t$-dependence of $mu_{sf}$ and related quantities can be understood using a weighted integral over $G(t)$. This implies that the shear viscosity $eta(T)$ may be readily obtained from the $1/Delta t$-decay of $mu_{sf}$ above the glass transition.
The expansion of the velocity distribution function for the homogeneous cooling state (HCS) in a Sonine polynomial series around a Maxwellian is shown to be divergent, though Borel resummable. A convergent expansion for the HCS has been devised and employed to obtain the HCS velocity distribution function and (using it) the linear transport coefficients for a three dimensional monodisperse granular gas of smooth inelastic spheres, for all physical values of the coefficient of normal restitution. The results are in very good agreement with findings of DSMC simulations.
Sampling equilibrium ensembles of dense polymer mixtures is a paradigmatically hard problem in computational physics, even in lattice-based models. Here, we develop a formalism based on interacting binary tensors that allows for tackling this problem using quantum annealing machines. Our approach is general in that properties such as self-avoidance, branching, and looping can all be specified in terms of quadratic interactions of the tensors. Microstates realizations of different lattice polymer ensembles are then seamlessly generated by solving suitable discrete energy-minimization problems. This approach enables us to capitalize on the strengths of quantum annealing machines, as we demonstrate by sampling polymer mixtures from low to high densities, using the D-Wave quantum computer. Our systematic approach offers a promising avenue to harness the rapid development of quantum computers for sampling discrete models of filamentous soft-matter systems.
We extensively investigated the critical behavior of mixtures of colloids and polymers via the two-component Asakura-Oosawa model and its reduction to a one-component colloidal fluid using accurate theoretical and simulation techniques. In particular the theoretical approach, hierarchical reference theory [Adv. Phys. 44, 211 (1995)], incorporates realistically the effects of long-range fluctuations on phase separation giving exponents which differ strongly from their mean-field values, and are in good agreement with those of the three-dimensional Ising model. Computer simulations combined with finite-size scaling analysis confirm the Ising universality and the accuracy of the theory, although some discrepancy in the location of the critical point between one-component and full-mixture description remains. To assess the limit of the pair-interaction description, we compare one-component and two-component results.
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