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Register a new userMeasurement and analysis of the Hall effect of A-Fe$_2$As$_2$ single crystals with A = Ba, Ca or Sr
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We report measurements of the Hall coefficient $R_H$ for single crystals of AFe$_2$As$_2$ with $A = Ba, Ca$ or $Sr$ which are the anti-ferromagnetic parent compounds of some high temperature pnictide superconductors. We show that $R_H$ of Sr-122 is consistent with high field quantum oscillation data. Our $R_H(T)$ data can also be used to estimate values of the spin density wave gap, giving $Delta_{SDW}(0) = 710pm 70$ K for Sr-122 and $435pm 20$ K for Ba-122.
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The detailed optical properties have been determined for the iron-based materials $A$Fe$_2$As$_2$, where $A=,$Ca, Sr, and Ba, for light polarized in the iron-arsenic ($a-b$) planes over a wide frequency range, above and below the magnetic and structural transitions at $T_N =$ 172, 195, and 138 K, respectively. The real and imaginary parts of the complex conductivity are fit simultaneously using two Drude terms in combination with a series of oscillators. Above $T_N$, the free-carrier response consists of a weak, narrow Drude term, and a strong, broad Drude term, both of which show only a weak temperature dependence. Below $T_N$ there is a slight decrease of the plasma frequency but a dramatic drop in the scattering rate for the narrow Drude term, and for the broad Drude term there is a significant decrease in the plasma frequency, while the decrease in the scattering rate, albeit significant, is not as severe. The small values observed for the scattering rates for the narrow Drude term for $Tll{T_N}$ may be related to the Dirac cone-like dispersion of the electronic bands. Below $T_N$ new features emerge in the optical conductivity that are associated with the reconstruction Fermi surface and the gapping of bands at $Delta_1 simeq$ 45 $-$ 80 meV, and $Delta_2 simeq$ 110 $-$ 210 meV. The reduction in the spectral weight associated with the free carriers is captured by the gap structure, specifically, the spectral weight from the narrow Drude term appears to be transferred into the low-energy gap feature, while the missing weight from the broad term shifts to the high-energy gap.
We have studied the electronic and magnetic structures of the ternary iron arsenides AFe$_2$As$_2$ (A = Ba, Ca, or Sr) using the first-principles density functional theory. The ground states of these compounds are in a collinear antiferromagnetic order, resulting from the interplay between the nearest and the next-nearest neighbor superexchange antiferromagnetic interactions bridged by As $4p$ orbitals. The correction from the spin-orbit interaction to the band structure is small. The pressure can reduce dramatically the magnetic moment and diminish the collinear antiferromagnetic order. Based on the calculations, we propose that the low energy dynamics of these materials is described effectively by a $t-J_H-J_1-J_2$-type model.
We have successfully grown high quality single crystals of SrFe$_2$As$_2$ and A$_{0.6}$K$_{0.4}$Fe$_2$As$_2$(A=Sr, Ba) using flux method. The resistivity, specific heat and Hall coefficient have been measured. For parent compound SrFe$_2$As$_2$, an anisotropic resistivity with $rho_c$ / $rho_{ab}$ as large as 130 is obtained at low temperatures. A sharp drop in both in-plane and out-plane resistivity due to the SDW instability is observed below 200 K. The angular dependence of in-plane magnetoresistance shows 2-fold symmetry with field rotating within ab plane below SDW transition temperature. This is consistent with a stripe-type spin ordering in SDW state. In K doped A$_{0.6}$K$_{0.4}$Fe$_2$As$_2$(A=Sr. Ba), the SDW instability is suppressed and the superconductivity appears with T$_c$ above 35 K. The rather low anisotropy in upper critical field between H$parallel$ab and H$parallel$c indicates inter-plane coupling play an important role in hole doped Fe-based superconductors.
We report the synthesis and basic physical properties of single crystals of CaFe2As2, an isostructural compound to BaFe2As2 which has been recently doped to produce superconductivity. CaFe2As2 crystalizes in the ThCr2Si2 structure with lattice parameters a = 3.907(4) A and c = 11.69(2) A. Magnetic susceptibility, resistivity, and heat capacity all show a first order phase transition at T_0 171 K. The magnetic susceptibility is nearly isotropic from 2 K to 350 K. The heat capacity data gives a Sommerfeld coefficient of 8.2 +- 0.3 mJ/molK2, and does not reveal any evidence for the presence of high frequency (> 300 K) optical phonon modes. The Hall coefficient is negative below the transition indicating dominant n-type carriers.
Single crystals of Ba(Fe$_{1-x}$Ru$_x$)$_2$As$_2$, $x<0.37$, have been grown and characterized by structural, magnetic and transport measurements. These measurements show that the structural/magnetic phase transition found in pure BaFe$_2$As$_2$ at 134 K is suppressed monotonically by Ru doping, but, unlike doping with TM=Co, Ni, Cu, Rh or Pd, the coupled transition seen in the parent compound does not detectably split into two separate ones. Superconductivity is stabilized at low temperatures for $x>0.2$ and continues through the highest doping levels we report. The superconducting region is dome like, with maximum T$_c$ ($sim16.5$ K) found around $xsim 0.29$. A phase diagram of temperature versus doping, based on electrical transport and magnetization measurements, has been constructed and compared to those of the Ba(Fe$_{1-x}$TM$_x$)$_2$As$_2$ (TM=Co, Ni, Rh, Pd) series as well as to the temperature-pressure phase diagram for pure BaFe$_2$As$_2$. Suppression of the structural/magnetic phase transition as well as the appearance of superconductivity is much more gradual in Ru doping, as compared to Co, Ni, Rh and Pd doping, and appears to have more in common with BaFe$_2$As$_2$ tuned with pressure; by plotting $T_S/T_m$ and $T_c$ as a function of changes in unit cell dimensions, we find that changed in the $c/a$ ratio, rather than changes in $c$, $a$ or V, unify the $T(p)$ and $T(x)$ phase diagrams for BaFe$_2$As$_2$ and Ba(Fe$_{1-x}$Ru$_x$)$_2$As$_2$ respectively.
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