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Register a new userUnusual signatures of the ferromagnetic transition in the heavy Fermion compound UMn$_2$Al$_{20}$
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Magnetic susceptibility results for single crystals of the new cubic compounds UT$_2$Al$_{20}$ (T=Mn, V, and Mo) are reported. Magnetization, specific heat, resistivity, and neutron diffraction results for a single crystal and neutron diffraction and inelastic spectra for a powder sample are reported for UMn$_2$Al$_{20}$. For T = V and Mo, temperature independent Pauli paramagnetism is observed. For UMn$_2$Al$_{20}$, a ferromagnetic transition is observed in the magnetic susceptibility at $T_c$ = 20 K. The specific heat anomaly at $T_c$ is very weak while no anomaly in the resistivity is seen at $T_c$. We discuss two possible origins for this behavior of UMn$_2$Al$_{20}$: moderately small moment itinerant ferromagnetism, or induced local moment ferromagnetism.
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Inelastic neutron scattering experiments on poly crystalline sample of heavy-fermion compound YbCo$_2$Zn$_{20}$ were carried out in order to obtain microscopic insights on the ground state and its magnetic field response. At zero field at 300 mK, inelastic response consists of two features: quasielastic scattering and a sharp peak at 0.6 meV. With increasing temperature, a broad peak comes up around 2.1 meV, whereas quasielastic response gets broader and the peak at 0.6 meV becomes unclear. By applying magnetic field, the quasielastic response exhibits significant broadening above 1 T, and the peak at 0.6 meV is obscure under fields. The peaks in inelastic spectra and its temperature variation can be ascribed to the suggested crystal-field model of ${{Gamma}_6}$ - ${{Gamma}_8}$ - ${{Gamma}_7}$ with the overall splitting of less than 3 meV. The observed quasielastic response and its rapid broadening with magnetic field indicates that the heavy-electron state arises from the ground state doublets, and are strongly suppressed by external field in YbCo$_2$Zn$_{20}$.
We present results from point-contact spectroscopy of the antiferromagnetic heavy-fermion superconductor UPd$_2$Al$_3$: conductance spectra are taken from single crystals with two major surface orientations as a function of temperature and magnetic field, and analyzed using a theory of co-tunneling into an Anderson lattice. Spectroscopic signatures are clearly identified including the distinct asymmetric double-peak structure arising from the opening of a hybridization gap when a coherent heavy Fermi liquid is formed. Both the hybridization gap, found to be 7.2 $pm$ 0.3 meV at 4 K, and the conductance enhancement above a flat background decrease upon increasing temperature. While the hybridization gap is extrapolated to remain finite up to $sim$28 K, close to the temperature around which the magnetic susceptibility displays a broad peak, the conductance enhancement vanishes at $sim$18 K, slightly above the antiferromagnetic transition temperature ($T_textrm{N}$ $approx$ 14 K). This rapid decrease of the conductance enhancement is understood as a consequence of the junction drifting away from the ballistic regime due to increased scattering off magnons associated with the localized U 5$f$ electrons. This shows that while the hybridization gap opening is not directly associated with the antiferromagnetic ordering, its visibility in the conductance is greatly affected by the temperature-dependent magnetic excitations. Our findings are not only consistent with the 5$f$ dual-nature picture in the literature but also shed new light on the interplay between the itinerant and localized electrons in UPd$_2$Al$_3$.
We report a comprehensive investigation of the lattice dynamics of URu$_2$Si$_2$ as a function of temperature using Raman scattering, optical conductivity and inelastic neutron scattering measurements as well as theoretical {it ab initio} calculations. The main effects on the optical phonon modes are related to Kondo physics. The B$_{1g}$ ($Gamma_3$ symmetry) phonon mode slightly softens below $sim$100~K, in connection with the previously reported softening of the elastic constant, $C_{11}-C_{12}$, of the same symmetry, both observations suggesting a B$_{1g}$ symmetry-breaking instability in the Kondo regime. Through optical conductivity, we detect clear signatures of strong electron-phonon coupling, with temperature dependent spectral weight and Fano line shape of some phonon modes. Surprisingly, the line shapes of two phonon modes, E$_u$(1) and A$_{2u}$(2), show opposite temperature dependencies. The A$_{2u}$(2) mode loses its Fano shape below 150 K, whereas the E$_u$(1) mode acquires it below 100~K, in the Kondo cross-over regime. This may point out to momentum-dependent Kondo physics. By inelastic neutron scattering measurements, we have drawn the full dispersion of the phonon modes between 300~K and 2~K. No remarkable temperature dependence has been obtained including through the hidden order transition. {it Ab initio} calculations with the spin-orbit coupling are in good agreement with the data except for a few low energy branches with propagation in the (a,b) plane.
We report the discovery of giant and anisotropic magnetoresistance due to the orbital rearrangement in a non-magnetic correlated metal. In particular, we measured the magnetoresistance under fields up to 31.4 T in the cubic Pr-based heavy fermion superconductor PrV$_2$Al$_{20}$ with a non-magnetic $Gamma _3$ doublet ground state, exhibiting antiferro-quadrupole ordering below 0.7 K. For the [100] direction, we find that the high-field phase appears between 12 T and 25 T, accompanied by a large jump at 12 T in the magnetoresistance ($Delta MR sim $ 100 $% $) and in the anisotropic magnetoresistivity (AMR) ratio by $sim $ 20 $% $. These observations indicate that the strong hybridization between the conduction electrons and anisotropic quadrupole moments leads to the Fermi surface reconstruction upon crossing the field-induced antiferro-quadrupole (orbital) rearrangement.
In the heavy fermion materials, the characteristic energy scales of many exotic strongly correlated phenomena (Kondo effect, magnetic order, superconductivity, etc.) are at milli-electron-volt order, implying that the heavy fermion materials are surface sensitive. Here, we investigate the electronic structures for Si- and Ce-terminated surfaces of CeRh$_2$Si$_2$ by first-principles methods. Our research reveals three notable impacts of surface effects on electronic structures, which are consistent with recent angle-resolved photoemission spectroscopy (ARPES) experiments. Firstly, the relaxation of surface crystal structures changes the relative position of Fermi level, adjusts the dispersion of bands and enhances the Kondo resonance. Secondly, the decrease of the hybridization between the Ce-4$f$ and conduction electrons in the surface layer leads to a weaker Kondo resonance peak and the shift of spin-orbit bands. Thirdly, the variation of crystal electric field around surface Ce atoms affects the splitting of Kondo resonance peaks, and also pushes down the lower-Hubbard bands of surface 4$f$ electrons. Moreover, we find the characteristic of bulks lower-Hubbard bands, which was overlooked in previous works. Our investigation suggests that these surface effects are potentially important and highlighted in the future researches on properties of strongly correlated materials.
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