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Register a new userLoading Stark-decelerated molecules into electrostatic quadrupole traps
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Added by
Sebastiaan Y.T. van de Meerakker
Publication date
2009
fields
Physics
and research's language is
English
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Beams of neutral polar molecules in a low-field seeking quantum state can be slowed down using a Stark decelerator, and can subsequently be loaded and confined in electrostatic quadrupole traps. The efficiency of the trap loading process is determined by the ability to couple the decelerated packet of molecules into the trap without loss of molecules and without heating. We discuss the inherent difficulties to obtain ideal trap loading, and describe and compare different trap loading strategies. A new split-endcap quadrupole trap design is presented that enables improved trap loading efficiencies. This is experimentally verified by comparing the trapping of OH radicals using the conventional and the new quadrupole trap designs.
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Cold, velocity-controlled molecular beams consisting of a single quantum state promise to be a powerful tool for exploring molecular scattering interactions. In recent years, Stark deceleration has emerged as one of the main methods for producing velocity-controlled molecular beams. However, Stark deceleration is shown not to be effective at producing a molecular beam consisting of a single quantum state in many circumstances. Therefore, quantum state purity must be carefully considered when using Stark decelerated beams, particularly in collision experiments where contributions from all quantum states must be addressed.
We produce SO_2 molecules with a centre of mass velocity near zero using a Stark decelerator. Since the initial kinetic energy of the supersonic SO_2 molecular beam is high, and the removed kinetic energy per stage is small, 326 deceleration stages are necessary to bring SO_2 to a complete standstill, significantly more than in other experiments. We show that in such a decelerator possible loss due to coupling between the motional degrees of freedom must be considered. Experimental results are compared with 3D Monte-Carlo simulations and the quantum state selectivity of the Stark decelerator is demonstrated.
Stark deceleration has been utilized for slowing and trapping several species of neutral, ground-state polar molecules generated in a supersonic beam expansion. Due to the finite physical dimension of the electrode array and practical limitations of the applicable electric fields, only molecules within a specific range of velocities and positions can be efficiently slowed and trapped. These constraints result in a restricted phase space acceptance of the decelerator in directions both transverse and parallel to the molecular beam axis; hence, careful modeling is required for understanding and achieving efficient Stark decelerator operation. We present work on slowing of the hydroxyl radical (OH) elucidating the physics controlling the evolution of the molecular phase space packets both with experimental results and model calculations. From these results we deduce experimental conditions necessary for efficient operation of a Stark decelerator.
We report on the Stark deceleration and electrostatic trapping of $^{14}$NH ($a ^1Delta$) radicals. In the trap, the molecules are excited on the spin-forbidden $A ^3Pi leftarrow a ^1Delta$ transition and detected via their subsequent fluorescence to the $X ^3Sigma^-$ ground state. The 1/e trapping time is 1.4 $pm$ 0.1 s, from which a lower limit of 2.7 s for the radiative lifetime of the $a ^1Delta, v=0,J=2$ state is deduced. The spectral profile of the molecules in the trapping field is measured to probe their spatial distribution. Electrostatic trapping of metastable NH followed by optical pumping of the trapped molecules to the electronic ground state is an important step towards accumulation of these radicals in a magnetic trap.
We present an effective and fast (few microseconds) procedure for transferring ultra-cold atoms from the ground state in a harmonic trap into the desired bands of an optical lattice. Our shortcut method is a designed pulse sequence where the time duration and the interval in each step are fully optimized in order to maximize robustness and fidelity of the final state with respect to the target state. The atoms can be prepared in a single band with even or odd parity, and superposition states of different bands can be prepared and manipulated. Furthermore, we extend this idea to the case of two-dimensional or three-dimensional optical lattices where the energies of excited states are degenerate. We experimentally demonstrate various examples and show very good agreement with the theoretical model. Efficient shortcut methods will find applications in the preparation of quantum systems, in quantum information processing, in precise measurement and as a starting point to investigate dynamics in excited bands.
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