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Register a new userMagnetic phase transitions and magnetoelectric coupling of GdFeO_3 single crystals probed by low-temperature heat transport
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The low-temperature thermal conductivity (kappa) of GdFeO_3 single crystals is found to be strongly dependent on magnetic field. The low-field kappa (H) curves show two dips for H parallel a and only one dip for H parallel c, with the characteristic fields having good correspondence with the spin-flop and the spin-polarization transitions. A remarkable phenomenon is that the subKelvin thermal conductivity shows hysteretic behaviors on the history of applying magnetic field, that is, the kappa(H) isotherms measured with field increasing are larger than those with field decreasing. Intriguingly, the broad region of magnetic field (sim 0--3 T) showing the irreversibility of heat transport coincides with that presenting the ferroelectricity. It is discussed that the irreversible kappa(H) behaviors are due to the phonon scattering by ferroelectric domain walls. This result shows an experimental feature that points to the capability of controlling the ferroelectric domain structures by magnetic field in multiferroic materials.
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We study the low-temperature heat transport, as well as the magnetization and the specific heat, of TmMnO_3 single crystals to probe the transitions of magnetic structure induced by magnetic field. It is found that the low-T thermal conductivity (kappa) shows strong magnetic-field dependence and the overall behaviors can be understood in the scenario of magnetic scattering on phonons. In addition, a strong dip-like feature shows up in kappa(H) isotherms at 3.5--4 T for H parallel c, which is related to a known spin re-orientation of Mn^{3+} moments. The absence of this phenomenon for H parallel a indicates that the magnetic-structure transition of TmMnO_3 cannot be driven by the in-plane field. In comparison, the magnetothermal conductivity of TmMnO_3 is much larger than that of YMnO_3 but smaller than that of HoMnO_3, indicating that the magnetisms of rare-earth ions are playing the key role in the spin-phonon coupling of the hexagonal manganites.
We propose a phase diagram for FexBi2Te3 (0 < x < 0.1) single crystals, which belong to a class of magnetically bulk-doped topological insulators. The evolution of magnetic correlations from ferromagnetic- to antiferromagnetic- gives rise to topological phase transitions, where the paramagnetic topological insulator of Bi2Te3 turns into a band insulator with ferromagnetic-cluster glassy behaviours around x ~ 0.025, and it further evolves to a topological insulator with valence-bond glassy behaviours, which spans over the region between x ~ 0.03 up to x ~ 0.1. This phase diagram is verified by measuring magnetization, magnetotransport, and angle-resolved photoemission spectra with theoretical discussions.
Electrical transport and specific heat properties of Nd_{1-x}Pb_{x}MnO_{3} single crystals for 0.15 < x 0.5 have been studied in low temperature regime. The resistivity in the ferromagnetic insulating (FMI) phase for x < 0.3 has an activated character. The dependence of the activation gap Delta on doping x has been determined and the critical concentration for the zero-temperature metal-insulator transition was determined as x_{c} ~ 0.33. For a metallic sample with x=0.42, a conventional electron-electron (e-e) scattering term proportional T^{2} is found in the low-temperature electrical resistivity, although the Kadowaki-Woods ratio is found to be much larger for this manganite than for a normal metal. For a metallic sample with x=0.5, a resistivity minimum is observed for x= 0.5. The effect is attributed to weak localization and can be described by a negative T^{1/2} weak-localization contribution to resistivity for a disordered three-dimensional electron system. The specific heat data have been fitted to contributions from free electrons (gamma), spin excitations (beta_{3/2}), lattice and a Schottky-like anomaly related to the rare-earth magnetism of the Nd ions. The value of gamma is larger than for normal metals, which is ascribed to magnetic ordering effects involving Nd. Also, the Schottky-like anomaly appears broadened and weakened suggesting inhomogeneous molecular fields at the Nd-sites.
Magnetic phase transitions in multiferroic bismuth ferrite (BiFeO3) induced by magnetic field, epitaxial strain, and composition modification are considered. These transitions from a spatially modulated spin spiral state to a homogenous antiferromagnetic one are accompanied by the release of latent magnetization and a linear magnetoelectric effect that makes BiFeO3-based materials efficient room-temperature single phase multiferroics.
We report a study on the thermal conductivity of CuFe$_{1-x}$Ga$_x$O$_2$ ($x =$ 0--0.12) single crystals at temperatures down to 0.3 K and in magnetic fields up to 14 T. CuFeO$_2$ is a well-known geometrically frustrated triangular lattice antiferromagnet and can be made to display multiferroicity either by applying magnetic field along the $c$ axis or by doping nonmagnetic impurities, accompanied with rich behaviors of magnetic phase transitions. The main experimental findings of this work are: (i) the thermal conductivities ($kappa_a$ and $kappa_c$) show drastic anomalies at temperature- or field-induced magnetic transitions; (ii) the low-$T$ $kappa(H)$ isotherms exhibit irreversibility in a broad region of magnetic fields; (iii) there are phonon scattering effect caused by magnetic fluctuations at very low temperatures. These results demonstrate strong spin-phonon coupling in this material and reveal the non-negligible magnetic fluctuations in the ground state of pure and Ga-doped samples.
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