No Arabic abstract
The current emission noise of a carbon nanotube quantum dot in the Kondo regime is measured at frequencies $ u$ of the order or higher than the frequency associated with the Kondo effect $k_B T_K/h$, with $T_K$ the Kondo temperature. The carbon nanotube is coupled via an on-chip resonant circuit to a quantum noise detector, a superconductor-insulator-superconductor junction. We find for $h u approx k_B T_K$ a Kondo effect related singularity at a voltage bias $eV approx h u $, and a strong reduction of this singularity for $h u approx 3 k_B T_K$, in good agreement with theory. Our experiment constitutes a new original tool for the investigation of the non-equilibrium dynamics of many-body phenomena in nanoscale devices.
We investigate a tunable two-impurity Kondo system in a strongly correlated carbon nanotube double quantum dot, accessing the full range of charge regimes. In the regime where both dots contain an unpaired electron, the system approaches the two-impurity Kondo model. At zero magnetic field the interdot coupling disrupts the Kondo physics and a local singlet state arises, but we are able to tune the crossover to a Kondo screened phase by application of a magnetic field. All results show good agreement with a numerical renormalization group study of the device.
Illumination of atoms by resonant lasers can pump electrons into a coherent superposition of hyperfine levels which can no longer absorb the light. Such superposition is known as dark state, because fluorescent light emission is then suppressed. Here we report an all-electric analogue of this destructive interference effect in a carbon nanotube quantum dot. The dark states are a coherent superposition of valley (angular momentum) states which are decoupled from either the drain or the source leads. Their emergence is visible in asymmetric current-voltage characteristics, with missing current steps and current suppression which depend on the polarity of the applied source-drain bias. Our results demonstrate for the first time coherent-population trapping by all-electric means in an artificial atom.
Most of the time, electronic excitations in mesoscopic conductors are well described, around equilibrium, by non-interacting Landau quasi-particles. This allows a good understanding of the transport properties in the linear regime. However, the role of interaction in the non-equilibrium properties beyond this regime has still to be established. A paradigmatic example is the Kondo many body state, which can be realized in a carbon nanotube (CNT) quantum dot for temperatures below the Kondo temperature $T_K$. As CNT possess spin and orbital quantum numbers, it is possible to investigate the twofold degenerate SU(2) Kondo effect as well as the four fold degenerate SU(4) state by tuning the degeneracies and filling factor. This article aims at providing a comprehensive review on our recent works on the Kondo correlations probed by quantum noise measurement both at low and high frequencies and demonstrate how current noise measurements yield new insight on interaction effects and dynamics of a Kondo correlated state.
We systematically study the coupling of longitudinal modes (shells) in a carbon nanotube quantum dot. Inelastic cotunneling spectroscopy is used to probe the excitation spectrum in parallel, perpendicular and rotating magnetic fields. The data is compared to a theoretical model including coupling between shells, induced by atomically sharp disorder in the nanotube. The calculated excitation spectra show good correspondence with experimental data.
We study the Kondo effect in a CNT(left lead)-CNT(QD)-CNT(right lead) structure. Here CNT is a single-wall metallic carbon nanotube, for which 1) the valence and conduction bands of electrons with zero orbital angular momentum ($m=0$) coalesc at the two valley points ${bf{K}}$ and ${bf{K}}$ of the first Brillouin zone and 2) the energy spectrum of electrons with $m e 0$ has a gap whose size is proportional to $|m|$. Following adsorption of hydrogen atoms and application of an appropriately designed gate potential, electron energy levels in the CNT(QD) are tunable to have: 1) two-fold spin degeneracy; 2) two-fold isospin (valley) degeneracy; 3) three-fold orbital degeneracy $m=0,pm1$. As a result, an SU(12) Kondo effect is realized with remarkably high Kondo temperature. Unlike the SU(2) case, the low temperature conductance and magnetic susceptibility have a peak at finite temperature. Moreover, the magnetic susceptibilities for parallel and perpendicular magnetic fields (WRT the tube axis) display anisotropy with a universal ratio $chi_{rm{imp}}^parallel / chi_{rm{imp}}^perp=eta$ that depends only on the electrons orbital and spin $g$ factors.