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Feshbach spectroscopy of an ultracold mixture of $^{85}$Rb and $^{133}$Cs

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 Added by Daniel McCarron
 Publication date 2012
  fields Physics
and research's language is English




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We report the observation of interspecies Feshbach resonances in an optically trapped mixture of $^{85}$Rb and $^{133}$Cs. We measure 14 interspecies features in the lowest spin channels for a magnetic field range from 0 to 700 G and show that they are in good agreement with coupled-channel calculations. The interspecies background scattering length is close to zero over a large range of magnetic fields, permitting the sensitive detection of Feshbach resonances through interspecies thermalisation. Our results confirm the quality of the Rb-Cs potential curves and offer promising starting points for the production of ultracold polar molecules.



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We report on the observation of interspecies Feshbach resonances in an ultracold, optically trapped mixture of Rb and Cs atoms. In a magnetic field range up to 300 G we find 23 interspecies Feshbach resonances in the lowest spin channel and 2 resonances in a higher channel of the mixture. The extraordinarily rich Feshbach spectrum suggests the importance of different partial waves in both the open and closed channels of the scattering problem along with higher-order coupling mechanisms. Our results provide, on one hand, fundamental experimental input to characterize the Rb-Cs scattering properties and, on the other hand, identify possible starting points for the association of ultracold heteronuclear RbCs molecules.
We report the production of a high phase-space density mixture of $^{87}$Rb and $^{133}$Cs atoms in a levitated crossed optical dipole trap as the first step towards the creation of ultracold RbCs molecules via magneto-association. We present a simple and robust experimental setup designed for the sympathetic cooling of $^{133}$Cs via interspecies elastic collisions with $^{87}$Rb. Working with the $|F=1, m_F=+1 >$ and the $|3, +3 >$ states of $^{87}$Rb and $^{133}$Cs respectively, we measure a high interspecies three-body inelastic collision rate $sim 10^{-25}-10^{-26} rm{cm}^{6}rm{s}^{-1}$ which hinders the sympathetic cooling. Nevertheless by careful tailoring of the evaporation we can produce phase-space densities near quantum degeneracy for both species simultaneously. In addition we report the observation of an interspecies Feshbach resonance at 181.7(5) G and demonstrate the creation of Cs$_{2}$ molecules via magneto-association on the 4g(4) resonance at 19.8 G. These results represent important steps towards the creation of ultracold RbCs molecules in our apparatus.
We measure higher partial wave Feshbach resonances in an ultracold mixture of fermionic $^6$Li and bosonic $^{133}$Cs by magnetic field dependent atom-loss spectroscopy. For the $p$-wave Feshbach resonances we observe triplet structures corresponding to different projections of the pair rotation angular momentum onto the external magnetic field axis. We attribute the splittings to the spin-spin and spin-rotation couplings by modelling the observation using a full coupled-channel calculation. Comparison with an oversimplified model, estimating the spin-rotation coupling by describing the weakly bound close-channel molecular state with the perturbative multipole expansion, reveals the significant contribution of the molecular wavefunction at short internuclear distances. Our findings highlight the potential of Feshbach resonances in providing precise information on short- and intermediate-range molecular couplings and wavefunctions. The observed $d$-wave Feshbach resonances allow us to refine the LiCs singlet and triplet ground-state molecular potential curves at large internuclear separations.
We observe interspecies Feshbach resonances due to s-wave bound states in ultracold $^{39}$K-$^{133}$Cs scattering for three different spin mixtures. The resonances are observed as joint atom loss and heating of the K sample. We perform least-squares fits to obtain improved K-Cs interaction potentials that reproduce the observed resonances, and carry out coupled-channel calculations to characterize the scattering and bound-state properties for $^{39}$K-Cs, $^{40}$K-Cs and $^{41}$K-Cs. Our results open up the possibilities of tuning interactions in K-Cs atomic mixtures and of producing ultracold KCs molecules.
We report the binding energy of $^{87}$Rb$^{133}$Cs molecules in their rovibrational ground state measured using an offset-free optical frequency comb based on difference frequency generation technology. We create molecules in the absolute ground state using stimulated Raman adiabatic passage (STIRAP) with a transfer efficiency of 88%. By measuring the absolute frequencies of our STIRAP lasers, we find the energy-level difference from an initial weakly-bound Feshbach state to the rovibrational ground state with a resolution of 5 kHz over an energy-level difference of more than 114 THz; this lets us discern the hyperfine splitting of the ground state. Combined with theoretical models of the Feshbach state binding energies and ground-state hyperfine structure, we determine a zero-field binding energy of $htimes114,268,135,237(5)(50)$ kHz. To our knowledge, this is the most accurate determination to date of the dissociation energy of a molecule.
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