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Register a new userEnvironmental Effects on TPB Wavelength-Shifting Coatings
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The scintillation detection systems of liquid argon time projection chambers (LArTPCs) require wavelength shifters to detect the 128 nm scintillation light produced in liquid argon. Tetraphenyl butadiene (TPB) is a fluorescent material that can shift this light to a wavelength of 425 nm, lending itself well to use in these detectors. We can coat the glass of photomultiplier tubes (PMTs) with TPB or place TPB-coated plates in front of the PMTs. In this paper, we investigate the degradation of a chemical TPB coating in a laboratory or factory environment to assess the viability of long-term TPB film storage prior to its initial installation in an LArTPC. We present evidence for severe degradation due to common fluorescent lights and ambient sunlight in laboratories, with potential losses at the 40% level in the first day and eventual losses at the 80% level after a month of exposure. We determine the degradation is due to wavelengths in the UV spectrum, and we demonstrate mitigating methods for retrofitting lab and factory environments.
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We present a model for the Global Quantum Efficiency (GQE) of the MicroBooNE optical units. An optical unit consists of a flat, circular acrylic plate, coated with tetraphenyl butadiene (TPB), positioned near the photocathode of a 20.2-cm diameter photomultiplier tube. The plate converts the ultra-violet scintillation photons from liquid argon into visible-spectrum photons to which the cryogenic phototubes are sensitive. The GQE is the convolution of the efficiency of the plates that convert the 128 nm scintillation light from liquid argon to visible light, the efficiency of the shifted light to reach the photocathode, and the efficiency of the cryogenic photomultiplier tube. We develop a GEANT4-based model of the optical unit, based on first principles, and obtain the range of probable values for the expected number of detected photoelectrons ($N_{rm PE}$) given the known systematic errors on the simulation parameters. We compare results from four measurements of the $N_{rm PE}$ determined using alpha-particle sources placed at two distances from a TPB-coated plate in a liquid argon cryostat test stand. We also directly measured the radial dependence of the quantum efficiency, and find that this has the same shape as predicted by our model. Our model results in a GQE of $0.0055pm0.0009$ for the MicroBooNE optical units. While the information shown here is MicroBooNE specific, the approach to the model and the collection of simulation parameters will be widely applicable to many liquid-argon-based light collection systems.
We study the stability of three types of popularly employed TPB coatings under immersion in liquid argon. TPB emanation from each coating is quantified by fluorescence assay of molecular sieve filter material after a prolonged soak time. Two of the coatings are shown to emanate a detectable concentration of TPB into argon over a 24 hour period, which corresponds to tens of parts per billion in argon by mass. In an independent setup, the dissolved or suspended TPB is shown to produce a wavelength shifting effect in the argon bulk. Interpretations of these results and implications for present and future liquid argon time projection chamber experiments are discussed.
The Mu2e experiment will search for a neutrino-less muon-to-electron conversion process with almost four orders of magnitude of sensitivity improvement relative to the current best limit. One important background is caused by cosmic ray muons, and particles produced by their decay or interactions, mimicking the conversion electron signature. In order to reach the design sensitivity, Mu2e needs to obtain a cosmic ray veto (CRV) efficiency of 99.99%. The CRV system consists of four layers of plastic scintillating counters read out by silicon photo-multipliers (SiPM) through wavelength shifting fibers. The CRV counters must produce sufficient photo statistics in order to achieve the required veto efficiency. We study the light properties of several wavelength shifting fiber sizes in order to optimize the total light yield for the CRV system. The measurements are performed using a scanner designed to ensure fiber quality for the CRV.
Based on test-beam measurements, we study the response of a liquid-scintillator detector equipped with wavelength-shifting optical modules, that are proposed e.g. for the IceCube experiment and the SHiP experiment, and adiabatic light guides that are viewed either by a photomultiplier tube or by an array of silicon photomultipliers. We report on the efficiency, the time resolution and the detector response to different particle types and point out potential ways to improve the detector performance.
Cherenkov detectors employ various methods to maximize light collection at the photomultiplier tubes (PMTs). These generally involve the use of highly reflective materials lining the interior of the detector, reflective materials around the PMTs, or wavelength-shifting sheets around the PMTs. Recently, the use of water-soluble wavelength-shifters has been explored to increase the measurable light yield of Cherenkov radiation in water. These wave-shifting chemicals are capable of absorbing light in the ultravoilet and re-emitting the light in a range detectable by PMTs. Using a 250 L water Cherenkov detector, we have characterized the increase in light yield from three compounds in water: 4-Methylumbelliferone, Carbostyril-124, and Amino-G Salt. We report the gain in PMT response at a concentration of 1 ppm as: 1.88 $pm$ 0.02 for 4-Methylumbelliferone, stable to within 0.5% over 50 days, 1.37 $pm$ 0.03 for Carbostyril-124, and 1.20 $pm$ 0.02 for Amino-G Salt. The response of 4-Methylumbelliferone was modeled, resulting in a simulated gain within 9% of the experimental gain at 1 ppm concentration. Finally, we report an increase in neutron detection performance of a large-scale (3.5 kL) gadolinium-doped water Cherenkov detector at a 4-Methylumbelliferone concentration of 1 ppm.
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