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Register a new userDynamics of the non-classical light from a single solid-state quantum emitter
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We measure the dynamics of a non-classical optical field using two-time second-order correlations in conjunction with pulsed excitation. The technique quantifies single-photon purity and coherence during the excitation-decay cycle of an emitter, illustrated here using a quantum dot. We observe that for certain pump wavelengths, photons detected early in the cycle have reduced single-photon purity and coherence compared to those detected later. A model indicates that the single-photon purity dynamics are due to exciton recapture after initial emission and within the same pulse cycle.
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By pulsed s-shell resonant excitation of a single quantum dot-micropillar system, we generate long streams of a thousand of near transform-limited single photons with high mutual indistinguishability. Hong-Ou-Mandel interference of two photons are measured as a function of their emission time separation varying from 13 ns to 14.7 {mu}s, where the visibility slightly drops from 95.9(2)% to a plateau of 92.1(5)% through a slow dephasing process occurring at time scale of 0.7 {mu}s. Temporal and spectral analysis reveal the pulsed resonance fluorescence single photons are close to transform limit, which are readily useful for multi-photon entanglement and interferometry experiments.
We report the first experimental demonstration of interference-induced spectral line elimination predicted by Zhu and Scully [Phys. Rev. Lett. 76, 388 (1996)] and Ficek and Rudolph [Phys. Rev. A 60, 4245 (1999)]. We drive an exciton transition of a self-assembled quantum dot in order to realize a two-level system exposed to bichromatic laser field and observe nearly complete elimination of the resonance fluorescence spectral line at the driving laser frequency. This is caused by quantum interference between coupled transitions among the doubly dressed excitonic states, without population trapping. We also demonstrate multiphoton ac Stark effect with shifted subharmonic resonances and dynamical modifications of resonance fluorescence spectra by using double dressing.
Quantum frequency conversion (QFC), a nonlinear optical process in which the frequency of a quantum light field is altered while conserving its non-classical correlations, was first demonstrated 20 years ago. Meanwhile, it is considered an essential tool for the implementation of quantum repeaters since it allows for interfacing quantum memories with telecom-wavelength photons as quantum information carriers. Here we demonstrate efficient (>30%) QFC of visible single photons (711 nm) emitted by a quantum dot (QD) to a telecom wavelength (1,313 nm). Analysis of the first and second-order coherence before and after wavelength conversion clearly proves that important properties, such as the coherence time and photon antibunching, are fully conserved during the frequency translation process. Our findings underline the great potential of single photon sources on demand in combination with QFC as a promising technique for quantum repeater schemes.
Quantum networks using photonic channels require control of the interactions between the photons, carrying the information, and the elements comprising the nodes. In this work we theoretically analyse the spectral properties of an optical photon emitted by a solid-state quantum memory, which acts as a converter of a photon absorbed in another frequency range. We determine explicitly the expression connecting the stored and retrieved excitation taking into account possible mode and phase mismatching of the experimental setup. The expression we obtain describes the output field as a function of the input field for a transducer working over a wide range of frequencies, from optical-to-optical to microwave-to-optical. We apply this result to analyse the photon spectrum and the retrieval probability as a function of the optical depth for microwave-to-optical transduction. In the absence of losses, the efficiency of the solid-state quantum transducer is intrinsically determined by the capability of designing the retrieval process as the time-reversal of the storage dynamics.
We investigate the reduction of the electromagnetic field fluctuations in resonance fluorescence from a single emitter coupled to an optical nanostructure. We find that such hybrid system can lead to the creation of squeezed states of light, with quantum fluctuations significantly below the shot noise level. Moreover, the physical conditions for achieving squeezing are strongly relaxed with respect to an emitter in free space. A high degree of control over squeezed light is feasible both in the far and near fields, opening the pathway to its manipulation and applications on the nanoscale with state-of-the-art setups.
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