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Production and characterization of a custom-made 228Th source with reduced neutron source strength for the Borexino experiment

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 Added by Werner Maneschg
 Publication date 2011
  fields Physics
and research's language is English




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A custom-made 228Th source of several MBq activity was produced for the Borexino experiment for studying the external background of the detector. The aim was to reduce the unwanted neutron emission produced via (alpha,n) reactions in ceramics used typically for commercial 228Th sources. For this purpose a ThCl4 solution was converted chemically into ThO2 and embedded into a gold foil. The paper describes the production and the characterization of the custom-made source by means of gamma-activity, dose rate and neutron source strength measurements. From gamma-spectroscopic measurements it was deduced that the activity transfer from the initial solution to the final source was >91% (at 68% C.L.) and the final activity was (5.41+-0.30) MBq. The dose rate was measured by two dosimeters yielding 12.1 mSv/h and 14.3 mSv/h in 1 cm distance. The neutron source strength of the 5.41 MBq 228Th source was determined as (6.59+-0.85)/sec.



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The GERDA experiment at the Laboratori Nazionali del Gran Sasso (LNGS) searches for the neutrinoless double beta decay of 76-Ge. In view of the GERDA Phase II data collection, four new 228-Th radioactive sources for the calibration of the germanium detectors enriched in 76-Ge have been produced with a new technique, leading to a reduced neutron flux from ( alpha; n ) reactions. The gamma activities of the sources were determined with a total uncertainty of 4 percent using an ultra-low background HPGe detector operated underground at LNGS. The emitted neutron flux was determined using a low background LiI(Eu) detector and a 3-He counter at LNGS. In both cases, a reduction of about one order of magnitude with respect to commercially available 228-Th sources was obtained. Additionally, a specific leak test with a sensitivity to leaks down to 10 mBq was developed to investigate the tightness of the stainless steel capsules housing the sources after their use in cryogenic environment.
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