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Magnetism, superconductivity and coupling in cuprate heterostructures probed by low-energy muon-spin rotation

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 Added by Bastian M. Wojek
 Publication date 2011
  fields Physics
and research's language is English




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We present a low-energy muon-spin-rotation study of the magnetic and superconducting properties of YBa2Cu3O7/PrBa2Cu3O7 trilayer and bilayer heterostructures. By determining the magnetic-field profiles throughout these structures we show that a finite superfluid density can be induced in otherwise semiconducting PrBa2Cu3O7 layers when juxtaposed to YBa2Cu3O7 electrodes while the intrinsic antiferromagnetic order is unaffected.



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We report a detailed $mu$SR study of the pressure evolution of the magnetic order in the manganese based pnictide MnP, which has been recently found to undergo a superconducting transition under pressure once the magnetic ground state is suppressed. Using the muon as a volume sensitive local magnetic probe, we identify a ferromagnetic state as well as two incommensurate helical states (with propagation vectors ${bf Q}$ aligned along the crystallographic $c-$ and $b-$directions, respectively) which transform into each other through first order phase transitions as a function of pressure and temperature. Our data appear to support that the magnetic state from which superconductivity develops at higher pressures is an incommensurate helical phase.
We report muon-spin relaxation measurements on SrFeAsF, which is the parent compound of a newly discovered iron-arsenic-fluoride based series of superconducting materials. We find that this material has very similar magnetic properties to LaFeAsO, such as separated magnetic and structural transitions (TN = 120 K, Ts = 175 K), contrasting with SrFe2As2 where they are coincident. The muon oscillation frequencies fall away very sharply at TN, which suggests that the magnetic exchange between the layers is weaker than in comparable oxypnictide compounds. This is consistent with our specific heat measurements, which find that the entropy change S = 0.05 J/mol/K largely occurs at the structural transition and there is no anomaly at TN.
The magnetic response of CaK(Fe$_{0.949}$Ni$_{0.051}$)$_4$As$_4$ was investigated by means of the muon-spin rotation/relaxation. The long-range commensurate magnetic order sets in below the N{e}el temperature $T_{rm N}= 50.0(5)$~K. The density-functional theory calculations have identified three possible muon stopping sites. The experimental data were found to be consistent with only one type of magnetic structure, namely, the long-range magnetic spin-vortex-crystal order with the hedgehog motif within the $ab-$plane and the antiferromagnetic stacking along the $c-$direction. The value of the ordered magnetic moment at $Tapprox3$ K was estimated to be $m_{rm Fe}=0.38(11)$ $mu_{rm B}$ ($mu_{rm B}$ is the Bohr magneton). A microscopic coexistence of magnetic and superconducting phases accompanied by a reduction of the magnetic order parameter below the superconducting transition temperature $T_{rm c}simeq 9$ K is observed. Comparison with 11, 122, and 1144 families of Fe-based pnictides points to existence of correlation between the reduction of the magnetic order parameter at $Trightarrow 0$ and the ratio of the transition temperatures $T_{rm c}/T_{rm N}$. Such correlations were found to be described by Machidas model for coexistence of itinerant spin-density wave magnetism and superconductivity [Machida, J. Phys. Soc. Jpn. 50, 2195 (1981) and Budko et al., Phys. Rev. B 98, 144520 (2018)].
The Pr-rich end of the alloy series Pr$_{1-x}$Nd$_x$Os$_4$Sb$_{12}$ has been studied using muon spin rotation and relaxation. The end compound PrOs$_4$Sb$_{12}$ is an unconventional heavy-fermion superconductor, which exhibits a spontaneous magnetic field in the superconducting phase associated with broken time-reversal symmetry. No spontaneous field is observed in the Nd-doped alloys for x $>$ 0.05. The superfluid density is insensitive to Nd concentration, and no Nd$^{3+}$ static magnetism is found down to the lowest temperatures of measurement. Together with the slow suppression of the superconducting transition temperature with Nd doping, these results suggest anomalously weak coupling between Nd spins and conduction-band states.
The recent observation of superconductivity with critical temperatures up to 55 K in the FeAs based pnictide compounds marks the first discovery of a non copper-oxide based layered high-Tc superconductor (HTSC) [1-3]. It has raised the suspicion that these new materials share a similar pairing mechanism to the cuprates, since both exhibit superconductivity following charge doping of a magnetic parent material. Here we present a muon spin rotation study on SmFeAsO1-xFx (x=0-0.30), which shows that static magnetism persists well into the superconducting regime. The analogy with the cuprates is quite surprising since the parent compounds appear to have different magnetic ground states: itinerant spin density wave for the pnictides contrasted with the Mott-Hubbard insulator in the cuprates. Our findings suggest that proximity to magnetic order and associated soft magnetic fluctuations, rather than the strong electronic correlations in the vicinity of a Mott-Hubbard-metal-to-insulator transition, may be the key ingredients of HTSC.
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